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Title: Radionuclide characterization of reactor decommissioning waste and spent fuel assembly hardware

Technical Report ·
DOI:https://doi.org/10.2172/6340508· OSTI ID:6340508

This study is providing the NRC and licensees with a more comprehensive and defensible data base and regulatory assessment of the radiological factors associated with reactor decommissioning and disposal of wastes generated during these activities. The objectives of this study are being accomplished during a two-phase sampling, measurement, and assessment program involving the actual decommissioning of Shippingport Station and the detailed analysis of neutron-activated materials from commercial reactors. Radiological characterization studies at Shippingport have shown that neutron activation products, dominated by {sup 60}Co, comprised the residual radionuclide inventory. Fission products and transuranic radionuclides were essentially absent. Waste classification assessments have shown that all decommissioning materials (except reactor pressure vessel internals) could be disposed of as Class A waste. Measurements and assessments of spent fuel assembly hardware have shown that {sup 63}Ni, {sup 59}Ni, and {sup 94}Nb sometimes greatly exceed the 10CFR61 Class C limit for some components, and thus would require disposal in a high level waste repository. These measurements are providing the basis for an assessment of the disposal options for these types of highly radioactive materials. Comparisons of predicted (calculated) activation product concentrations with the empirical data are providing as assessment of the accuracy of calculational methods. Work is continuing on radiological characterization of spent PWR and BWR control rod assemblies. Additional work is planned on current issues/problems relating to reactor decommissioning. These efforts will be reported on in future supplements to this report. 20 refs., 23 figs., 34 tabs.

Research Organization:
Nuclear Regulatory Commission, Washington, DC (USA). Div. of Regulatory Applications; Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
Sponsoring Organization:
USNRC
DOE Contract Number:
AC06-76RL01830
OSTI ID:
6340508
Report Number(s):
NUREG/CR-5343; PNL-6806; ON: TI91007071; TRN: 91-004410
Country of Publication:
United States
Language:
English

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