Imaging Spectroscopy: A Novel Use for the Velocity Mapped Ion Imaging Technique.
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
The ability to measure the velocity of neutral atoms and molecules with a precision of several meter/sec provides an opportunity to measure subtle perturbations on electronic states with high resolution. Using Velocity Mapped Ion Imaging we are able to measure induced perturbations of electronic states such as broadening and magnetic and electric field splittings . We demonstrate this ability utilizing the 5s[3/2]2 → 5p[5/2]3 cycling transition at 811.5 nm in metastable Kr atoms to investigate the saturation broadening caused by Rabi cycling on a resonant transition with MHz resolution. In addition we investigate the lifetime broadening associated with ionization from the cycling states and the Zeeman splitting of the states. We discuss the inherent limits to resolution obtained with this technique.
- Research Organization:
- Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- DOE Contract Number:
- AC04-94AL85000
- OSTI ID:
- 1429739
- Report Number(s):
- SAND-2017-1901J; 653976
- Country of Publication:
- United States
- Language:
- English
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