Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam

Zhou, Haiqing; Yu, Fang; Huang, Yufeng; Sun, Jingying; Zhu, Zhuan; Nielsen, Robert J.; He, Ran; Bao, Jiming; Goddard III, William A.; Chen, Shuo; Ren, Zhifeng

doi:10.1038/ncomms12765

Title: Efficient hydrogen evolution by ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam

Journal Article · Fri Sep 16 00:00:00 EDT 2016 · Nature Communications

DOI:https://doi.org/10.1038/ncomms12765· OSTI ID:1435783

Zhou, Haiqing ^[1]; Yu, Fang ^[1]; Huang, Yufeng ^[2]; Sun, Jingying ^[1]; Zhu, Zhuan ^[3]; Nielsen, Robert J. ^[2]; He, Ran ^[1];

^[3]; Goddard III, William A. ^[2]; Chen, Shuo ^[1]; Ren, Zhifeng ^[1]

Univ. of Houston, Houston, TX (United States). Dept. of Physics and Texas Center for Superconductivity (TcSUH)
California Inst. of Technology (CalTech), Pasadena, CA (United States). Materials and Process Simulation Center
Univ. of Houston, Houston, TX (United States). Dept. of Electrical and Computer Engineering

With the massive consumption of fossil fuels and its detrimental impact on the environment, methods of generating clean power are urgent. Hydrogen is an ideal carrier for renewable energy; however, hydrogen generation is inefficient because of the lack of robust catalysts that are substantially cheaper than platinum. Therefore, robust and durable earth-abundant and cost-effective catalysts are desirable for hydrogen generation from water splitting via hydrogen evolution reaction. In this paper, we report an active and durable earth-abundant transition metal dichalcogenide-based hybrid catalyst that exhibits high hydrogen evolution activity approaching the state-of-the-art platinum catalysts, and superior to those of most transition metal dichalcogenides (molybdenum sulfide, cobalt diselenide and so on). Our material is fabricated by growing ternary molybdenum sulfoselenide particles on self-standing porous nickel diselenide foam. This advance provides a different pathway to design cheap, efficient and sizable hydrogen-evolving electrode by simultaneously tuning the number of catalytic edge sites, porosity, heteroatom doping and electrical conductivity.

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Research Organization:: California Institute of Technology (CalTech), Pasadena, CA (United States); Univ. of Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC); Defense Threat Reduction Agency (DTRA); National Science Foundation (NSF); Welch Foundation, Houston, TX (United States)

Grant/Contract Number:: SC0004993; FA 7000-13-1-0001; ECCS-1240510; E-1728

OSTI ID:: 1435783

Journal Information:: Nature Communications, Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 262 works

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MoS2 Decorated Carbon Nanofibers as Efficient and Durable Electrocatalyst for Hydrogen Evolution Reaction Zhang, C.; Wang, Z.; Bhoyate, S. C, Vol. 3, Issue 4 https://doi.org/10.3390/c3040033	journal	October 2017
Fabrication of Robust Hydrogen Evolution Reaction Electrocatalyst Using Ag2Se by Vacuum Evaporation Hussain, Sajjad; Chae, Jinwoong; Akbar, Kamran Nanomaterials, Vol. 9, Issue 10 https://doi.org/10.3390/nano9101460	journal	October 2019
Electronically Double‐Layered Metal Boride Hollow Nanoprism as an Excellent and Robust Water Oxidation Electrocatalysts Han, HyukSu; Hong, Yu‐Rim; Woo, Jungwook Advanced Energy Materials, Vol. 9, Issue 15 https://doi.org/10.1002/aenm.201900736	journal	February 2019
A structurally versatile nickel phosphite acting as a robust bifunctional electrocatalyst for overall water splitting Menezes, Prashanth W.; Panda, Chakadola; Loos, Stefan Freie Universität Berlin https://doi.org/10.17169/refubium-1718	text	January 2018
Helical cobalt borophosphates to master durable overall water-splitting Menezes, Prashanth W.; Indra, Arindam; Zaharieva, Ivelina Freie Universität Berlin https://doi.org/10.17169/refubium-25605	text	January 2019
Facile Synthesis of Molybdenum Diselenide Layers for High-Performance Hydrogen Evolution Electrocatalysts Vikraman, Dhanasekaran; Hussain, Sajjad; Akbar, Kamran ACS Omega, Vol. 3, Issue 5 https://doi.org/10.1021/acsomega.8b00459	journal	May 2018
Synthesis of Mo2C and W2C Nanoparticle Electrocatalysts for the Efficient Hydrogen Evolution Reaction in Alkali and Acid Electrolytes Hussain, Sajjad; Vikraman, Dhanasekaran; Feroze, Asad Frontiers in Chemistry, Vol. 7 https://doi.org/10.3389/fchem.2019.00716	journal	October 2019

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