Synthesis of Type I PbSe/CdSe Dot-on-Plate Heterostructures with Near-Infrared Emission

Williams, Kali R.; Diroll, Benjamin T.; Watkins, Nicolas E.; Rui, Xue; Brumberg, Alexandra; Klie, Robert F.; Schaller, Richard D.

doi:10.1021/jacs.8b13794

Title: Synthesis of Type I PbSe/CdSe Dot-on-Plate Heterostructures with Near-Infrared Emission

Journal Article · Mon Mar 18 00:00:00 EDT 2019 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.8b13794· OSTI ID:1510305

Williams, Kali R. ^[1];

^[2]; Watkins, Nicolas E. ^[1]; Rui, Xue ^[3];

^[1]; Klie, Robert F. ^[3];

^[4]

Northwestern Univ., Evanston, IL (United States)
Argonne National Lab. (ANL), Lemont, IL (United States)
Univ. of Illinois at Chicago, Chicago, IL (United States)
Northwestern Univ., Evanston, IL (United States); Argonne National Lab. (ANL), Lemont, IL (United States)

Zero-dimensional PbSe quantum dots are heterogeneously nucleated and grown onto two-dimensional zincblende CdSe nanoplatelets. Electron microscopy shows ad-grown dots predominantly decorate edges and corners of the nanoplatelets. Spectroscopic characterizations relate type I electronic alignment as demonstrated via photoluminescence excitation spectroscopy enhancement of near-infrared emission. Transient photoluminescence and absorption convey ultrafast transfer of excitons to the lower energy semiconductor dots. Furthermore these structures combine benefits of large absorption cross sections of nanoplatelets and efficient near-infrared emission of PbSe with quantum confinement tuning of energy gap.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1510305

Journal Information:: Journal of the American Chemical Society, Vol. 141, Issue 13; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 21 works

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Polarized near-infrared intersubband absorptions in CdSe colloidal quantum wells Diroll, Benjamin T.; Chen, Menglu; Coropceanu, Igor Nature Communications, Vol. 10, Issue 1 https://doi.org/10.1038/s41467-019-12503-z	journal	October 2019
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