Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

Sun, X. M.; Cong, D. Y.; Li, Z.; Zhang, Y. L.; Chen, Z.; Ren, Y.; Liss, K. -D.; Ma, Z. Y.; Li, R. G.; Qu, Y. H.; Yang, Z.; Wang, L.; Wang, Y. D.

doi:10.1103/PhysRevMaterials.3.034404

Title: Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

Journal Article · Mon Mar 11 00:00:00 EDT 2019 · Physical Review Materials

DOI:https://doi.org/10.1103/PhysRevMaterials.3.034404· OSTI ID:1524778

Sun, X. M. ^[1]; Cong, D. Y. ^[1]; Li, Z. ^[2]; Zhang, Y. L. ^[2]; Chen, Z. ^[1]; Ren, Y. ^[3]; Liss, K. -D. ^[4]; Ma, Z. Y. ^[5]; Li, R. G. ^[1]; Qu, Y. H. ^[1]; Yang, Z. ^[1]; Wang, L. ^[6]; Wang, Y. D. ^[1]

Univ. of Science and Technology Beijing, (China)
Qujing Normal Univ., (China)
Argonne National Lab. (ANL), Lemont, IL (United States)
Australian Nuclear Science and Technology Organisation (ANSTO), Lucas Heights, NSW (Australia); Guangdong Technion-Israel Inst. of Technology, Shantou (China)
China Univ. of Petroleum, Beijing (China)
Beijing Inst. of Technology, Beijing (China)

Promising multifunctional magnetoresponsive effects such as magnetoresistance, magnetostrain, and the magnetocaloric effect have recently been extensively studied in Ni-Mn-based metamagnetic shape memory alloys, but large reversible magnetoresponsive effects are usually obtained under high magnetic fields, which is an obstacle for practical applications. In this work, through manipulating magnetostructural transition, we achieved large reversible magnetoresponsive effects under a relatively low magnetic field of 3 T in a Ni-Co-Mn-In alloy. By systematically tuning the Mn/In ratio and Co substitution, an optimum composition Ni₄₉Co₃Mn₃₄In₁₄ with a low thermal hysteresis (8 K), a narrow transformation interval (7 K) and a high sensitivity of transformation temperature to field change (6KT^-1), was obtained. Good geometric compatibility between austenite and martensite was revealed by in situ synchrotron high-energy x-ray diffraction experiment, which accounts for the low hysteresis and narrow transformation interval. A reversible transformation between pure austenite and pure martensite is induced by a relatively low field of 3 T, which was directly evidenced by in situ neutron diffraction experiments. As a result, a large reversible magnetocaloric effect with entropy change of 16.5Jkg^-1K^-1, a large reversible magnetostrain of 0.26%, and a large reversible magnetoresistance of 60%, under a relatively low field of 3 T, were simultaneously achieved. These reversible magnetoresponsive effects are comparable to the maximum reversible values obtained under high fields in other Ni-Mn-based alloys, but the magnetic field we applied is much lower. This research may guide the design of metamagnetic shape memory alloys with low-field-induced magnetoresponsive properties for magnetic refrigeration, magnetic sensing, and magnetic recording applications.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities Division; National Natural Science Foundation of China (NSFC)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1524778

Alternate ID(s):: OSTI ID: 1498811

Journal Information:: Physical Review Materials, Vol. 3, Issue 3; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 16 works

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Title: Manipulation of magnetostructural transition and realization of prominent multifunctional magnetoresponsive properties in NiCoMnIn alloys

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