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Title: Aluminum Clad Spent Nuclear Fuel Task 2: Oxide Layer Radiolytic Gas Generation Resolution Experiment Test Plan

Technical Report ·
DOI:https://doi.org/10.2172/1469387· OSTI ID:1469387
 [1]
  1. Idaho National Lab. (INL), Idaho Falls, ID (United States)

This document presents the test plan for Task 2 of the Aluminum Clad Spent Nuclear Fuel Long Term Dry Storage Technical Issues Action Plan. This task’s overarching goal is the resolution of gas generation resulting from the radiolytic degradation of the oxide layers on aluminum. The uncertainty associated with the build-up of gaseous radiolytic products inside the ASNF storage canisters is one of the dominant technical challenges associated with long term dry storage of aluminum clad fuel. The objectives of the Task 2 test plan are to: 1. Understand how radiation chemistry inside the ASNF dry storage canister impacts extended dry storage performance. 2. Understand the radiation induced mechanisms governing the production of radiolytic gases and alteration of gas composition within a canister. 3. Correlate the observed changes in material properties of ASNF with the radiolytic degradation of aluminum oxide in fill environments of variable moisture and gas composition. 4. Compile a predictive kinetic modeling tool, to provide quantitative mechanistic insight into the in-cask radiation chemistry of ASNF. 5. Interface with the canister modeling activity of Task 3 to deliver degradation rates for package performance of both sealed and vented scenarios.

Research Organization:
Idaho National Lab. (INL), Idaho Falls, ID (United States)
Sponsoring Organization:
USDOE Office of Environmental Management (EM)
DOE Contract Number:
AC07-05ID14517
OSTI ID:
1469387
Report Number(s):
INL/EXT-18-45858-Rev000; TRN: US1902592
Country of Publication:
United States
Language:
English