High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media

Todt, Michael A.; Albert, Daniel R.; Davis, H. Floyd

doi:10.1063/1.4952749

Title: High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media

Abstract

A method is described for generating intense pulsed vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) laser radiation by resonance enhanced four-wave mixing of commercial pulsed nanosecond lasers in laser vaporized mercury under windowless conditions. By employing noncollinear mixing of the input beams, the need of dispersive elements such as gratings for separating the VUV/XUV from the residual UV and visible beams is eliminated. A number of schemes are described, facilitating access to the 9.9–14.6 eV range. A simple and convenient scheme for generating wavelengths of 125 nm, 112 nm, and 104 nm (10 eV, 11 eV, and 12 eV) using two dye lasers without the need for dye changes is described.

Authors:

Todt, Michael A. ^[1];

^[1]; Davis, H. Floyd ^[1]

Cornell Univ., Ithaca, NY (United States). Baker Lab., Dept. of Chemistry and Chemical Biology

Publication Date:: Mon Jun 13 00:00:00 EDT 2016

Research Org.:: Cornell Univ., Ithaca, NY (United States)

Sponsoring Org.:: USDOE; National Science Foundation (NSF)

OSTI Identifier:: 1471507

Alternate Identifier(s):: OSTI ID: 1256782

Grant/Contract Number:: FG02-00ER15095; CHE-1301156

Resource Type:: Journal Article: Accepted Manuscript

Journal Name:: Review of Scientific Instruments

Additional Journal Information:: Journal Volume: 87; Journal Issue: 6; Journal ID: ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)

Country of Publication:: United States

Language:: English

Subject:: 47 OTHER INSTRUMENTATION; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY

Citation Formats


                    Todt, Michael A., Albert, Daniel R., and Davis, H. Floyd. High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media.  United States: N. p., 2016. 
        Web.  doi:10.1063/1.4952749.

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                    Todt, Michael A., Albert, Daniel R., & Davis, H. Floyd. High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media.  United States.  https://doi.org/10.1063/1.4952749

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                    Todt, Michael A., Albert, Daniel R., and Davis, H. Floyd. 2016.  
        "High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media".  United States.  https://doi.org/10.1063/1.4952749.  https://www.osti.gov/servlets/purl/1471507.

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@article{osti_1471507,

  title        = {High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media},

  author       = {Todt, Michael A. and Albert, Daniel R. and Davis, H. Floyd},

  abstractNote = {A method is described for generating intense pulsed vacuum ultraviolet (VUV) and extreme ultraviolet (XUV) laser radiation by resonance enhanced four-wave mixing of commercial pulsed nanosecond lasers in laser vaporized mercury under windowless conditions. By employing noncollinear mixing of the input beams, the need of dispersive elements such as gratings for separating the VUV/XUV from the residual UV and visible beams is eliminated. A number of schemes are described, facilitating access to the 9.9–14.6 eV range. A simple and convenient scheme for generating wavelengths of 125 nm, 112 nm, and 104 nm (10 eV, 11 eV, and 12 eV) using two dye lasers without the need for dye changes is described.},

  doi          = {10.1063/1.4952749},

  url          = {https://www.osti.gov/biblio/1471507},
  journal      = {Review of Scientific Instruments},

  issn         = {0034-6748},

  number       = 6,

  volume       = 87,

  place        = {United States},

  year         = {Mon Jun 13 00:00:00 EDT 2016},

  month        = {Mon Jun 13 00:00:00 EDT 2016}

}

Copy to clipboard

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Works referenced in this record:

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Koudoumas, E.; Efthimiopoulos, T.
Laser Chemistry, Vol. 13, Issue 2
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Excitation of H2 using continuously tunable coherent XUV radiation (97.3–102.3 nm)
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High-intensity coherent vacuum ultraviolet source using unfocussed commercial dye lasers
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Albert, Daniel R.; Proctor, David L.; Floyd Davis, H.
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Generation of high-energy broadband femtosecond deep-ultraviolet pulses by highly nondegenerate noncollinear four-wave mixing in a thin transparent solid
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Lyman alpha (1216 Å) generation in krypton
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Hilbig, R.; Wallenstein, R.
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Tunable VUV radiation generated by two-photon resonant frequency mixing in xenon
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Hilbig, R.; Wallenstein, R.
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Broadly tunable vacuum-ultraviolet radiation source employing resonant enhanced sum–difference frequency mixing in krypton
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Frequency up-conversion to the VUV in Hg vapor
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Mahon, R.; Tomkins, F.
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Generation of 30-fs ultraviolet pulses by four-wave optical parametric chirped pulse amplification
journal, January 2010

Darginavicius, J.; Tamošauskas, G.; Piskarskas, A.
Optics Express, Vol. 18, Issue 15
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Efficient monochromator to isolate VUV light generated by four-wave mixing techniques
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Laser ablation for analytical sampling: what can we learn from modeling?
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Bogaerts, Annemie; Chen, Zhaoyang; Gijbels, Renaat
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High-efficiency, energy-scalable, coherent 130-nm source by four-wave mixing in Hg vapor
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Third-harmonic generation in argon, krypton, and xenon: Bandwidth limitations in the vicinity of Lyman-α
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Mahon, R.; McIlrath, T.; Myerscough, V.
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Capillary array: a new type of window for the vacuum ultraviolet
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Molecular gases as a source of coherent, tunable XUV radiation
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Hellner, L.; Lukasik, J.
Optics Communications, Vol. 51, Issue 5
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Isotope Effects in the Photoionization Yields and the Absorption Cross Sections for Acetylene, Propyne, and Propene
journal, September 1970

Person, James C.; Nicole, Paul P.
The Journal of Chemical Physics, Vol. 53, Issue 5
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Frequency tripling into the 720–1025‐Å region with pulsed free jets
journal, September 1987

Page, Ralph H.; Larkin, Robert J.; Kung, A. H.
Review of Scientific Instruments, Vol. 58, Issue 9
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VUV generation by frequency mixing in a mercury beam
journal, January 1996

Hector, R.; Meiwes-Broer, K. H.
Optics Communications, Vol. 123, Issue 1-3
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Energy transfer in mercury vapour following laser excitation of the 7 ¹ S ₀ state by two-photon absorption
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Bras, N.; Jeannet, J. C.; Perrin, D.
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Enhanced generation of vacuum-ultraviolet radiation by four-wave mixing in mercury using pulsed laser vaporization
journal, September 2007

Chénais, S.; Forget, S.; Philippet, L.
Applied Physics B, Vol. 89, Issue 2-3
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Applications of Coherent Vacuum Ultraviolet to Photofragment and Photoionization Spectroscopy
book, June 1991

Hepburn, John W.
Vacuum Ultraviolet Photoionization and Photodissociation of Molecules and Clusters
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Reflectance Spectra of Single Materials
book, January 2000

Hunter, W. R.
Vacuum Ultraviolet Spectroscopy
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Works referencing / citing this record:

Trapped Hg ⁺ ion crystal generated by isotope-selective photoionization
journal, January 2019

Liu, Qu; Zou, Hongxin; He, Xiaokang
Review of Scientific Instruments, Vol. 90, Issue 1
https://doi.org/10.1063/1.5068692

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Title: High intensity vacuum ultraviolet and extreme ultraviolet production by noncollinear mixing in laser vaporized media

Abstract

Citation Formats

Two-Photon Resonant Third Harmonic Generation IN Hg journal, January 1993

Pulsed free jets: novel nonlinear media for generation of vacuum ultraviolet and extreme ultraviolet radiation journal, September 1984

A broadly tunable extreme ultraviolet laser source with a 0.008 cm[sup −1] bandwidth journal, January 2000

Generation of coherent radiation at 89.6 nm through two-photon resonant phase-matched tripling of fourth-harmonic Nd: Glass laser radiation in Hg vapors journal, February 1978

Resonant sum and difference frequency mixing in Hg journal, December 1983

Broadband four-wave optical parametric amplification in bulk isotropic media in the ultraviolet journal, July 2009

Effects of focusing on third-order nonlinear processes in isotropic media journal, June 1975

Continuous Wave Coherent Lyman- α Radiation journal, November 1999

High-power Lyman-? source generated with an ArF excimer laser journal, January 1998

Tunable extreme-ultraviolet radiation from 105 to 875 nm using Hg vapor journal, January 1985

Third-harmonic generation in a pulsed supersonic jet of xenon journal, January 1983

Production of narrowband tunable extreme-ultraviolet radiation by noncollinear resonance-enhanced four-wave mixing journal, January 2005

Generation of high-energy vacuum UV femtosecond pulses by multiple-beam cascaded four-wave mixing in a transparent solid journal, January 2011

Gas-phase generation of resonance-enhanced third harmonic with crossed laser beams journal, December 2002

Ultranarrow bandwidth VUV‐XUV laser system journal, September 1989

Excitation of H2 using continuously tunable coherent XUV radiation (97.3–102.3 nm) journal, March 1983

High-intensity coherent vacuum ultraviolet source using unfocussed commercial dye lasers journal, June 2013

Generation of high-energy broadband femtosecond deep-ultraviolet pulses by highly nondegenerate noncollinear four-wave mixing in a thin transparent solid journal, March 2013

Windowless Vacuum-Ultraviolet Matrix Photolysis journal, July 1977

Development of a coherent vacuum ultraviolet source at 104–108 nm generated by four-wave sum frequency mixing in Hg vapor journal, May 2003

Lyman alpha (1216 Å) generation in krypton journal, July 1980

Narrowband tunable VUV radiation generated by nonresonant sum- and difference-frequency mixing in xenon and krypton journal, January 1982

Tunable VUV radiation generated by two-photon resonant frequency mixing in xenon journal, February 1983

Broadly tunable vacuum-ultraviolet radiation source employing resonant enhanced sum–difference frequency mixing in krypton journal, January 1990

Frequency up-conversion to the VUV in Hg vapor journal, May 1982

Generation of 30-fs ultraviolet pulses by four-wave optical parametric chirped pulse amplification journal, January 2010

Efficient monochromator to isolate VUV light generated by four-wave mixing techniques journal, January 1988

Laser ablation for analytical sampling: what can we learn from modeling? journal, November 2003

Practical guide for 7S resonant frequency mixing in mercury: generation of light in the 230–185-and 140–120-nm ranges journal, January 1987

Near-threshold absolute photoionization cross-sections of some reaction intermediates in combustion journal, February 2008

High-efficiency, energy-scalable, coherent 130-nm source by four-wave mixing in Hg vapor journal, January 1988

Vacuum ultraviolet oscillator strengths of Hg measured by sum-frequency mixing journal, May 1986

A very convenient setup to generate intense VUV coherent light at 125 nm with use of nonlinear effects in mercury vapor at room temperature journal, January 1995

Polarization properties of coherent VUV light at 125 nm generated by sum-frequency four-wave mixing in mercury journal, April 2000

Third-harmonic generation in argon, krypton, and xenon: Bandwidth limitations in the vicinity of Lyman-α journal, June 1979

Capillary array: a new type of window for the vacuum ultraviolet journal, January 1979

Molecular gases as a source of coherent, tunable XUV radiation journal, October 1984

Isotope Effects in the Photoionization Yields and the Absorption Cross Sections for Acetylene, Propyne, and Propene journal, September 1970

Frequency tripling into the 720–1025‐Å region with pulsed free jets journal, September 1987

VUV generation by frequency mixing in a mercury beam journal, January 1996

Energy transfer in mercury vapour following laser excitation of the 7 1 S 0 state by two-photon absorption journal, August 1993

Enhanced generation of vacuum-ultraviolet radiation by four-wave mixing in mercury using pulsed laser vaporization journal, September 2007

Applications of Coherent Vacuum Ultraviolet to Photofragment and Photoionization Spectroscopy book, June 1991

Reflectance Spectra of Single Materials book, January 2000

Trapped Hg + ion crystal generated by isotope-selective photoionization journal, January 2019

Two-Photon Resonant Third Harmonic Generation IN Hg
journal, January 1993

Pulsed free jets: novel nonlinear media for generation of vacuum ultraviolet and extreme ultraviolet radiation
journal, September 1984

A broadly tunable extreme ultraviolet laser source with a 0.008 cm[sup −1] bandwidth
journal, January 2000

Generation of coherent radiation at 89.6 nm through two-photon resonant phase-matched tripling of fourth-harmonic Nd: Glass laser radiation in Hg vapors
journal, February 1978

Resonant sum and difference frequency mixing in Hg
journal, December 1983

Broadband four-wave optical parametric amplification in bulk isotropic media in the ultraviolet
journal, July 2009

Effects of focusing on third-order nonlinear processes in isotropic media
journal, June 1975

Continuous Wave Coherent Lyman- $α$ Radiation
journal, November 1999

High-power Lyman-? source generated with an ArF excimer laser
journal, January 1998

Tunable extreme-ultraviolet radiation from 105 to 875 nm using Hg vapor
journal, January 1985

Third-harmonic generation in a pulsed supersonic jet of xenon
journal, January 1983

Production of narrowband tunable extreme-ultraviolet radiation by noncollinear resonance-enhanced four-wave mixing
journal, January 2005

Generation of high-energy vacuum UV femtosecond pulses by multiple-beam cascaded four-wave mixing in a transparent solid
journal, January 2011

Gas-phase generation of resonance-enhanced third harmonic with crossed laser beams
journal, December 2002

Ultranarrow bandwidth VUV‐XUV laser system
journal, September 1989

Excitation of H2 using continuously tunable coherent XUV radiation (97.3–102.3 nm)
journal, March 1983

High-intensity coherent vacuum ultraviolet source using unfocussed commercial dye lasers
journal, June 2013

Generation of high-energy broadband femtosecond deep-ultraviolet pulses by highly nondegenerate noncollinear four-wave mixing in a thin transparent solid
journal, March 2013

Windowless Vacuum-Ultraviolet Matrix Photolysis
journal, July 1977

Development of a coherent vacuum ultraviolet source at 104–108 nm generated by four-wave sum frequency mixing in Hg vapor
journal, May 2003

Lyman alpha (1216 Å) generation in krypton
journal, July 1980

Narrowband tunable VUV radiation generated by nonresonant sum- and difference-frequency mixing in xenon and krypton
journal, January 1982

Tunable VUV radiation generated by two-photon resonant frequency mixing in xenon
journal, February 1983

Broadly tunable vacuum-ultraviolet radiation source employing resonant enhanced sum–difference frequency mixing in krypton
journal, January 1990

Frequency up-conversion to the VUV in Hg vapor
journal, May 1982

Generation of 30-fs ultraviolet pulses by four-wave optical parametric chirped pulse amplification
journal, January 2010

Efficient monochromator to isolate VUV light generated by four-wave mixing techniques
journal, January 1988

Laser ablation for analytical sampling: what can we learn from modeling?
journal, November 2003

Practical guide for 7S resonant frequency mixing in mercury: generation of light in the 230–185-and 140–120-nm ranges
journal, January 1987

Near-threshold absolute photoionization cross-sections of some reaction intermediates in combustion
journal, February 2008

High-efficiency, energy-scalable, coherent 130-nm source by four-wave mixing in Hg vapor
journal, January 1988

Vacuum ultraviolet oscillator strengths of Hg measured by sum-frequency mixing
journal, May 1986

A very convenient setup to generate intense VUV coherent light at 125 nm with use of nonlinear effects in mercury vapor at room temperature
journal, January 1995

Polarization properties of coherent VUV light at 125 nm generated by sum-frequency four-wave mixing in mercury
journal, April 2000

Third-harmonic generation in argon, krypton, and xenon: Bandwidth limitations in the vicinity of Lyman-α
journal, June 1979

Capillary array: a new type of window for the vacuum ultraviolet
journal, January 1979

Molecular gases as a source of coherent, tunable XUV radiation
journal, October 1984

Isotope Effects in the Photoionization Yields and the Absorption Cross Sections for Acetylene, Propyne, and Propene
journal, September 1970

Frequency tripling into the 720–1025‐Å region with pulsed free jets
journal, September 1987

VUV generation by frequency mixing in a mercury beam
journal, January 1996

Energy transfer in mercury vapour following laser excitation of the 7 ¹ S ₀ state by two-photon absorption
journal, August 1993

Enhanced generation of vacuum-ultraviolet radiation by four-wave mixing in mercury using pulsed laser vaporization
journal, September 2007

Applications of Coherent Vacuum Ultraviolet to Photofragment and Photoionization Spectroscopy
book, June 1991

Reflectance Spectra of Single Materials
book, January 2000

Trapped Hg ⁺ ion crystal generated by isotope-selective photoionization
journal, January 2019