Light-trapping and recycling for extraordinary power conversion in ultra-thin gallium-arsenide solar cells
Abstract
Here, we demonstrate nearly 30% power conversion efficiency in ultra-thin (~200 nm) gallium arsenide photonic crystal solar cells by numerical solution of the coupled electromagnetic Maxwell and semiconductor drift-diffusion equations. Our architecture enables wave-interference-induced solar light trapping in the wavelength range from 300-865 nm, leading to absorption of almost 90% of incoming sunlight. Our optimized design for 200 nm equivalent bulk thickness of GaAs, is a square-lattice, slanted conical-pore photonic crystal (lattice constant 550 nm, pore diameter 600 nm, and pore depth 290 nm), passivated with AlGaAs, deposited on a silver back-reflector, with ITO upper contact and encapsulated with SiO2. Our model includes both radiative and non-radiative recombination of photo-generated charge carriers. When all light from radiative recombination is assumed to escape the structure, a maximum achievable photocurrent density (MAPD) of 27.6 mA/cm2 is obtained from normally incident AM 1.5 sunlight. For a surface non-radiative recombination velocity of 103 cm/s, this corresponds to a solar power conversion efficiency of 28.3%. When all light from radiative recombination is trapped and reabsorbed (complete photon recycling) the power conversion efficiency increases to 29%. If the surface recombination velocity is reduced to 10 cm/sec, photon recycling is much more effective and the power conversionmore »
- Authors:
-
- Univ. of Toronto, Toronto, ON (Canada). Dept. of Physics
- Publication Date:
- Research Org.:
- Univ. of Toronto, Toronto, ON (Canada)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1285868
- Grant/Contract Number:
- FG02-06ER46347
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Scientific Reports
- Additional Journal Information:
- Journal Volume: 6; Journal ID: ISSN 2045-2322
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 14 SOLAR ENERGY; efficiency; localization; absorption; devices
Citation Formats
Eyderman, Sergey, and John, Sajeev. Light-trapping and recycling for extraordinary power conversion in ultra-thin gallium-arsenide solar cells. United States: N. p., 2016.
Web. doi:10.1038/srep28303.
Eyderman, Sergey, & John, Sajeev. Light-trapping and recycling for extraordinary power conversion in ultra-thin gallium-arsenide solar cells. United States. https://doi.org/10.1038/srep28303
Eyderman, Sergey, and John, Sajeev. Thu .
"Light-trapping and recycling for extraordinary power conversion in ultra-thin gallium-arsenide solar cells". United States. https://doi.org/10.1038/srep28303. https://www.osti.gov/servlets/purl/1285868.
@article{osti_1285868,
title = {Light-trapping and recycling for extraordinary power conversion in ultra-thin gallium-arsenide solar cells},
author = {Eyderman, Sergey and John, Sajeev},
abstractNote = {Here, we demonstrate nearly 30% power conversion efficiency in ultra-thin (~200 nm) gallium arsenide photonic crystal solar cells by numerical solution of the coupled electromagnetic Maxwell and semiconductor drift-diffusion equations. Our architecture enables wave-interference-induced solar light trapping in the wavelength range from 300-865 nm, leading to absorption of almost 90% of incoming sunlight. Our optimized design for 200 nm equivalent bulk thickness of GaAs, is a square-lattice, slanted conical-pore photonic crystal (lattice constant 550 nm, pore diameter 600 nm, and pore depth 290 nm), passivated with AlGaAs, deposited on a silver back-reflector, with ITO upper contact and encapsulated with SiO2. Our model includes both radiative and non-radiative recombination of photo-generated charge carriers. When all light from radiative recombination is assumed to escape the structure, a maximum achievable photocurrent density (MAPD) of 27.6 mA/cm2 is obtained from normally incident AM 1.5 sunlight. For a surface non-radiative recombination velocity of 103 cm/s, this corresponds to a solar power conversion efficiency of 28.3%. When all light from radiative recombination is trapped and reabsorbed (complete photon recycling) the power conversion efficiency increases to 29%. If the surface recombination velocity is reduced to 10 cm/sec, photon recycling is much more effective and the power conversion efficiency reaches 30.6%.},
doi = {10.1038/srep28303},
journal = {Scientific Reports},
number = ,
volume = 6,
place = {United States},
year = {Thu Jun 23 00:00:00 EDT 2016},
month = {Thu Jun 23 00:00:00 EDT 2016}
}
Web of Science
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