Polonium problem in lead-bismuth flow target
- State Scientific Centre of Russian Federation-Institute of Physics and Power Engineering, Obninsk (Russian Federation)
Alpha-active polonium nuclides Po198 - Po210 are formed in a lead-bismuth target as results of reactions Bi{sup 209}(n,{gamma})Bi{sup 210} {yields} Po{sup 210}, Bi{sup 209}(p,xn)Po{sup 210} {yields} Po{sup 210 {minus} x} (x = 1-12), Pb{sup 208}({alpha},xn) {yields} Po{sup 210 {minus} x + 2} (x = 2-14). The most important nuclides are Po-210 (T{sub {1/2}}=138.4 day), Po-209 (T{sub {1/2}}=102 years) and Po-208 (T{sub {1/2}}=2.9 years). Polonium activity of the circuit for SINQ - conditions is about 15,000 Ci after 1-year operation. Polonium radiation hazard is connected with its output from the coolant and formation of aerosol and surface alpha-activity after the circuit break-down for repair works or in accidents. One of the important issues of polonium removal system creation is containing and storing polonium removed. Its storage in solidified alkaline is not expedient because of secondary neutron formation as a result of ({alpha},n) - reaction on oxygen and sodium nucleus. The estimations carried out demonstrated that by polonium concentration {approx} 100 Ci/l neutron current on the container surface can reach {approx} 10{sup 4}n/(cm{sup 2}s). Concentration and storage of polonium in solidified lead-bisumth seems the most convenient. The calculations demonstrated that in a 100 l container 50,000 Ci of polonium can be stored (as much as 3 times more than 1-year polonium product in SINQ-conditions) under temperature in the container less than melting point of lead bismuth (the wall temperature is about 100{degrees}C).
- Research Organization:
- Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
- OSTI ID:
- 381056
- Report Number(s):
- CONF-9603171-; ON: DE96014047; TRN: 96:005200-0019
- Resource Relation:
- Conference: International workshop on the technology and thermo hydrolics of heavy liquid metals (Hg,Pb,Bi, and their Eutectics), Schruns (Austria), 25-28 Mar 1996; Other Information: PBD: Jun 1996; Related Information: Is Part Of Proceedings of the international workshop on the technology and thermal hydraulics of heavy liquid metals (Hg, Pb, Bi, and their eutectics); Appleton, B.R.; Bauer, G.S. [comp.]; PB: 500 p.
- Country of Publication:
- United States
- Language:
- English
Similar Records
NEGATIVE PION PHOTOPRODUCTION FROM BISMUTH ACCOMPANIED BY NEUTRON EMISSION
MOUND LABORATORY PROGRESS REPORT FOR SEPTEMBER 1963