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Title: Theoretical analysis of mixing in liquid clouds – Part 3: Inhomogeneous mixing

Journal Article · · Atmospheric Chemistry and Physics (Online)
 [1];  [1];  [2]
  1. Hebrew Univ. of Jerusalem (Israel). Dept. of Atmospheric Sciences
  2. Environment Canada, Toronto, ON (Canada). Cloud Physics and Severe Weather Section

An idealized diffusion–evaporation model of time-dependent mixing between a cloud volume and a droplet-free volume is analyzed. The initial droplet size distribution (DSD) in the cloud volume is assumed to be monodisperse. It is shown that evolution of the microphysical variables and the final equilibrium state are unambiguously determined by two non-dimensional parameters. The first one is the potential evaporation parameter R, proportional to the ratio of the saturation deficit to the liquid water content in the cloud volume, that determines whether the equilibrium state is reached at 100 % relative humidity, or is characterized by a complete evaporation of cloud droplets. The second parameter Da is the Damkölher number equal to the ratio of the characteristic mixing time to the phase relaxation time. Parameters R and Da determine the type of mixing. The results are analyzed within a wide range of values of R and Da. It is shown that there is no pure homogeneous mixing, since the first mixing stage is always inhomogeneous. The mixing type can change during the mixing process. Any mixing type leads to formation of a tail of small droplets in DSD and, therefore, to DSD broadening that depends on Da. At large Da, the final DSD dispersion can be as large as 0.2. The total duration of mixing varies from several to 100 phase relaxation time periods, depending on R and Da. The definitions of homogeneous and inhomogeneous types of mixing are reconsidered and clarified, enabling a more precise delimitation between them. The paper also compares the results obtained with those based on the classic mixing concepts.

Research Organization:
Hebrew Univ. of Jerusalem (Israel)
Sponsoring Organization:
USDOE Office of Science (SC), Biological and Environmental Research (BER); Israel Science Foundation (ISF); United States-Israel Binational Science Foundation (BSF)
Grant/Contract Number:
SC0006788; 1393/14; 2010446
OSTI ID:
1436586
Journal Information:
Atmospheric Chemistry and Physics (Online), Vol. 16, Issue 14; ISSN 1680-7324
Publisher:
European Geosciences UnionCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 32 works
Citation information provided by
Web of Science

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Cited By (6)

Cloud Edge Properties Measured by the ARM Shortwave Spectrometer Over Ocean and Land journal August 2019
Theoretical study of mixing in liquid clouds – Part 1: Classical concepts journal January 2016
Theoretical analysis of mixing in liquid clouds – Part IV: DSD evolution and mixing diagrams journal January 2018
Observation of turbulent dispersion of artificially released SO2 puffs with UV cameras journal January 2018
Interactive comment on “Illustration of microphysical processes in Amazonian deep convective clouds in the Gamma phase space: Introduction and potential applications” by Micael A. Cecchini et al. journal September 2017
Influence of low-level blocking and turbulence on the microphysics of a mixed-phase cloud in an inner-Alpine valley journal September 2020

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