Site-Specific Substitutional Boron Doping of Semiconducting Armchair Graphene Nanoribbons

Cloke, Ryan R.; Marangoni, Tomas; Nguyen, Giang D.; Joshi, Trinity; Rizzo, Daniel J.; Bronner, Christopher; Cao, Ting; Louie, Steven G.; Crommie, Michael F.; Fischer, Felix R.

doi:10.1021/jacs.5b02523

Title: Site-Specific Substitutional Boron Doping of Semiconducting Armchair Graphene Nanoribbons

Journal Article · Wed Jul 08 00:00:00 EDT 2015 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.5b02523· OSTI ID:1512219

Cloke, Ryan R. ^[1]; Marangoni, Tomas ^[1]; Nguyen, Giang D. ^[1]; Joshi, Trinity ^[1]; Rizzo, Daniel J. ^[1]; Bronner, Christopher ^[1]; Cao, Ting ^[1]; Louie, Steven G. ^[2]; Crommie, Michael F. ^[2]; Fischer, Felix R. ^[2]

Univ. of California, Berkeley, CA (United States)
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

A fundamental requirement for the development of advanced electronic device architectures based on graphene nanoribbon (GNR) technology is the ability to modulate the band structure and charge carrier concentration by substituting specific carbon atoms in the hexagonal graphene lattice with p- or n-type dopant heteroatoms. Here we report the atomically precise introduction of group III dopant atoms into bottom-up fabricated semiconducting armchair GNRs (AGNRs). Trigonal-planar B atoms along the backbone of the GNR share an empty p-orbital with the extended π-band for dopant functionality. Scanning tunneling microscopy (STM) topography reveals a characteristic modulation of the local density of states along the backbone of the GNR that is superimposable with the expected position and concentration of dopant B atoms. First-principles calculations support the experimental findings and provide additional insight into the band structure of B-doped 7-AGNRs.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Materials Sciences & Engineering Division (SC-22.2)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1512219

Journal Information:: Journal of the American Chemical Society, Vol. 137, Issue 28; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 173 works

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