Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014

Irish, Victoria E.; Hanna, Sarah J.; Willis, Megan D.; China, Swarup; Thomas, Jennie L.; Wentzell, Jeremy J.  B.; Cirisan, Ana; Si, Meng; Leaitch, W. Richard; Murphy, Jennifer G.; Abbatt, Jonathan P.  D.; Laskin, Alexander; Girard, Eric; Bertram, Allan K.

doi:10.5194/acp-19-1027-2019

Title: Ice nucleating particles in the marine boundary layer in the Canadian Arctic during summer 2014

Journal Article · Fri Jan 25 00:00:00 EST 2019 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-19-1027-2019· OSTI ID:1501757

Irish, Victoria E. ^[1]; Hanna, Sarah J. ^[1];

^[2];

^[3]; Thomas, Jennie L. ^[4]; Wentzell, Jeremy J. B. ^[5]; Cirisan, Ana ^[6];

^[1]; Leaitch, W. Richard ^[5];

^[2];

^[7]; Girard, Eric ^[6];

^[1]

Univ. of British Columbia, Vancouver, BC (Canada)
Univ. of Toronto, ON (Canada)
Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
Univ. Grenoble Alpes (France); Univ. Pierre et Marie Curie, Paris (France)
Environment and Climate Change Canada, Toronto, ON (United States)
Univ. of Quebec (Canada)
Purdue Univ., West Lafayette, IN (United States)

Ice nucleating particles (INPs) in the Arctic can influence climateand precipitation in the region; yet our understanding of the concentrations and sourcesof INPs in this region remain uncertain. In the following, we (1) measured concentrationsof INPs in the immersion mode in the Canadian Arctic marine boundary layer duringsummer 2014 on board the CCGS Amundsen, (2) determined ratios of surface areasof mineral dust aerosol to sea spray aerosol, and (3) investigated the source region ofthe INPs using particle dispersion modelling. Average concentrations of INPs at -15,-20, and -25^-C were 0.005, 0.044, and 0.154L^-1,respectively. These concentrations fall within the range of INP concentrations measuredin other marine environments. For the samples investigated the ratio of mineral dustsurface area to sea spray surface area ranged from 0.03 to 0.09. Based on these ratiosand the ice active surface site densities of mineral dust and sea spray aerosoldetermined in previous laboratory studies, our results suggest that mineral dust is amore important contributor to the INP population than sea spray aerosol for the samplesanalysed. Based on particle dispersion modelling, the highest concentrations of INPs wereoften associated with lower-latitude source regions such as the Hudson Bay area, easternGreenland, or north-western continental Canada. On the other hand, the lowestconcentrations were often associated with regions further north of the sampling sites andover Baffin Bay. A weak correlation was observed between INP concentrations and the timethe air mass spent over bare land, and a weak negative correlation was observed betweenINP concentrations and the time the air mass spent over ice and open water. Thesecombined results suggest that mineral dust from local sources is an important contributorto the INP population in the Canadian Arctic marine boundary layer during summer 2014.

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Research Organization:: Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC05-76RL01830

OSTI ID:: 1501757

Report Number(s):: PNNL-SA-138062

Journal Information:: Atmospheric Chemistry and Physics (Online), Vol. 19, Issue 2; ISSN 1680-7324

Publisher:: European Geosciences UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 39 works

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Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments Hoose, C.; Möhler, O. Karlsruhe https://doi.org/10.5445/ir/110089633	text	January 2012
Heterogeneous ice nucleation on atmospheric aerosols: a review of results from laboratory experiments Hoose, Corinna; Möhler, Ottmar Karlsruhe https://doi.org/10.5445/ir/1000038466	text	January 2012
Supporting data for manuscript titled "Marine and terrestrial organic ice nucleating particles in pristine marine to continentally-influenced northeast Atlantic air masses" McCluskey, C. S.; Ovadnevaite, J.; Rinaldi, M. Mountain Scholar https://doi.org/10.25675/10217/187808	dataset	January 2018

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Overview paper: New insights into aerosol and climate in the Arctic Abbatt, Jonathan P. D.; Leaitch, W. Richard; Aliabadi, Amir A. Atmospheric Chemistry and Physics, Vol. 19, Issue 4 https://doi.org/10.5194/acp-19-2527-2019	journal	January 2019
Concentrations, composition, and sources of ice-nucleating particles in the Canadian High Arctic during spring 2016 Si, Meng; Evoy, Erin; Yun, Jingwei Atmospheric Chemistry and Physics, Vol. 19, Issue 5 https://doi.org/10.5194/acp-19-3007-2019	journal	January 2019
Annual variability of ice-nucleating particle concentrations at different Arctic locations Wex, Heike; Huang, Lin; Zhang, Wendy Atmospheric Chemistry and Physics, Vol. 19, Issue 7 https://doi.org/10.5194/acp-19-5293-2019	journal	January 2019
Ice-nucleating particles in a coastal tropical site Ladino, Luis A.; Raga, Graciela B.; Alvarez-Ospina, Harry Atmospheric Chemistry and Physics, Vol. 19, Issue 9 https://doi.org/10.5194/acp-19-6147-2019	journal	January 2019
Revisiting properties and concentrations of ice-nucleating particles in the sea surface microlayer and bulk seawater in the Canadian Arctic during summer Irish, Victoria E.; Hanna, Sarah J.; Xi, Yu Atmospheric Chemistry and Physics, Vol. 19, Issue 11 https://doi.org/10.5194/acp-19-7775-2019	journal	January 2019
Characterization of aerosol particles at Cabo Verde close to sea level and at the cloud level – Part 2: Ice-nucleating particles in air, cloud and seawater Gong, Xianda; Wex, Heike; van Pinxteren, Manuela Atmospheric Chemistry and Physics, Vol. 20, Issue 3 https://doi.org/10.5194/acp-20-1451-2020	journal	January 2020
Spatial and temporal variability in the ice-nucleating ability of alpine snowmelt and extension to frozen cloud fraction Brennan, Killian P.; David, Robert O.; Borduas-Dedekind, Nadine Atmospheric Chemistry and Physics, Vol. 20, Issue 1 https://doi.org/10.5194/acp-20-163-2020	journal	January 2020

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