Reconciling satellite aerosol optical thickness and surface fine particle mass through aerosol liquid water

Nguyen, Thien Khoi V.; Ghate, Virendra P.; Carlton, Annmarie G.

doi:10.1002/2016GL070994

Title: Reconciling satellite aerosol optical thickness and surface fine particle mass through aerosol liquid water

Journal Article · Sat Nov 05 00:00:00 EDT 2016 · Geophysical Research Letters

DOI:https://doi.org/10.1002/2016GL070994· OSTI ID:1392096

Nguyen, Thien Khoi V. ^[1];

^[2];

^[3]

Rutgers Univ., New Brunswick, NJ (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)
Univ. of California, Irvine, CA (United States)

Summertime aerosol optical thickness (AOT) over the southeast U.S. is sharply enhanced over wintertime values. This seasonal pattern is unique and of particular interest because temperatures there have not warmed over the past 100 years. Patterns in surface fine particle mass are inconsistent with satellite reported AOT. In this work, we attempt to reconcile the spatial and temporal distribution of AOT over the U.S. with particle mass measurements at the surface by examining trends in aerosol liquid water (ALW), a particle constituent that scatters radiation and affects satellite AOT but is removed in mass measurements at routine surface monitoring sites. Herein, we employ the thermodynamic model ISORROPIAv2.1 to estimate ALW mass concentrations at Interagency Monitoring of PROtected Visual Environments sites using measured ion mass concentrations and North American Regional Reanalysis meteorological data. Excellent agreement between Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations AOT and estimated ALW provides a plausible explanation for the discrepancies in the geographical patterns of AOT and aerosol mass measurements.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USEPA; National Science Foundation (NSF); USDOE Office of Science (SC), Biological and Environmental Research (BER)

Contributing Organization:: Atmospheric System Research

Grant/Contract Number:: AC02-06CH11357; R835041; AGS-1242155; AGS-1445831

OSTI ID:: 1392096

Journal Information:: Geophysical Research Letters, Vol. 43, Issue 22; ISSN 0094-8276

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 18 works

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54 ENVIRONMENTAL SCIENCES
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hygroscopicity
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Title: Reconciling satellite aerosol optical thickness and surface fine particle mass through aerosol liquid water

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