Macrocycles as Ion Pair Receptors

He, Qing; Vargas-Zúñiga, Gabriela I.; Kim, Seung Hyun; Kim, Sung Kuk; Sessler, Jonathan L.

doi:10.1021/acs.chemrev.8b00734

Title: Macrocycles as Ion Pair Receptors

Journal Article · Mon May 13 00:00:00 EDT 2019 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.8b00734· OSTI ID:1598892

^[1]; Vargas-Zúñiga, Gabriela I. ^[2]; Kim, Seung Hyun ^[3];

^[3];

^[4]

Univ. of Texas, Austin, TX (United States); Hunan Univ., Changsha (China)
Univ. of Texas, Austin, TX (United States)
Gyeongsang National Univ., Jinju (Korea)
Shanghai Univ. (China); Univ. of Texas, Austin, TX (United States)

Cation and anion recognition have both played central roles in the development of supramolecular chemistry. Additionally, much of the associated research has focused on the development of receptors for individual cations or anions, as well as their applications in different areas. Rarely is complexation of the counterions considered. In contrast, ion pair recognition chemistry, emerging from cation and anion coordination chemistry, is a specific research field where co-complexation of both anions and cations, so-called ion pairs, is the center of focus. Systems used for the purpose, known as ion pair receptors, are typically di- or polytopic hosts that contain recognition sites for both cations and anions and which permit the concurrent binding of multiple ions. The field of ion pair recognition has blossomed during the past decades. Several smaller reviews on the topic were published roughly 5 years ago. They provided a summary of synthetic progress and detailed the various limiting ion recognition modes displayed by both acyclic and macrocyclic ion pair receptors known at the time. The present review is designed to provide a comprehensive and up-to-date overview of the chemistry of macrocycle-based ion pair receptors. Finally, we specifically focus on the relationship between structure and ion pair recognition, as well as applications of ion pair receptors in sensor development, cation and anion extraction, ion transport, and logic gate construction.

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Research Organization:: Univ. of Texas, Austin, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Institutes of Health (NIH); Robert A. Welch Foundation; National Research Foundation of Korea (NRF)

Grant/Contract Number:: FG02-01ER15186; R01 GM 103790; F-0018; 2017R1A4A1014595

OSTI ID:: 1598892

Journal Information:: Chemical Reviews, Vol. 119, Issue 17; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 183 works

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