Evidence of long-range ferromagnetic order and spin frustration effects in the double perovskite La2CoMnO6

Madhogaria, R. P.; Das, R.; Clements, E. M.; Kalappattil, V.; Phan, M. H.; Srikanth, H.; Dang, N. T.; Kozlenko, D. P.; Bingham, N. S.

doi:10.1103/physrevb.99.104436

Title: Evidence of long-range ferromagnetic order and spin frustration effects in the double perovskite ${La}_{2} {CoMnO}_{6}$

Journal Article · Fri Mar 29 00:00:00 EDT 2019 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.99.104436· OSTI ID:1609900

Madhogaria, R. P. ^[1]; Das, R. ^[1]; Clements, E. M. ^[1]; Kalappattil, V. ^[1]; Phan, M. H. ^[1]; Srikanth, H. ^[1]; Dang, N. T. ^[2]; Kozlenko, D. P. ^[3]; Bingham, N. S. ^[4]

Univ. of South Florida, Tampa, FL (United States)
Duy Tan Univ., Da Nang (Vietnam)
Joint Inst. for Nuclear Research, Dubna (Russia)
Yale Univ., New Haven, CT (United States)

We present a comprehensive study on the magnetic structure, dynamics, and phase evolution in the single phase double perovskite La₂CoMnO₆. The mixed valence state due to oxygen deficiency is verified by x-ray photoelectron spectroscopy and confirms a double ferromagnetic transition observed in dc magnetization. Neutron diffraction reveals that the magnetic structure is dominated by long-range ferromagnetic ordering, which is further corroborated by a critical exponents analysis of the paramagnetic to ferromagnetic phase transition. An analysis of the magnetization dynamics by means of linear and nonlinear ac magnetic susceptibilities marks the presence of two distinct cluster-glass-like states that emerge at low temperatures. The isothermal entropy change as a function of temperature and magnetic field (H) is exploited to investigate the mechanism of stabilization of the magnetic phases across the H – T phase diagram. In the regime of the phase diagram where thermal energy is sufficiently low, regions of competing interactions due to local disorder become stabilized and display glasslike dynamics. The freezing mechanism of clusters is illustrated using a unique probe of transverse susceptibility that isolates the effects of the local anisotropy of the spin clusters. Here, the results are summarized in a H – T phase diagram of La₂CoMnO₆ from these data.

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Research Organization:: Univ. of South Florida, Tampa, FL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division; Vietnam National Foundation for Science and Technology Development (NAFOSTED)

Grant/Contract Number:: FG02-07ER46438; 103.02-2017.364

OSTI ID:: 1609900

Alternate ID(s):: OSTI ID: 1504549

Journal Information:: Physical Review B, Vol. 99, Issue 10; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 48 works

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Title: Evidence of long-range ferromagnetic order and spin frustration effects in the double perovskite La 2 CoMnO 6

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