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Title: Theoretical Investigation of Dynamic Properties of Magnetic Molecule Systems as Probed by NMR and Pulsed Fields Experiments

Thesis/Dissertation ·
DOI:https://doi.org/10.2172/861633· OSTI ID:861633
 [1]
  1. Iowa State Univ., Ames, IA (United States)

The field of molecular magnetism[l-6] has become a subject of intense theoretical and experimental interest and has rapidly evolved during the last years. This inter-disciplinary field concerns magnetic systems at the molecular or "nanoscopic" level, whose realization has become feasible due to recent advances in the field of chemical synthesis. The present theoretical work provides a first step towards exploiting the possibilities that are offered by probing magnetic molecules using external magnetic fields with high sweep rates. These probes, apart for providing information specific to magnetic molecules, offer the possibility of conducting a detailed study of the relaxational behavior of interacting spin systems as a result of their coupling with a "heat bath" and in particular the excitations of the host lattice. Development of a broad theoretical framework for dealing with relaxational phenomena induced by dynamical magnetic fields is indeed a worthy goal.

Research Organization:
Ames Lab., Ames, IA (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
W-7405-Eng-82
OSTI ID:
861633
Report Number(s):
IS-T-2765; TRN: US200602%%214
Country of Publication:
United States
Language:
English

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