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Title: In-pile Thermal Conductivity Characterization with Time Resolved Raman

Technical Report ·
DOI:https://doi.org/10.2172/1427519· OSTI ID:1427519
 [1];  [2]
  1. Iowa State Univ., Ames, IA (United States). Dept. of Mechanical Engineering
  2. Idaho National Lab. (INL), Idaho Falls, ID (United States)

The project is designed to achieve three objectives: (1) Develop a novel time resolved Raman technology for direct measurement of fuel and cladding thermal conductivity. (2) Validate and improve the technology development by measuring ceramic materials germane to the nuclear industry. (3) Conduct instrumentation development to integrate optical fiber into our sensing system for eventual in-pile measurement. We have developed three new techniques: time-domain differential Raman (TD-Raman), frequency-resolved Raman (FR-Raman), and energy transport state-resolved Raman (ET-Raman). The TD-Raman varies the laser heating time and does simultaneous Raman thermal probing, the FR-Raman probes the material’s thermal response under periodical laser heating of different frequencies, and the ET-Raman probes the thermal response under steady and pulsed laser heating. The measurement capacity of these techniques have been fully assessed and verified by measuring micro/nanoscale materials. All these techniques do not need the data of laser absorption and absolute material temperature rise, yet still be able to measure the thermal conductivity and thermal diffusivity with unprecedented accuracy. It is expected they will have broad applications for in-pile thermal characterization of nuclear materials based on pure optical heating and sensing.

Research Organization:
Iowa State Univ., Ames, IA (United States); Idaho National Lab. (INL), Idaho Falls, ID (United States)
Sponsoring Organization:
USDOE Office of Nuclear Energy (NE)
DOE Contract Number:
NE0000671
OSTI ID:
1427519
Country of Publication:
United States
Language:
English