Exceptional enhancement of Raman scattering on silver chlorobromide nanocube photonic crystals: chemical and photonic contributions

Li, Zheng; Gosztola, David J.; Sun, Cheng-Jun; Heald, Steve M.; Sun, Yugang

doi:10.1039/c5tc00077g

Title: Exceptional enhancement of Raman scattering on silver chlorobromide nanocube photonic crystals: chemical and photonic contributions

Journal Article · Mon Feb 02 00:00:00 EST 2015 · Journal of Materials Chemistry C

DOI:https://doi.org/10.1039/c5tc00077g· OSTI ID:1392364

Li, Zheng ^[1]; Gosztola, David J. ^[1]; Sun, Cheng-Jun ^[1]; Heald, Steve M. ^[1]; Sun, Yugang ^[1]

Argonne National Lab. (ANL), Argonne, IL (United States)

Photonic crystals made from self-assembly of mono-dispersed AgCl_xBr_1-x nanocubes, which are not plasmonically active, have been discovered to exceptionally enhance Raman scattering of molecules chemically adsorbed on their surfaces. Comprehensive control measurements and X-ray absorption near-edge structure spectroscopy indicate that the Raman enhancement on the AgCl_xBr_1-x nanocube photonic crystals is primarily ascribed to the chemical enhancement mechanism associated with the chemical interactions between adsorbing molecules and the AgCl_xBr_1-x surfaces. In addition, the ordering of the AgCl_xBr_1-x nanocubes in the photonic crystals can selectively reflect Raman scattering back to the detector at the bandgap position of the photonic crystals to provide additional enhancement, i.e., photonic mode enhancement. The thiophenol molecules adsorbed on the AgCl_0.44Br_0.56 nanocube photonic crystals exhibit astonishingly strong Raman signals that are on the same order of magnitude as those recorded from the thiophenol molecules adsorbed on the assembled Ag nanocubes.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1392364

Journal Information:: Journal of Materials Chemistry C, Vol. 3, Issue 11; ISSN 2050-7526

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 4 works

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