Transient Negative Optical Nonlinearity of Indium Oxide Nanorod Arrays in the Full-Visible Range

Guo, Peijun; Chang, Robert P. H.; Schaller, Richard D.

doi:10.1021/acsphotonics.7b00278

Title: Transient Negative Optical Nonlinearity of Indium Oxide Nanorod Arrays in the Full-Visible Range

Journal Article · Fri Jun 09 00:00:00 EDT 2017 · ACS Photonics

DOI:https://doi.org/10.1021/acsphotonics.7b00278· OSTI ID:1406113

^[1]; Chang, Robert P. H. ^[2];

^[3]

Argonne National Lab. (ANL), Lemont, IL (United States)
Northwestern Univ., Evanston, IL (United States)
Argonne National Lab. (ANL), Lemont, IL (United States); Northwestern Univ., Evanston, IL (United States)

Dynamic control of the optical response of materials at visible wavelengths is key to future metamaterials and photonic integrated circuits. Here we demonstrate large amplitude, negative optical nonlinearity (Δn from -0.05 to -0.09) of indium oxide nanorod arrays in the full-visible range. We experimentally quantify and theoretically calculate the optical nonlinearity, which arises from the modifications of interband optical transitions. Furthermore, the approach towards negative optical nonlinearity can be generalized to other transparent semiconductors and opens door to reconfigurable, sub-wavelength optical components.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22), Scientific User Facilities Division

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1406113

Journal Information:: ACS Photonics, Vol. 4, Issue 6; ISSN 2330-4022

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 10 works

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36 MATERIALS SCIENCE
37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
negative optical nonlinearity
transient
full-visible range
indium oxide
transparent semiconducting oxide
ultrafast

Title: Transient Negative Optical Nonlinearity of Indium Oxide Nanorod Arrays in the Full-Visible Range

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