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Title: Geometric Frustration in the Mixed Layer Pnictide Oxides

Conference ·
DOI:https://doi.org/10.1139/p01-105· OSTI ID:791736

The authors present results from a Monte Carlo investigation of a simple bilayer model with geometrically frustrated interactions similar to those found in the mixed layer pnictide oxides (Sr{sub 2}Mn{sub 3}Pn{sub 2}O{sub 2}, Pn = As, Sb). The model is composed of two inequivalent square lattices with nearest-neighbor intra- and interlayer interactions. They find a ground state composed of two independent Neel ordered layers when the interlayer exchange is an order of magnitude weaker than the intralayer exchange, as suggested by experiment. Evidence for local orthogonal order between the layers is found, but it occurs in regions of parameter space which are not experimentally realized. Qualitatively similar results were observed in models with a larger number of layers. They conclude that frustration caused by nearest-neighbor interactions in the mixed layer pnictide oxides is not sufficient to explain the long-range orthogonal order that is observed experimentally.

Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE Office of Defense Programs (DP) (US)
DOE Contract Number:
W-7405-Eng-48
OSTI ID:
791736
Report Number(s):
UCRL-JC-139107; TRN: US200304%%523
Resource Relation:
Journal Volume: 79; Journal Issue: 11-12; Conference: Highly Frustrated Magnetism 2000, Waterloo, Ontario (CA), 06/11/2000--06/15/2000; Other Information: PBD: 6 Jun 2000
Country of Publication:
United States
Language:
English

References (12)

Critical Properties of Helimagnets journal December 1988
Incommensurate correlations in the t - J and frustrated spin-1/2 Heisenberg models journal October 1990
Comparative Studies of Magnetism in KNi F 3 and K 2 Ni F 4 journal December 1967
Synthesis and Characterization of a New Compound with Alternating MnO22- and Zn2As22- Layers:  Ba2MnZn2As2O2 journal January 1998
Magnetic states in frustrated bilayer models: The ordered phase of mixed-layer pnictide oxides journal June 2000
Neutron diffraction study of magnetic ordering in ErMn2Si2, ErMn2Ge2 and ErFe2Si2 journal January 1984
Ordering due to disorder in a frustrated vector antiferromagnet journal April 1989
Further aspects of the structure and magnetism of the layered compound Fe(III)ClMoO4: Mössbauer spectroscopy, susceptibility, and powder neutron diffraction studies journal January 1987
Neutron Scattering from K 2 Ni F 4 : A Two-Dimensional Heisenberg Antiferromagnet journal April 1969
Phase Transition of the Three-Dimensional Heisenberg Antiferromagnet on the Layered-Triangular Lattice journal September 1985
Spin glasses: Experimental facts, theoretical concepts, and open questions journal October 1986
The magnetic structures of the mixed layer pnictide oxide compounds Sr2Mn3Pn2O2 (Pn = As, Sb) journal April 1996

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