Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4

Ma, Qianli; Rule, Kirrily C.; Cronkwright, Zachary W.; Dragomir, Mirela; Mitchell, Gabrielle; Smith, Evan M.; Chi, Songxue; Kolesnikov, Alexander I.; Stone, Matthew B.; Gaulin, Bruce D.

doi:10.1103/PhysRevResearch.3.023151

Title: Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$

Abstract

Three-dimensional, commensurate long-range magnetic order in La₂CuO₄ quickly evolves to quasi-two-dimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La_2-xSr_x/Ba_xCuO₄ family of superconductors. The onset of superconductivity in these systems is known to be coincident with a remarkable rotation of the incommensurate spin order from “diagonal stripes” below x = 0.05 to “parallel stripes” above. However, little is known about the spin correlations at optimal and high doping levels, around and beyond the proposed quantum critical point for the pseudogap phase, p*. Here, we present elastic and inelastic neutron scattering measurements on single crystals of La_1.6-xNd_0.4Sr_xCuO₄ with x = 0.125, 0.19, 0.24, and 0.26 and show that two-dimensional, quasistatic, parallel spin stripes have an onset at temperatures such that the parallel spin stripe phase extends beyond p* and envelops the entirety of superconducting ground states in this system. We also show that the elastic order parameter for parallel spin stripes at optimum doping, x = 0.19, displays an inflection point at superconducting T_c, while the low-energy dynamic spectral weight of parallel stripe fluctuations grows with decreasing temperature and saturates below T_c.

Authors:

;

; Cronkwright, Zachary W.;

; Mitchell, Gabrielle;

; Chi, Songxue;

;

; Gaulin, Bruce D.

Publication Date:: Thu May 27 00:00:00 EDT 2021

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1785038

Alternate Identifier(s):: OSTI ID: 1856684

Grant/Contract Number:: AC05-00OR22725

Resource Type:: Published Article

Journal Name:: Physical Review Research

Additional Journal Information:: Journal Name: Physical Review Research Journal Volume: 3 Journal Issue: 2; Journal ID: ISSN 2643-1564

Publisher:: American Physical Society

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; superconductivity; cuprates; high-temperature superconductors; neutron scattering

Citation Formats


                    Ma, Qianli, Rule, Kirrily C., Cronkwright, Zachary W., Dragomir, Mirela, Mitchell, Gabrielle, Smith, Evan M., Chi, Songxue, Kolesnikov, Alexander I., Stone, Matthew B., and Gaulin, Bruce D. Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4.  United States: N. p., 2021. 
Web.  doi:10.1103/PhysRevResearch.3.023151.

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                    Ma, Qianli, Rule, Kirrily C., Cronkwright, Zachary W., Dragomir, Mirela, Mitchell, Gabrielle, Smith, Evan M., Chi, Songxue, Kolesnikov, Alexander I., Stone, Matthew B., & Gaulin, Bruce D. Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4.  United States.  https://doi.org/10.1103/PhysRevResearch.3.023151

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                    Ma, Qianli, Rule, Kirrily C., Cronkwright, Zachary W., Dragomir, Mirela, Mitchell, Gabrielle, Smith, Evan M., Chi, Songxue, Kolesnikov, Alexander I., Stone, Matthew B., and Gaulin, Bruce D. Thu .  
"Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4".  United States.  https://doi.org/10.1103/PhysRevResearch.3.023151.

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@article{osti_1785038,

  title        = {Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4},

  author       = {Ma, Qianli and Rule, Kirrily C. and Cronkwright, Zachary W. and Dragomir, Mirela and Mitchell, Gabrielle and Smith, Evan M. and Chi, Songxue and Kolesnikov, Alexander I. and Stone, Matthew B. and Gaulin, Bruce D.},

  abstractNote = {Three-dimensional, commensurate long-range magnetic order in La2CuO4 quickly evolves to quasi-two-dimensional, incommensurate correlations upon doping with mobile holes, and superconductivity follows for x as small as 0.05 in the La2-xSrx/BaxCuO4 family of superconductors. The onset of superconductivity in these systems is known to be coincident with a remarkable rotation of the incommensurate spin order from “diagonal stripes” below x = 0.05 to “parallel stripes” above. However, little is known about the spin correlations at optimal and high doping levels, around and beyond the proposed quantum critical point for the pseudogap phase, p*. Here, we present elastic and inelastic neutron scattering measurements on single crystals of La1.6-xNd0.4SrxCuO4 with x = 0.125, 0.19, 0.24, and 0.26 and show that two-dimensional, quasistatic, parallel spin stripes have an onset at temperatures such that the parallel spin stripe phase extends beyond p* and envelops the entirety of superconducting ground states in this system. We also show that the elastic order parameter for parallel spin stripes at optimum doping, x = 0.19, displays an inflection point at superconducting Tc, while the low-energy dynamic spectral weight of parallel stripe fluctuations grows with decreasing temperature and saturates below Tc.},

  doi          = {10.1103/PhysRevResearch.3.023151},

  journal      = {Physical Review Research},

  number       = 2,

  volume       = 3,

  place        = {United States},

  year         = {Thu May 27 00:00:00 EDT 2021},

  month        = {Thu May 27 00:00:00 EDT 2021}

}

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Title: Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in La 1.6 − x Nd 0.4 Sr x CuO 4

Abstract

Citation Formats

The Remarkable Underlying Ground States of Cuprate Superconductors journal, March 2019

Magnetic excitations in pure, lightly doped, and weakly metallic La 2 CuO 4 journal, December 1992

Staggered magnetization in La 2 − x Sr x CuO 4 from La 139 NQR and μSR: Effects of Sr doping in the range 0< x <0.02 journal, September 1995

SEQUOIA: A Newly Operating Chopper Spectrometer at the SNS journal, November 2010

Glassy nature of stripe ordering in La 1.6 − x Nd 0.4 Sr x CuO 4 journal, June 1999

Doping dependence of the spatially modulated dynamical spin correlations and the superconducting-transition temperature in La 2 − x Sr x CuO 4 journal, March 1998

Direct observation of a one-dimensional static spin modulation in insulating La 1.95 Sr 0.05 CuO 4 journal, February 2000

Materials preparation, single-crystal growth, and the phase diagram of the cuprate high-temperature superconductor La 1.6 − x Nd 0.4 Sr x Cu O 4 journal, November 2020

Spin-gap proximity effect mechanism of high-temperature superconductivity journal, September 1997

Superconductor-to-nonsuperconductor transition in ( La 1 − x Sr x ) 2 CuO 4 as investigated by transport and magnetic measurements journal, August 1989

Superconductivity at 93 K in a new mixed-phase Y-Ba-Cu-O compound system at ambient pressure journal, March 1987

Coexistence of, and Competition between, Superconductivity and Charge-Stripe Order in La 1 . 6 − x Nd 0.4 Sr x CuO 4 journal, January 1997

Diagonal and collinear incommensurate spin structures in underdoped La 2 − x Ba x CuO 4 journal, September 2008

Competing States in the t - J Model: Uniform d -Wave State versus Stripe State journal, July 2014

Two-dimensional incommensurate and three-dimensional commensurate magnetic order and fluctuations in La 2 − x Ba x CuO 4 journal, July 2013

Observation of modulated magnetic long-range order in La 1.88 Sr 0.12 CuO 4 journal, February 1998

Glassy low-energy spin fluctuations and anisotropy gap in La 1.88 Sr 0.12 CuO 4 journal, April 2013

Effective Hamiltonian for the superconducting Cu oxides journal, March 1988

Complete absence of isotope effect in Y Ba 2 Cu 3 O 7 : Consequences for phonon-mediated superconductivity journal, September 1987

Local Magnetic Order vs Superconductivity in a Layered Cuprate journal, August 2000

Theory of high- T c superconductivity in oxides journal, June 1987

Magnetic, transport, and optical properties of monolayer copper oxides journal, July 1998

Systematic 63 Cu NQR study of the stripe phase in La 1.6 − x Nd 0.4 Sr x CuO 4 for 0.07 <~ x <~ 0.25 journal, December 1999

The Resonating Valence Bond State in La2CuO4 and Superconductivity journal, March 1987

Muon spin relaxation study of the stripe phase order in La 1.6 − x Nd 0.4 Sr x CuO 4 and related 214 cuprates journal, October 1998

Structural instabilities in lanthanum cuprate superconductors journal, April 1994

Evidence for stripe correlations of spins and holes in copper oxide superconductors journal, June 1995

Spin-bag mechanism of high-temperature superconductivity journal, March 1988

Stripe order in superconducting La 2 − x Ba x CuO 4 ( 0 . 095 ⩽ x ⩽ 0 . 155 ) journal, March 2011

Scale-invariant magnetoresistance in a cuprate superconductor journal, August 2018

Linear temperature dependence of resistivity and change in the Fermi surface at the pseudogap critical point of a high-Tc superconductor journal, November 2008

Possible highT c superconductivity in the Ba?La?Cu?O system journal, June 1986

Stripe order, depinning, and fluctuations in La 1.875 Ba 0.125 CuO 4 and La 1.875 Ba 0.075 Sr 0.050 CuO 4 journal, September 2004

High- T c Superconductivity and Antiferromagnetism in Multilayered Copper Oxides –A New Paradigm of Superconducting Mechanism– journal, January 2012

From quantum matter to high-temperature superconductivity in copper oxides journal, February 2015

The physics of quantum materials journal, October 2017

Neutron-scattering study of stripe-phase order of holes and spins in La 1.48 Nd 0.4 Sr 0.12 CuO 4 journal, September 1996

Incommensurate spin ordering and fluctuations in underdoped La 2 − x Ba x CuO 4 journal, June 2008

Thermodynamic signatures of quantum criticality in cuprate superconductors journal, February 2019

Charge density waves in cuprate superconductors beyond the critical doping journal, March 2021

Interplay of electron–phonon interaction and strong correlations: the possible way to high-temperature superconductivity journal, November 2000

Charge density wave fluctuations in La 2 − x Sr x CuO 4 and their competition with superconductivity journal, June 2014

Hidden Quantum Spin-Gap State in the Static Stripe Phase of High-Temperature La 2 − x Sr x CuO 4 Superconductors journal, January 2009

Hidden magnetism at the pseudogap critical point of a cuprate superconductor journal, July 2020

Magnetic phase diagram of lightly doped La 2 − x Sr x CuO 4 from La 139 nuclear quadrupole resonance journal, October 1993

Glassy slowing of stripe modulation in ( L a , E u , N d ) 2 − x ( S r , B a ) x CuO 4 : A 63 Cu and 139 La NQR study down to 350 mK journal, September 2001

Superexchange mechanism and d -wave superconductivity journal, September 1988

Rotated stripe order and its competition with superconductivity in La 1.88 Sr 0.12 CuO 4 journal, September 2014

Diagonal static spin correlation in the low-temperature orthorhombic Pccn phase of La 1.55 Nd 0.4 Sr 0.05 CuO 4 journal, October 2001

Doping a Mott insulator: Physics of high-temperature superconductivity journal, January 2006

Scattering and Pairing in Cuprate Superconductors journal, August 2010

Structural phase transformations and superconductivity in La 2 − x Ba x CuO 4 journal, June 1989

Observation of incommensurate magnetic correlations at the lower critical concentration for superconductivity in La 2 − x Sr x CuO 4 ( x = 0.05 ) journal, July 1999

Antiferromagnetism and Its Relation to the Superconducting Phases of UP t 3 journal, August 1995

Coupling between Magnetic and Superconducting Order Parameters and Evidence for the Spin Excitation Gap in the Superconducting State of a Heavy Fermion Superconductor UPd 2 Al 3 journal, September 1997

A common thread: The pairing interaction for unconventional superconductors journal, October 2012

Phase Separation and Finite Size Scaling inLa 2 − x Sr x CuO 4 + δ [0⩽(x,γ)⩽0.03] journal, January 1993

Title: Parallel spin stripes and their coexistence with superconducting ground states at optimal and high doping in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$

The Remarkable Underlying Ground States of Cuprate Superconductors
journal, March 2019

Magnetic excitations in pure, lightly doped, and weakly metallic ${La}_{2}$ ${CuO}_{4}$
journal, December 1992

Staggered magnetization in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ from ${}^{139}{La}$ NQR and μSR: Effects of Sr doping in the range 0< x <0.02
journal, September 1995

SEQUOIA: A Newly Operating Chopper Spectrometer at the SNS
journal, November 2010

Glassy nature of stripe ordering in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$
journal, June 1999

Doping dependence of the spatially modulated dynamical spin correlations and the superconducting-transition temperature in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$
journal, March 1998

Direct observation of a one-dimensional static spin modulation in insulating ${La}_{1.95} {Sr}_{0.05} {CuO}_{4}$
journal, February 2000

Materials preparation, single-crystal growth, and the phase diagram of the cuprate high-temperature superconductor ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} Cu O_{4}$
journal, November 2020

Spin-gap proximity effect mechanism of high-temperature superconductivity
journal, September 1997

Superconductor-to-nonsuperconductor transition in ( ${La}_{1 - x}$ ${Sr}_{x}$ $)_{2}$ ${CuO}_{4}$ as investigated by transport and magnetic measurements
journal, August 1989

Superconductivity at 93 K in a new mixed-phase Y-Ba-Cu-O compound system at ambient pressure
journal, March 1987

Coexistence of, and Competition between, Superconductivity and Charge-Stripe Order in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$
journal, January 1997

Diagonal and collinear incommensurate spin structures in underdoped ${La}_{2 - x} {Ba}_{x} {CuO}_{4}$
journal, September 2008

Competing States in the $t$ - $J$ Model: Uniform $d$ -Wave State versus Stripe State
journal, July 2014

Two-dimensional incommensurate and three-dimensional commensurate magnetic order and fluctuations in La $_{2 - x}$ Ba $_{x}$ CuO $_{4}$
journal, July 2013

Observation of modulated magnetic long-range order in ${La}_{1.88} {Sr}_{0.12} {CuO}_{4}$
journal, February 1998

Glassy low-energy spin fluctuations and anisotropy gap in La $_{1.88}$ Sr $_{0.12}$ CuO $_{4}$
journal, April 2013

Effective Hamiltonian for the superconducting Cu oxides
journal, March 1988

Complete absence of isotope effect in Y ${Ba}_{2}$ ${Cu}_{3}$ $O_{7}$ : Consequences for phonon-mediated superconductivity
journal, September 1987

Local Magnetic Order vs Superconductivity in a Layered Cuprate
journal, August 2000

Theory of high- $T_{c}$ superconductivity in oxides
journal, June 1987

Magnetic, transport, and optical properties of monolayer copper oxides
journal, July 1998

Systematic $^{63} Cu$ NQR study of the stripe phase in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$ for $0.07 <~ x <~ 0.25$
journal, December 1999

The Resonating Valence Bond State in La2CuO4 and Superconductivity
journal, March 1987

Muon spin relaxation study of the stripe phase order in ${La}_{1.6 - x} {Nd}_{0.4} {Sr}_{x} {CuO}_{4}$ and related 214 cuprates
journal, October 1998

Structural instabilities in lanthanum cuprate superconductors
journal, April 1994

Evidence for stripe correlations of spins and holes in copper oxide superconductors
journal, June 1995

Spin-bag mechanism of high-temperature superconductivity
journal, March 1988

Stripe order in superconducting La $_{2 - x}$ Ba $_{x}$ CuO $_{4}$ ( $0.095 ⩽ x ⩽ 0.155$ )
journal, March 2011

Scale-invariant magnetoresistance in a cuprate superconductor
journal, August 2018

Linear temperature dependence of resistivity and change in the Fermi surface at the pseudogap critical point of a high-Tc superconductor
journal, November 2008

Possible highT c superconductivity in the Ba?La?Cu?O system
journal, June 1986

Stripe order, depinning, and fluctuations in ${La}_{1.875} {Ba}_{0.125} {CuO}_{4}$ and ${La}_{1.875} {Ba}_{0.075} {Sr}_{0.050} {CuO}_{4}$
journal, September 2004

High- T _c Superconductivity and Antiferromagnetism in Multilayered Copper Oxides –A New Paradigm of Superconducting Mechanism–
journal, January 2012

From quantum matter to high-temperature superconductivity in copper oxides
journal, February 2015

The physics of quantum materials
journal, October 2017

Neutron-scattering study of stripe-phase order of holes and spins in ${La}_{1.48}$ ${Nd}_{0.4}$ ${Sr}_{0.12}$ ${CuO}_{4}$
journal, September 1996

Incommensurate spin ordering and fluctuations in underdoped ${La}_{2 - x} {Ba}_{x} {CuO}_{4}$
journal, June 2008

Thermodynamic signatures of quantum criticality in cuprate superconductors
journal, February 2019

Charge density waves in cuprate superconductors beyond the critical doping
journal, March 2021

Interplay of electron–phonon interaction and strong correlations: the possible way to high-temperature superconductivity
journal, November 2000

Charge density wave fluctuations in ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ and their competition with superconductivity
journal, June 2014

Hidden Quantum Spin-Gap State in the Static Stripe Phase of High-Temperature ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ Superconductors
journal, January 2009

Hidden magnetism at the pseudogap critical point of a cuprate superconductor
journal, July 2020

Magnetic phase diagram of lightly doped ${La}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4}$ from ${}^{139}{La}$ nuclear quadrupole resonance
journal, October 1993

Glassy slowing of stripe modulation in ${(L a, E u, N d)}_{2 - x} ({S r, B a)}_{x} {CuO}_{4} : A^{63} Cu$ and $^{139} La$ NQR study down to 350 mK
journal, September 2001

Superexchange mechanism and d -wave superconductivity
journal, September 1988

Rotated stripe order and its competition with superconductivity in ${La}_{1.88} {Sr}_{0.12} {CuO}_{4}$
journal, September 2014

Diagonal static spin correlation in the low-temperature orthorhombic $Pccn$ phase of ${La}_{1.55} {Nd}_{0.4} {Sr}_{0.05} {CuO}_{4}$
journal, October 2001

Doping a Mott insulator: Physics of high-temperature superconductivity
journal, January 2006

Scattering and Pairing in Cuprate Superconductors
journal, August 2010

Structural phase transformations and superconductivity in ${La}_{2 - x}$ ${Ba}_{x}$ ${CuO}_{4}$
journal, June 1989

Observation of incommensurate magnetic correlations at the lower critical concentration for superconductivity in ${La}_{2 - x} {Sr}_{x} {CuO}_{4}$ $(x = 0.05)$
journal, July 1999

Antiferromagnetism and Its Relation to the Superconducting Phases of UP $t_{3}$
journal, August 1995

Coupling between Magnetic and Superconducting Order Parameters and Evidence for the Spin Excitation Gap in the Superconducting State of a Heavy Fermion Superconductor UPd ₂ Al ₃
journal, September 1997

A common thread: The pairing interaction for unconventional superconductors
journal, October 2012

Phase Separation and Finite Size Scaling ${inLa}_{2 - x}$ ${Sr}_{x}$ ${CuO}_{4 + δ}$ [0⩽(x,γ)⩽0.03]
journal, January 1993