STEM/EELS Study of Fission Product Transport in Neutron Irradiated TRISO Fuel Particles (NSUF report)
The objectives of this project are to study the distribution, composition and structure of fission products in neutron irradiated SiC layer of the TRISO particles, using electron microscopy including scanning transmission electron microscopy (STEM), energy dispersive x-ray spectroscopy (EDS), electron energy loss spectroscopy (EELS), high-resolution transmission electron microscopy (HRTEM) and precession electron diffraction (PED), in an effort to enhance the understanding of distribution, composition, structure and transport mechanisms of fission products. In the past 40 years, numerous studies, including reactor experiments, out-of-pile experiments, and simulations, have been performed to investigate the fission product transport behavior and mechanisms. Grain boundary (GB) diffusion, neutron-induced diffusion, catalytic Pd-assisted transport, and vapor-phase migration all have been suggested as possible governing transport mechanisms. The previous studies, however, have not been able to reproduce the transport behavior of fission products and the mechanisms remain poorly understood. This project is anticipated to contribute to enhancing the understanding of the mechanisms of fission product transport in irradiated SiC layer of the TRISO particles. Thorough understanding of fission product transport mechanisms in the SiC layer will improve fuel modeling and design and better SiC layers and TRISO coated particles can be designed to enhance retention of fission products and reduce their release. Eventually, TRISO coated particles with improved performance can be fabricated, and such advancement will expedite the qualifying and licensing processes for TRISO coated particles. Hence, this research is contributing to achieving the objectives of DOE-NE to develop the next generation nuclear reactors, particularly high-temperature gas reactors.
- Research Organization:
- Idaho National Lab. (INL), Idaho Falls, ID (United States)
- Sponsoring Organization:
- USDOE Office of Nuclear Energy (NE)
- DOE Contract Number:
- AC07-05ID14517
- OSTI ID:
- 1483612
- Report Number(s):
- INL/EXT-16-40709-Rev000
- Country of Publication:
- United States
- Language:
- English
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