Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance

Yan, Jun; Ren, Chang E.; Maleski, Kathleen; Hatter, Christine B.; Anasori, Babak; Urbankowski, Patrick; Sarycheva, Asya; Gogotsi, Yury G.

doi:10.1002/adfm.201701264

Title: Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance

Journal Article · Fri Jun 30 00:00:00 EDT 2017 · Advanced Functional Materials

DOI:https://doi.org/10.1002/adfm.201701264· OSTI ID:1399231

^[1]; Ren, Chang E. ^[2]; Maleski, Kathleen ^[2]; Hatter, Christine B. ^[2]; Anasori, Babak ^[2]; Urbankowski, Patrick ^[2]; Sarycheva, Asya ^[2];

^[2]

Drexel Univ., Philadelphia, PA (United States); Harbin Engineering Univ., Harbin (China)
Drexel Univ., Philadelphia, PA (United States)

A strategy to prepare flexible and conductive MXene/graphene (reduced graphene oxide, rGO) supercapacitor electrodes by using electrostatic self‐assembly between positively charged rGO modified with poly(diallyldimethylammonium chloride) and negatively charged titanium carbide MXene nanosheets is presented. After electrostatic assembly, rGO nanosheets are inserted in‐between MXene layers. As a result, the self‐restacking of MXene nanosheets is effectively prevented, leading to a considerably increased interlayer spacing. Accelerated diffusion of electrolyte ions enables more electroactive sites to become accessible. The freestanding MXene/rGO‐5 wt% electrode displays a volumetric capacitance of 1040 F cm ⁻³ at a scan rate of 2 mV s ⁻¹ , an impressive rate capability with 61% capacitance retention at 1 V s ⁻¹ and long cycle life. Moreover, the fabricated binder‐free symmetric supercapacitor shows an ultrahigh volumetric energy density of 32.6 Wh L ⁻¹ , which is among the highest values reported for carbon and MXene based materials in aqueous electrolytes. This work provides fundamental insight into the effect of interlayer spacing on the electrochemical performance of 2D hybrid materials and sheds light on the design of next‐generation flexible, portable and highly integrated supercapacitors with high volumetric and rate performances.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Energy Frontier Research Centers (EFRC) (United States). Fluid Interface Reactions, Structures and Transport Center (FIRST)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1399231

Alternate ID(s):: OSTI ID: 1401090

Journal Information:: Advanced Functional Materials, Vol. 27; ISSN 1616-301X

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 1151 works

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MXene-derived TiO ₂ /reduced graphene oxide composite with an enhanced capacitive capacity for Li-ion and K-ion batteries Fang, Yongzheng; Hu, Rong; Liu, Boya Journal of Materials Chemistry A, Vol. 7, Issue 10 https://doi.org/10.1039/c8ta12069b	journal	January 2019
Effect of the cobalt and zinc ratio on the preparation of zeolitic imidazole frameworks (ZIFs): synthesis, characterization and supercapacitor applications Chul, Ha Dong; Vinodh, Rajangam; Muralee Gopi, Chandu V. V. Dalton Transactions, Vol. 48, Issue 39 https://doi.org/10.1039/c9dt03306h	journal	January 2019
A recyclable route to produce biochar with a tailored structure and surface chemistry for enhanced charge storage Zhang, Mengdi; Yu, Chang; Ling, Zheng Green Chemistry, Vol. 21, Issue 8 https://doi.org/10.1039/c9gc00655a	journal	January 2019
Highly fluorescent Ti ₃ C ₂ MXene quantum dots for macrophage labeling and Cu ²⁺ ion sensing Guan, Qingwen; Ma, Junfei; Yang, Wenjing Nanoscale, Vol. 11, Issue 30 https://doi.org/10.1039/c9nr04421c	journal	January 2019
Room temperature ultrafast synthesis of N- and O-rich graphene films with an expanded interlayer distance for high volumetric capacitance supercapacitors Huang, Cong; Hu, Aiping; Li, Yanhua Nanoscale, Vol. 11, Issue 35 https://doi.org/10.1039/c9nr06001d	journal	January 2019
Exploring the microscopic mechanism of pseudocapacitance with electronic structures in monolayer 1T-MoS 2 electrodes for supercapacitors Zhang, Zhenzhou; Wu, Maokun; Wang, Lijing Materials Chemistry Frontiers, Vol. 3, Issue 7 https://doi.org/10.1039/c9qm00060g	journal	January 2019
Nitrogen-doped carbon sheets coated on CoNiO ₂ @textile carbon as bifunctional electrodes for asymmetric supercapacitors Guo, Rui; Li, Jing; Jia, Yufeng Journal of Materials Chemistry A, Vol. 7, Issue 8 https://doi.org/10.1039/c9ta00014c	journal	January 2019
Surface nitrogen-modified 2D titanium carbide (MXene) with high energy density for aqueous supercapacitor applications Tian, Yapeng; Que, Wenxiu; Luo, Yangyang Journal of Materials Chemistry A, Vol. 7, Issue 10 https://doi.org/10.1039/c9ta00076c	journal	January 2019
Pursuit of a high-capacity and long-life Mg-storage cathode by tailoring sandwich-structured MXene@carbon nanosphere composites Liu, Fanfan; Liu, Yongchang; Zhao, Xudong Journal of Materials Chemistry A, Vol. 7, Issue 28 https://doi.org/10.1039/c9ta02212k	journal	January 2019
Multivalent metal ion hybrid capacitors: a review with a focus on zinc-ion hybrid capacitors Dong, Liubing; Yang, Wang; Yang, Wu Journal of Materials Chemistry A, Vol. 7, Issue 23 https://doi.org/10.1039/c9ta02678a	journal	January 2019
Anionic P-substitution toward ternary Ni–S–P nanoparticles immobilized graphene with ultrahigh rate and long cycle life for hybrid supercapacitors Jiang, Bing; Ban, Xiaohan; Wang, Qian Journal of Materials Chemistry A, Vol. 7, Issue 42 https://doi.org/10.1039/c9ta09902f	journal	January 2019
Hierarchical self-assembly flower-like ammonium nickel phosphate as high-rate performance electrode material for asymmetric supercapacitors with enhanced energy density Wang, Zhuang; Gu, Jianmin; Liu, Xin Nanotechnology, Vol. 29, Issue 42 https://doi.org/10.1088/1361-6528/aad75f	journal	August 2018
Excellent air and water stability of two-dimensional black phosphorene/MXene heterostructure Li, Hua; Lian, Peichao; Lu, Qiuju Materials Research Express, Vol. 6, Issue 6 https://doi.org/10.1088/2053-1591/ab0b84	journal	March 2019
NiFe ₂ O ₄ nanoparticles on reduced graphene oxide for supercapacitor electrodes with improved capacitance Cai, Yong-Zhu; Cao, Wen-Qiang; He, Peng Materials Research Express, Vol. 6, Issue 10 https://doi.org/10.1088/2053-1591/ab3fff	journal	September 2019
Facile Synthesis of MXene/Electrochemically Reduced Graphene Oxide Composites and Their Application for Electrochemical Sensing of Carbendazim Xie, Yu; Gao, Feng; Tu, Xiaolong Journal of The Electrochemical Society, Vol. 166, Issue 16 https://doi.org/10.1149/2.0091916jes	journal	January 2019
Two-Dimensional Titanium Carbides (Ti3C2Tx) Functionalized by Poly(m-phenylenediamine) for Efficient Adsorption and Reduction of Hexavalent Chromium Jin, Linfeng; Chai, Liyuan; Yang, Weichun International Journal of Environmental Research and Public Health, Vol. 17, Issue 1 https://doi.org/10.3390/ijerph17010167	journal	December 2019
Hydrothermal Synthesis of Co-Doped NiSe2 Nanowire for High-Performance Asymmetric Supercapacitors Gu, Yun; Fan, Le-Qing; Huang, Jian-Ling Materials, Vol. 11, Issue 8 https://doi.org/10.3390/ma11081468	journal	August 2018
Electromagnetic Shielding by MXene-Graphene-PVDF Composite with Hydrophobic, Lightweight and Flexible Graphene Coated Fabric Raagulan, Kanthasamy; Braveenth, Ramanaskanda; Jang, Hee Materials, Vol. 11, Issue 10 https://doi.org/10.3390/ma11101803	journal	September 2018
Fabrication of Flexible, Lightweight, Magnetic Mushroom Gills and Coral-Like MXene–Carbon Nanotube Nanocomposites for EMI Shielding Application Raagulan, Kanthasamy; Braveenth, Ramanaskanda; Ro Lee, Lee Nanomaterials, Vol. 9, Issue 4 https://doi.org/10.3390/nano9040519	journal	April 2019
Stamping of Flexible, Coplanar Micro-Supercapacitors Using MXene Inks Zhang, Chuanfang John; Kremer, Matthias P.; Seral-Ascaso, Andrés Advanced Functional Materials, Vol. 28, Issue 9 https://doi.org/10.1002/adfm.201705506	journal	January 2018
Engineering 3D Ion Transport Channels for Flexible MXene Films with Superior Capacitive Performance Wang, Yuanming; Wang, Xue; Li, Xiaolong Advanced Functional Materials, Vol. 29, Issue 14 https://doi.org/10.1002/adfm.201900326	journal	February 2019
3D Macroscopic Architectures from Self‐Assembled MXene Hydrogels Shang, Tongxin; Lin, Zifeng; Qi, Changsheng Advanced Functional Materials, Vol. 29, Issue 33 https://doi.org/10.1002/adfm.201903960	journal	June 2019
Pristine Titanium Carbide MXene Films with Environmentally Stable Conductivity and Superior Mechanical Strength Chen, Hongwu; Wen, Yeye; Qi, Yingyi Advanced Functional Materials, Vol. 30, Issue 5 https://doi.org/10.1002/adfm.201906996	journal	November 2019
3D Printing of Freestanding MXene Architectures for Current‐Collector‐Free Supercapacitors Yang, Wenji; Yang, Jie; Byun, Jae Jong Advanced Materials, Vol. 31, Issue 37 https://doi.org/10.1002/adma.201902725	journal	July 2019
Ultrastrong and Highly Conductive MXene‐Based Films for High‐Performance Electromagnetic Interference Shielding Liu, Ji; Liu, Zhangshuo; Zhang, Hao‐Bin Advanced Electronic Materials, Vol. 6, Issue 1 https://doi.org/10.1002/aelm.201901094	journal	November 2019
Scalable Water-Based Production of Highly Conductive 2D Nanosheets with Ultrahigh Volumetric Capacitance and Rate Capability Jeon, Hyeonyeol; Jeong, Jae-Min; Kang, Heon Gyu Advanced Energy Materials, Vol. 8, Issue 18 https://doi.org/10.1002/aenm.201800227	journal	March 2018
Flexible Nitrogen-Doped 2D Titanium Carbides (MXene) Films Constructed by an Ex Situ Solvothermal Method with Extraordinary Volumetric Capacitance Yang, Chenhui; Tang, Yi; Tian, Yapeng Advanced Energy Materials, Vol. 8, Issue 31 https://doi.org/10.1002/aenm.201802087	journal	September 2018
Ultrahigh-Capacity and Fire-Resistant LiFePO ₄ -Based Composite Cathodes for Advanced Lithium-Ion Batteries Li, Heng; Peng, Long; Wu, Dabei Advanced Energy Materials, Vol. 9, Issue 10 https://doi.org/10.1002/aenm.201802930	journal	January 2019
High‐Performance Electrocatalytic Conversion of N ₂ to NH ₃ Using Oxygen‐Vacancy‐Rich TiO ₂ In Situ Grown on Ti ₃ C ₂ T _x MXene Fang, Yanfeng; Liu, Zaichun; Han, Jingrui Advanced Energy Materials, Vol. 9, Issue 16 https://doi.org/10.1002/aenm.201803406	journal	February 2019
Hydrous RuO ₂ ‐Decorated MXene Coordinating with Silver Nanowire Inks Enabling Fully Printed Micro‐Supercapacitors with Extraordinary Volumetric Performance Li, Hongpeng; Li, Xiran; Liang, Jiajie Advanced Energy Materials, Vol. 9, Issue 15 https://doi.org/10.1002/aenm.201803987	journal	February 2019
Regulating Fast Anionic Redox for High-Voltage Aqueous Hydrogen-Ion-based Energy Storage Wang, Shengping; Zhao, Xiaoli; Yan, Xiaojun Angewandte Chemie, Vol. 131, Issue 1 https://doi.org/10.1002/ange.201811220	journal	December 2018
Recent Progress of MXene-Based Nanomaterials in Flexible Energy Storage and Electronic Devices Yang, Qi; Wang, Yukun; Li, Xinliang Energy & Environmental Materials, Vol. 1, Issue 4 https://doi.org/10.1002/eem2.12023	journal	December 2018
A Conductive and Highly Deformable All-Pseudocapacitive Composite Paper as Supercapacitor Electrode with Improved Areal and Volumetric Capacitance Zhou, Jie; Yu, Jiali; Shi, Ludi Small, Vol. 14, Issue 51 https://doi.org/10.1002/smll.201803786	journal	November 2018
Freestanding Lamellar Porous Carbon Stacks for Low‐Temperature‐Foldable Supercapacitors Yang, Yu; Ng, Sze‐Wing; Chen, Dongdong Small, Vol. 15, Issue 48 https://doi.org/10.1002/smll.201902071	journal	July 2019
Room‐Temperature Liquid Metal Confined in MXene Paper as a Flexible, Freestanding, and Binder‐Free Anode for Next‐Generation Lithium‐Ion Batteries Wei, Chuanliang; Fei, Huifang; Tian, Yuan Small, Vol. 15, Issue 46 https://doi.org/10.1002/smll.201903214	journal	October 2019
Construction of cobaltous oxide/nickel–iron oxide electrodes with great cycle stability and high energy density for advanced asymmetry supercapacitor Zhao, Yan; Chen, Yuan; Liu, Qingqing Journal of Materials Science: Materials in Electronics, Vol. 30, Issue 24 https://doi.org/10.1007/s10854-019-02495-3	journal	November 2019
Electromagnetic simulation of MXene-based plasmonic metamaterials with enhanced optical absorption Jakšić, Zoran; Obradov, Marko; Tanasković, Dragan Optical and Quantum Electronics, Vol. 52, Issue 2 https://doi.org/10.1007/s11082-020-2227-8	journal	January 2020
A 2.4-V asymmetric supercapacitor based on cation-intercalated manganese oxide nanosheets in a low-cost “water-in-salt” electrolyte Bu, Xudong; Zhang, Yurong; Su, Lijun Ionics, Vol. 25, Issue 12 https://doi.org/10.1007/s11581-019-03141-y	journal	July 2019
Microfluidic-spinning construction of black-phosphorus-hybrid microfibres for non-woven fabrics toward a high energy density flexible supercapacitor Wu, Xingjiang; Xu, Yijun; Hu, Ying Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06914-7	journal	November 2018
Polyoxometalate-coupled MXene nanohybrid via poly(ionic liquid) linkers and its electrode for enhanced supercapacitive performance Chen, Shu; Xiang, Yuanfang; Banks, M. Katherine Nanoscale, Vol. 10, Issue 42 https://doi.org/10.1039/c8nr05760e	journal	January 2018
Electrolyte-assisted hydrothermal synthesis of holey graphene films for all-solid-state supercapacitors Liu, Daoqing; Li, Qianwei; Zhao, Huazhang Journal of Materials Chemistry A, Vol. 6, Issue 24 https://doi.org/10.1039/c8ta02580k	journal	January 2018
Surface modification of biomass-derived hard carbon by grafting porous carbon nanosheets for high-performance supercapacitors Dong, Shian; He, Xiaojun; Zhang, Hanfang Journal of Materials Chemistry A, Vol. 6, Issue 33 https://doi.org/10.1039/c8ta04080j	journal	January 2018
Editable asymmetric all-solid-state supercapacitors based on high-strength, flexible, and programmable 2D-metal–organic framework/reduced graphene oxide self-assembled papers Cheng, Junye; Chen, Shengmei; Chen, Da Journal of Materials Chemistry A, Vol. 6, Issue 41 https://doi.org/10.1039/c8ta06785f	journal	January 2018
Silicon quantum dot-assisted synthesis of MoS ₂ /rGO sandwich structures with excellent supercapacitive performance Wu, Jinzhu; Li, Beibei; Feng, Yaxiu New Journal of Chemistry, Vol. 43, Issue 22 https://doi.org/10.1039/c9nj01232j	journal	January 2019
A fully inkjet-printed transparent humidity sensor based on a Ti ₃ C ₂ /Ag hybrid for touchless sensing of finger motion Li, Ning; Jiang, Yue; Xiao, Yan Nanoscale, Vol. 11, Issue 44 https://doi.org/10.1039/c9nr06751e	journal	January 2019
Macroporous three-dimensional MXene architectures for highly efficient solar steam generation Zhao, Xing; Zha, Xiang-Jun; Pu, Jun-Hong Journal of Materials Chemistry A, Vol. 7, Issue 17 https://doi.org/10.1039/c9ta00176j	journal	January 2019
Designing chemical bonds between active materials and current collectors for packaging a high-performance supercapacitor Wang, Haoxiang; Yang, He; Wang, Dong Nanotechnology, Vol. 31, Issue 10 https://doi.org/10.1088/1361-6528/ab5a07	journal	December 2019
Effects of biaxial strain and functional groups on SiC/ti ₃ C ₂ heterostructure: a first principle calculation Li, Chenliang; Tian, Bingkun; Yang, Yong Materials Research Express, Vol. 6, Issue 12 https://doi.org/10.1088/2053-1591/ab49c8	journal	November 2019
Interfacial and electronic properties of heterostructures of MXene and graphene Li, Rui; Sun, Weiwei; Zhan, Cheng Physical Review B, Vol. 99, Issue 8 https://doi.org/10.1103/physrevb.99.085429	journal	February 2019
2D/2D SnS ₂ /MoS ₂ layered heterojunction for enhanced supercapacitor performance Wang, Bo; Hu, Rong; Zhang, Jun Journal of the American Ceramic Society, Vol. 103, Issue 2 https://doi.org/10.1111/jace.16778	journal	September 2019
Advances in Two-Dimensional MXenes for Nitrogen Electrocatalytic Reduction to Ammonia Yu, Lan-lan; Qin, Jiang-zhou; Zhao, Wen-jun International Journal of Photoenergy, Vol. 2020 https://doi.org/10.1155/2020/5251431	journal	February 2020
Strategies to Enhance the Performance of Electrochemical Capacitors Based on Carbon Materials Salinas-Torres, David; Ruiz-Rosas, Ramiro; Morallón, Emilia Frontiers in Materials, Vol. 6 https://doi.org/10.3389/fmats.2019.00115	journal	May 2019
Hollow MXene Sphere/Reduced Graphene Aerogel Composites for Piezoresistive Sensor with Ultra‐High Sensitivity Zhu, Meng; Yue, Yang; Cheng, Yongfa Advanced Electronic Materials, Vol. 6, Issue 2 https://doi.org/10.1002/aelm.201901064	journal	December 2019
Two‐Dimensional Transition Metal Carbides and Nitrides (MXenes): Synthesis, Properties, and Electrochemical Energy Storage Applications Zhang, Chuanfang (John); Ma, Yonglu; Zhang, Xuetao ENERGY & ENVIRONMENTAL MATERIALS, Vol. 3, Issue 1 https://doi.org/10.1002/eem2.12058	journal	March 2020
Highly Conductive Ti ₃ C ₂ T _x MXene Hybrid Fibers for Flexible and Elastic Fiber-Shaped Supercapacitors Zhang, Jizhen; Seyedin, Shayan; Qin, Si Small, Vol. 15, Issue 8 https://doi.org/10.1002/smll.201804732	journal	January 2019
A nanoporous MXene film enables flexible supercapacitors with high energy storage Fan, Zhimin; Wang, Youshan; Xie, Zhimin Nanoscale, Vol. 10, Issue 20 https://doi.org/10.1039/c8nr01550c	journal	January 2018
Ti ₂ C ₃ T _x nanosheets as photothermal agents for near-infrared responsive hydrogels Yang, Changyu; Xu, Danyun; Peng, WenChao Nanoscale, Vol. 10, Issue 32 https://doi.org/10.1039/c8nr05301d	journal	January 2018
Mixed transition metal oxide nanowire arrays enabling hybrid capacitor performance enhancement Zhao, Depeng; Dai, Meizhen; Tong, Yongli CrystEngComm, Vol. 21, Issue 38 https://doi.org/10.1039/c9ce01169b	journal	January 2019
The solvent-free mechanochemical synthesis of mildly oxidized graphene oxide and its application as a novel conductive surfactant Chen, Jianhui; Chen, Wufeng; Song, Dongcheng New Journal of Chemistry, Vol. 43, Issue 18 https://doi.org/10.1039/c9nj00529c	journal	January 2019
Few-layered Ti ₃ C ₂ T _x MXenes coupled with Fe ₂ O ₃ nanorod arrays grown on carbon cloth as anodes for flexible asymmetric supercapacitors Li, Fei; Liu, Yi-Lin; Wang, Gui-Gen Journal of Materials Chemistry A, Vol. 7, Issue 39 https://doi.org/10.1039/c9ta08144e	journal	January 2019
Solvent-regulated preparation of well-intercalated Ti ₃ C ₂ T _x MXene nanosheets and application for highly effective electromagnetic wave absorption Xu, Gengfang; Wang, Xiaoxia; Gong, Shida Nanotechnology, Vol. 29, Issue 35 https://doi.org/10.1088/1361-6528/aac8f6	journal	June 2018
Printable Nanomaterials for the Fabrication of High-Performance Supercapacitors Sun, Jiazhen; Cui, Bo; Chu, Fuqiang Nanomaterials, Vol. 8, Issue 7 https://doi.org/10.3390/nano8070528	journal	July 2018
Modified MXene/Holey Graphene Films for Advanced Supercapacitor Electrodes with Superior Energy Storage Fan, Zhimin; Wang, Youshan; Xie, Zhimin Advanced Science, Vol. 5, Issue 10 https://doi.org/10.1002/advs.201800750	journal	August 2018
Ultrathin Titanate Nanosheets/Graphene Films Derived from Confined Transformation for Excellent Na/K Ion Storage Zeng, Cheng; Xie, Fangxi; Yang, Xianfeng Angewandte Chemie, Vol. 130, Issue 28 https://doi.org/10.1002/ange.201803511	journal	June 2018
Regulating Fast Anionic Redox for High-Voltage Aqueous Hydrogen-Ion-based Energy Storage Wang, Shengping; Zhao, Xiaoli; Yan, Xiaojun Angewandte Chemie International Edition, Vol. 58, Issue 1 https://doi.org/10.1002/anie.201811220	journal	December 2018
Two‐Dimensional Ti ₃ C ₂ T _X /Polyaniline Nanocomposite from the Decoration of Small‐Sized Graphene Nanosheets: Promoted Pseudocapacitive Electrode Performance for Supercapacitors Wang, Shuhao; Ma, Zhengwei; Lü, Qiu‐Feng ChemElectroChem, Vol. 6, Issue 10 https://doi.org/10.1002/celc.201900433	journal	April 2019
An MXene/CNTs@P nanohybrid with stable Ti–O–P bonds for enhanced lithium ion storage Zhang, Shixue; Liu, Huan; Cao, Bin Journal of Materials Chemistry A, Vol. 7, Issue 38 https://doi.org/10.1039/c9ta07357d	journal	January 2019
Assembling 2D MXenes into Highly Stable Pseudocapacitive Electrodes with High Power and Energy Densities VahidMohammadi, Armin; Mojtabavi, Mehrnaz; Caffrey, Nuala Mai Advanced Materials, Vol. 31, Issue 8 https://doi.org/10.1002/adma.201806931	journal	December 2018
A Solid-State Fibriform Supercapacitor Boosted by Host-Guest Hybridization between the Carbon Nanotube Scaffold and MXene Nanosheets Yu, Chenyang; Gong, Yujiao; Chen, Ruyi Small, Vol. 14, Issue 29 https://doi.org/10.1002/smll.201801203	journal	June 2018
2D Stacks of MXene Ti ₃ C ₂ and 1T‐Phase WS ₂ with Enhanced Capacitive Behavior Vyskočil, Jan; Mayorga‐Martinez, Carmen C.; Szőkölová, Kateřina ChemElectroChem, Vol. 6, Issue 15 https://doi.org/10.1002/celc.201900643	journal	May 2019
Interlayer Hydrogen‐Bonded Metal Porphyrin Frameworks/MXene Hybrid Film with High Capacitance for Flexible All‐Solid‐State Supercapacitors Zhao, Weiwei; Peng, Jiali; Wang, Weikang Small, Vol. 15, Issue 18 https://doi.org/10.1002/smll.201901351	journal	March 2019
Carbon nanotubes enhance flexible MXene films for high-rate supercapacitors Chen, He; Yu, Lanyong; Lin, Zifeng Journal of Materials Science, Vol. 55, Issue 3 https://doi.org/10.1007/s10853-019-04003-8	journal	September 2019
All-Solid-State Supercapacitors Based on Flexible Co3O4 Nanoflowers/rGO Nanocomposites Xiong, Zhihong; Hu, Po; Zhang, Yue Journal of Electronic Materials, Vol. 47, Issue 10 https://doi.org/10.1007/s11664-018-6479-z	journal	July 2018
Electrostatic Self-assembly of 0D–2D SnO2 Quantum Dots/Ti3C2Tx MXene Hybrids as Anode for Lithium-Ion Batteries Liu, Huan; Zhang, Xin; Zhu, Yifan Nano-Micro Letters, Vol. 11, Issue 1 https://doi.org/10.1007/s40820-019-0296-7	journal	August 2019
Sticky-note supercapacitors Cao, Jingyu; Zhao, Yang; Xu, Yifan Journal of Materials Chemistry A, Vol. 6, Issue 8 https://doi.org/10.1039/c7ta10756k	journal	January 2018
A general way to fabricate transition metal dichalcogenide/oxide-sandwiched MXene nanosheets as flexible film anodes for high-performance lithium storage Wang, Chuang; Zhu, Xiao-Dong; Wang, Ke-Xin Sustainable Energy & Fuels, Vol. 3, Issue 10 https://doi.org/10.1039/c9se00635d	journal	January 2019
A Facile Method to Construct MXene/CuO Nanocomposite with Enhanced Catalytic Activity of CuO on Thermal Decomposition of Ammonium Perchlorate Zhao, Haifeng; Lv, Jing; Sang, Junshan Materials, Vol. 11, Issue 12 https://doi.org/10.3390/ma11122457	journal	December 2018
Nitrogen Doped Intercalation TiO2/TiN/Ti3C2Tx Nanocomposite Electrodes with Enhanced Pseudocapacitance Yang, Ben; She, Yin; Zhang, Changgeng Nanomaterials, Vol. 10, Issue 2 https://doi.org/10.3390/nano10020345	journal	February 2020

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