An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3
Abstract
A symmetric sodium-ion battery with an aqueous electrolyte is demonstrated; it utilizes the NASICON-structured Na3MnTi(PO4)3 as both the anode and the cathode. The NASICON-structured Na3MnTi(PO4)3 possesses two electrochemically active transition metals with the redox couples of Ti4+/Ti3+ and Mn3+/Mn2+ working on the anode and cathode sides, respectively. The symmetric cell based on this bipolar electrode material exhibits a well-defined voltage plateau centered at about 1.4 V in an aqueous electrolyte with a stable cycle performance and superior rate capability. The advent of aqueous symmetric sodium-ion battery with high safety and low cost may provide a solution for large-scale stationary energy storage.
- Authors:
-
- Univ. of Texas, Austin, TX (United States). Texas Materials Inst.
- Publication Date:
- Research Org.:
- Univ. of Texas, Austin, TX (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1533083
- Grant/Contract Number:
- SC0005397
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Angewandte Chemie (International Edition)
- Additional Journal Information:
- Journal Volume: 55; Journal Issue: 41; Journal ID: ISSN 1433-7851
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; 25 ENERGY STORAGE; aqueous electrolyte; energy storage; sodium-ion battery; symmetric battery
Citation Formats
Gao, Hongcai, and Goodenough, John B. An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3. United States: N. p., 2016.
Web. doi:10.1002/anie.201606508.
Gao, Hongcai, & Goodenough, John B. An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3. United States. https://doi.org/10.1002/anie.201606508
Gao, Hongcai, and Goodenough, John B. 2016.
"An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3". United States. https://doi.org/10.1002/anie.201606508. https://www.osti.gov/servlets/purl/1533083.
@article{osti_1533083,
title = {An Aqueous Symmetric Sodium-Ion Battery with NASICON-Structured Na3MnTi(PO4)3},
author = {Gao, Hongcai and Goodenough, John B.},
abstractNote = {A symmetric sodium-ion battery with an aqueous electrolyte is demonstrated; it utilizes the NASICON-structured Na3MnTi(PO4)3 as both the anode and the cathode. The NASICON-structured Na3MnTi(PO4)3 possesses two electrochemically active transition metals with the redox couples of Ti4+/Ti3+ and Mn3+/Mn2+ working on the anode and cathode sides, respectively. The symmetric cell based on this bipolar electrode material exhibits a well-defined voltage plateau centered at about 1.4 V in an aqueous electrolyte with a stable cycle performance and superior rate capability. The advent of aqueous symmetric sodium-ion battery with high safety and low cost may provide a solution for large-scale stationary energy storage.},
doi = {10.1002/anie.201606508},
url = {https://www.osti.gov/biblio/1533083},
journal = {Angewandte Chemie (International Edition)},
issn = {1433-7851},
number = 41,
volume = 55,
place = {United States},
year = {Tue Sep 13 00:00:00 EDT 2016},
month = {Tue Sep 13 00:00:00 EDT 2016}
}
Web of Science
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- Shi, Huifeng; Liu, Xianqiang; Wu, Rui
- Applied Sciences, Vol. 9, Issue 5
Electrospun NaVPO 4 F/C Nanofibers as Self-Standing Cathode Material for Ultralong Cycle Life Na-Ion Batteries
journal, April 2017
- Jin, Ting; Liu, Yongchang; Li, Yang
- Advanced Energy Materials, Vol. 7, Issue 15
Aqueous Batteries Operated at −50 °C
journal, November 2019
- Nian, Qingshun; Wang, Jiayue; Liu, Shuang
- Angewandte Chemie International Edition, Vol. 58, Issue 47
Nanocrystal-Assembled Porous Na 3 MgTi(PO 4 ) 3 Aggregates as Highly Stable Anode for Aqueous Sodium-Ion Batteries
journal, August 2017
- Zhang, Fang; Li, Wanfeng; Xiang, Xingde
- Chemistry - A European Journal, Vol. 23, Issue 52
Conversion Synthesis of Self‐Standing Potassium Zinc Hexacyanoferrate Arrays as Cathodes for High‐Voltage Flexible Aqueous Rechargeable Sodium‐Ion Batteries
journal, December 2019
- He, Bing; Man, Ping; Zhang, Qichong
- Small, Vol. 15, Issue 52
Sodium-ion batteries: present and future
journal, January 2017
- Hwang, Jang-Yeon; Myung, Seung-Taek; Sun, Yang-Kook
- Chemical Society Reviews, Vol. 46, Issue 12
An ion-conducting SnS–SnS 2 hybrid coating for commercial activated carbons enabling their use as high performance anodes for sodium-ion batteries
journal, January 2019
- Zhang, Si-Wei; Lv, Wei; Qiu, Dong
- Journal of Materials Chemistry A, Vol. 7, Issue 17
A Multi-Ion Strategy towards Rechargeable Sodium-Ion Full Batteries with High Working Voltage and Rate Capability
journal, November 2018
- Jiang, Chunlei; Fang, Yue; Zhang, Wenyong
- Angewandte Chemie, Vol. 130, Issue 50
An Abnormal 3.7 Volt O3-Type Sodium-Ion Battery Cathode
journal, May 2018
- Wang, Peng-Fei; Xin, Hanshen; Zuo, Tong-Tong
- Angewandte Chemie International Edition, Vol. 57, Issue 27
A Hydrostable Cathode Material Based on the Layered P2@P3 Composite that Shows Redox Behavior for Copper in High-Rate and Long-Cycling Sodium-Ion Batteries
journal, January 2019
- Yan, Zichao; Tang, Liang; Huang, Yangyang
- Angewandte Chemie International Edition, Vol. 58, Issue 5
In Situ SEM Observation of Structured Si/C Anodes Reactions in an Ionic-Liquid-Based Lithium-Ion Battery
text, January 2019
- Shi, Huifeng; Liu, Xianqiang; Wu, Rui
- Karlsruhe
Electrolytes and Interphases in Sodium-Based Rechargeable Batteries : Recent Advances and Perspectives
text, January 2020
- Eshetu, Gebrekidan Gebresilassie; Elia, Giuseppe Antonio; Armand, Michel
- RWTH Aachen University
Electrolytes and Interphases in Sodium-Based Rechargeable Batteries: Recent Advances and Perspectives
text, January 2020
- Eshetu, Gebrekidan Gebresilassie; Elia, Giuseppe Antonio; Armand, Michel
- Karlsruhe
Intermixed Cation-Anion Aqueous Battery Based on an Extremely Fast and Long-Cycling Di-Block Bipyridinium-Naphthalene Diimide Oligomer
text, January 2019
- Perticarari, Sofia; Doizy, Tom; Soudan, Patrick
- arXiv
An Efficient Evaluation of F-doped Polyanion Cathode Materials with Long Cycle Life for Na-Ion Batteries Applications
journal, November 2017
- Muruganantham, Rasu; Chiu, Yi-Tang; Yang, Chun-Chuen
- Scientific Reports, Vol. 7, Issue 1