Recent advances in ultrafast X-ray sources

Schoenlein, Robert; Elsaesser, Thomas; Holldack, Karsten; Huang, Zhirong; Kapteyn, Henry; Murnane, Margaret; Woerner, Michael

doi:10.1098/rsta.2018.0384

Title: Recent advances in ultrafast X-ray sources

Journal Article · Mon Apr 01 00:00:00 EDT 2019 · Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences

DOI:https://doi.org/10.1098/rsta.2018.0384· OSTI ID:1528864

Schoenlein, Robert ^[1]; Elsaesser, Thomas ^[2]; Holldack, Karsten ^[3]; Huang, Zhirong ^[1]; Kapteyn, Henry ^[4]; Murnane, Margaret ^[4]; Woerner, Michael ^[2]

SLAC National Accelerator Lab., Menlo Park, CA (United States)
Max Born Inst. for Nonlinear Optics and Short Pulse Spectroscopy (MBI), Berlin (Germany)
Helmholtz-Zentrum Berlin (HZB), (Germany). German Research Centre for Materials and Energy
Univ. of Colorado, Boulder, CO (United States)

Over more than a century, X-rays have transformed our understanding of the fundamental structure of matter and have been an indispensable tool for chemistry, physics, biology, materials science and related fields. Current advances in ultrafast X-ray sources operating in the femtosecond to attosecond regimes have opened an important new frontier in X-ray science. These advances now allow: (i) sensitive probing of structural dynamics in matter on the fundamental timescales of atomic motion, (ii) element-specific probing of electronic structure and charge dynamics on fundamental timescales of electronic motion, and (iii) powerful new approaches for unravelling the coupling between electronic and atomic structural dynamics that underpin the properties and function of matter. Most notable is the recent realization of X-ray free-electron lasers (XFELs) with numerous new XFEL facilities in operation or under development worldwide. Advances in XFELs are complemented by advances in synchrotron-based and table-top laser-plasma X-ray sources now operating in the femtosecond regime, and laser-based high-order harmonic XUV sources operating in the attosecond regime. This article is part of the theme issue ‘Measurement of ultrafast electronic and structural dynamics with X-rays’.

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Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Univ. of Colorado, Boulder, CO (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Defence Advanced Research Projects Agency

Grant/Contract Number:: AC02-76SF00515; FG02-99ER14982; SC0002002

OSTI ID:: 1528864

Alternate ID(s):: OSTI ID: 1907874; OSTI ID: 1957805

Journal Information:: Philosophical Transactions of the Royal Society. A, Mathematical, Physical and Engineering Sciences, Vol. 377, Issue 2145; ISSN 1364-503X

Publisher:: The Royal Society PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 68 works

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