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Title: Particle size influence on material properties of BaTiO3 ceramics fabricated using freeze-form extrusion 3D printing

Journal Article · · Materials Research Express (Online)
ORCiD logo [1];  [1];  [2];  [3]; ORCiD logo [1];  [1]; ORCiD logo [4];  [1];  [3];  [1]
  1. Univ. of Texas at El Paso, TX (United States). Dept. of Mechanical Engineering
  2. Shantou Univ. (China). Dept. of Physics
  3. Univ. of Texas at El Paso, TX (United States). Dept. of Industrial, Manufacturing, and Systems Engineering
  4. Univ. of Oklahoma, Norman, OK (United States). Dept. of Aerospace and Mechanical Engineering

Barium titanate (BaTiO3; BTO) is a well-known lead-free piezoelectric material commonly used for sensors and actuators applications. There are several traditional methods to fabricate bulk BTO ceramics; however, most of those methods have restrictions regarding being able to produce a functional and complex shape for specific application needs. Recently, additive manufacturing techniques such as binder jetting have enabled the fabrication of complex designs of piezoelectric ceramics. However, the density achieved is relatively low thus narrowing their applications. This paper presents the fabrication of high-density BaTiO3 ceramics using Freeze-form Extrusion Fabrication (FEF). The influence on material properties for different ceramic particle size was assessed. It was found that parts printed using finer BaTiO3 particle sizes achieved better results in terms of density, piezoelectric, and dielectric properties. For this study, the 100 nm BaTiO3 samples achieved 85.24% density, a high piezoelectric property of 204.61pC/N and dielectric permittivity of 2551. These results demonstrated the feasibility of using FEF additive manufacturing to fabricate high-quality functional ceramics with designed geometry in a mold-free fashion.

Research Organization:
Univ. of Texas at El Paso, TX (United States)
Sponsoring Organization:
USDOE Office of Fossil Energy (FE); USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
FE0027502; NA0003865
OSTI ID:
1799871
Alternate ID(s):
OSTI ID: 1958034
Journal Information:
Materials Research Express (Online), Vol. 6, Issue 11; ISSN 2053-1591
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

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