Chemiresistive Sensor Arrays from Conductive 2D Metal–Organic Frameworks

Campbell, Michael G.; Liu, Sophie F.; Swager, Timothy M.; Dinca, Mircea

doi:10.1021/jacs.5b09600

Title: Chemiresistive Sensor Arrays from Conductive 2D Metal–Organic Frameworks

Journal Article · Sun Oct 11 00:00:00 EDT 2015 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.5b09600· OSTI ID:1386738

Campbell, Michael G. ^[1]; Liu, Sophie F. ^[1]; Swager, Timothy M. ^[1]; Dinca, Mircea ^[1]

Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Applications of porous metal–organic frameworks (MOFs) in electronic devices are rare, owing in large part to a lack of MOFs that display electrical conductivity. Here, we describe the use of conductive two-dimensional (2D) MOFs as a new class of materials for chemiresistive sensing of volatile organic compounds (VOCs). We demonstrate that a family of structurally analogous 2D MOFs can be used to construct a cross-reactive sensor array that allows for clear discrimination between different categories of VOCs. Lastly, experimental data show that multiple sensing mechanisms are operative with high degrees of orthogonality, establishing that the 2D MOFs used here are mechanistically unique and offer advantages relative to other known chemiresistor materials.

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Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Excitonics (CE)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0001088

OSTI ID:: 1386738

Journal Information:: Journal of the American Chemical Society, Vol. 137, Issue 43; Related Information: CE partners with Massachusetts Institute of Technology (lead); Brookhaven National Laboratory; Harvard University; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 523 works

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Morphology-dependent third-order optical nonlinearity of a 2D Co-based metal–organic framework with a porphyrinic skeleton Niu, Ru-Jie; Zhou, Wen-Fa; Liu, Yan Chemical Communications, Vol. 55, Issue 33 https://doi.org/10.1039/c9cc01363f	journal	January 2019
The Interaction of Guest Molecules with Co-MOF-74: A Vis/NIR and Raman Approach Strauss, Ina; Mundstock, Alexander; Hinrichs, Dominik Angewandte Chemie International Edition, Vol. 57, Issue 25 https://doi.org/10.1002/anie.201801966	journal	April 2018
High Performance Hollow Metal-Organic Framework Nanoshell-Based Etalons for Volatile Organic Compounds Detection Li, Cheng; Li, Limei; Yu, Shimo Advanced Materials Technologies, Vol. 1, Issue 7 https://doi.org/10.1002/admt.201600127	journal	August 2016
On‐Chip Tailorability of Capacitive Gas Sensors Integrated with Metal–Organic Framework Films Yuan, Hongye; Tao, Jifang; Li, Nanxi Angewandte Chemie, Vol. 131, Issue 40 https://doi.org/10.1002/ange.201906222	journal	July 2019
Chiral self-sorted multifunctional supramolecular biocoordination polymers and their applications in sensors Shang, Xiaobo; Song, Inho; Jung, Gwan Yeong Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-06147-8	journal	September 2018
Syntheses, structures and luminescence properties of five coordination polymers based on designed 2,7-bis(4-benzoic acid)-N-(4-benzoic acid) carbazole Chen, Dong-Hui; Lin, Ling; Sheng, Tian-Lu CrystEngComm, Vol. 19, Issue 19 https://doi.org/10.1039/c7ce00361g	journal	January 2017
STA-27, a porous Lewis acidic scandium MOF with an unexpected topology type prepared with 2,3,5,6-tetrakis(4-carboxyphenyl)pyrazine Prasad, Ram R. R.; Seidner, Sarah E.; Cordes, David B. Journal of Materials Chemistry A, Vol. 7, Issue 10 https://doi.org/10.1039/c8ta10610j	journal	January 2019
Gas transport regulation in a MO/MOF interface for enhanced selective gas detection Yao, Ming-Shui; Cao, Lin-An; Tang, Yong-Xiang Journal of Materials Chemistry A, Vol. 7, Issue 31 https://doi.org/10.1039/c9ta05226g	journal	January 2019
A mixed-valent Cu ^I /Cu ^II metal–organic framework with selective chemical sensing properties Jiao, Chengli; Jiang, Xia; Chu, Hailiang CrystEngComm, Vol. 18, Issue 44 https://doi.org/10.1039/c6ce01827k	journal	January 2016
Demonstration of a Broadband Photodetector Based on a Two‐Dimensional Metal–Organic Framework Arora, Himani; Dong, Renhao; Venanzi, Tommaso Advanced Materials, Vol. 32, Issue 9 https://doi.org/10.1002/adma.201907063	journal	January 2020
Discrimination of saturated alkanes and relevant volatile compounds via the utilization of a conceptual fluorescent sensor array based on organoboron-containing polymers Qi, Yanyu; Xu, Wenjun; Kang, Rui Chemical Science, Vol. 9, Issue 7 https://doi.org/10.1039/c7sc05243j	journal	January 2018
Van der Waals Heterostructured MOF‐on‐MOF Thin Films: Cascading Functionality to Realize Advanced Chemiresistive Sensing Yao, Ming‐Shui; Xiu, Jing‐Wei; Huang, Qing‐Qing Angewandte Chemie International Edition, Vol. 58, Issue 42 https://doi.org/10.1002/anie.201907772	journal	October 2019
Synthesis and characterization of a single-layer conjugated metal–organic structure featuring a non-trivial topological gap Gao, Zi'Ang; Hsu, Chia-Hsiu; Liu, Jing Nanoscale, Vol. 11, Issue 3 https://doi.org/10.1039/c8nr08477g	journal	January 2019
Reticular control of interpenetration in a complex metal–organic framework Nguyen, Trang T. M.; Le, Hung M.; Kawazoe, Yoshiyuki Materials Chemistry Frontiers, Vol. 2, Issue 11 https://doi.org/10.1039/c8qm00368h	journal	January 2018
Two-dimensional metal–organic frameworks and their derivatives for electrochemical energy storage and electrocatalysis Zhao, Kuangmin; Zhu, Weiwei; Liu, Suqin Nanoscale Advances, Vol. 2, Issue 2 https://doi.org/10.1039/c9na00719a	journal	January 2020
[Cu ₃ (C ₆ Se ₆ )] _n : The First Highly Conductive 2D π–d Conjugated Coordination Polymer Based on Benzenehexaselenolate Cui, Yutao; Yan, Jie; Chen, Zhijun Advanced Science, Vol. 6, Issue 9 https://doi.org/10.1002/advs.201802235	journal	March 2019
Layer-by-Layer Assembled Conductive Metal-Organic Framework Nanofilms for Room-Temperature Chemiresistive Sensing Yao, Ming-Shui; Lv, Xiao-Jing; Fu, Zhi-Hua Angewandte Chemie, Vol. 129, Issue 52 https://doi.org/10.1002/ange.201709558	journal	November 2017
Spontaneously Self‐Assembled Naphthalimide Nanosheets: Aggregation‐Induced Emission and Unveiling a‐PET for Sensitive Detection of Organic Volatile Contaminants in Water Meher, Niranjan; Iyer, Parameswar Krishnan Angewandte Chemie International Edition, Vol. 57, Issue 28 https://doi.org/10.1002/anie.201802842	journal	June 2018
A Calixarene-Based Metal-Organic Framework for Highly Selective NO ₂ Detection Schulz, Marcel; Gehl, Adrian; Schlenkrich, Jakob Angewandte Chemie International Edition, Vol. 57, Issue 39 https://doi.org/10.1002/anie.201805355	journal	August 2018
A Dual‐Ligand Porous Coordination Polymer Chemiresistor with Modulated Conductivity and Porosity Yao, Ming‐Shui; Zheng, Jia‐Jia; Wu, Ai‐Qian Angewandte Chemie International Edition, Vol. 59, Issue 1 https://doi.org/10.1002/anie.201909096	journal	January 2020
2D Semiconducting Metal–Organic Framework Thin Films for Organic Spin Valves Song, Xiaoyu; Wang, Xinyue; Li, Yusen Angewandte Chemie International Edition, Vol. 59, Issue 3 https://doi.org/10.1002/anie.201911543	journal	November 2019
Coordination Polymers with Grinding-Size-Dependent Mechanoresponsive Luminescence Induced by π···π Stacking Interactions: Coordination Polymers with Grinding-Size-Dependent Mechanoresponsive Luminescence Induced by π···π Stacking Interactions Yan, Yong; Zhang, Ning-Ning; Li, Rong European Journal of Inorganic Chemistry, Vol. 2017, Issue 32 https://doi.org/10.1002/ejic.201700574	journal	August 2017
Two‐dimensional π‐conjugated metal‐organic framework with high electrical conductivity for electrochemical sensing Wu, Fei; Fang, Wei; Yang, Xueyuan Journal of the Chinese Chemical Society, Vol. 66, Issue 5 https://doi.org/10.1002/jccs.201800198	journal	November 2018
Regulating the spatial distribution of metal nanoparticles within metal-organic frameworks to enhance catalytic efficiency Yang, Qiu; Liu, Wenxian; Wang, Bingqing Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms14429	journal	February 2017
Fingerprint Detection and Differentiation of Gas-phase Amines Using a Fluorescent Sensor Array Assembled from Asymmetric Perylene Diimides Hu, Yanyong; Zhou, Zichao; Zhao, Feiping Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-28556-x	journal	July 2018
Metal-oxide-semiconductor based gas sensors: screening, preparation, and integration Zhang, Jian; Qin, Ziyu; Zeng, Dawen Physical Chemistry Chemical Physics, Vol. 19, Issue 9 https://doi.org/10.1039/c6cp07799d	journal	January 2017
An amine functionalized zirconium metal–organic framework as an effective chemiresistive sensor for acidic gases DMello, Marilyn Esclance; Sundaram, Nalini G.; Singh, Akash Chemical Communications, Vol. 55, Issue 3 https://doi.org/10.1039/c8cc06875e	journal	January 2019
Two-dimensional light-emitting materials: preparation, properties and applications Wang, Zhiwei; Jingjing, Qiu; Wang, Xiaoshan Chemical Society Reviews, Vol. 47, Issue 16 https://doi.org/10.1039/c8cs00332g	journal	January 2018
Tuning the ease of formation of on-surface metal-adatom coordination polymers featuring diketones Papageorgiou, Anthoula C.; Li, Jiang; Oh, Seung Cheol Nanoscale, Vol. 10, Issue 20 https://doi.org/10.1039/c8nr02537a	journal	January 2018
Nano Pt-decorated transparent solution-processed oxide semiconductor sensor with ppm detection capability Kang, Jingu; Kim, Kyung-Tae; Jeon, Seoung-Pil RSC Advances, Vol. 9, Issue 11 https://doi.org/10.1039/c8ra09917k	journal	January 2019
A dual-functionalized, luminescent and highly crystalline covalent organic framework: molecular decoding strategies for VOCs and ultrafast TNP sensing Das, Prasenjit; Mandal, Sanjay K. Journal of Materials Chemistry A, Vol. 6, Issue 33 https://doi.org/10.1039/c8ta05070h	journal	January 2018
Photo-exfoliation of a highly photo-responsive two-dimensional metal–organic framework Xie, Jian; Wang, Yaxing; Zhang, Duo Chemical Communications, Vol. 55, Issue 78 https://doi.org/10.1039/c9cc05455c	journal	January 2019
Rational modifications of PCN-700 to induce electrical conductivity: a computational study Chong, Sanggyu; Kim, Jihan Dalton Transactions, Vol. 49, Issue 1 https://doi.org/10.1039/c9dt03865e	journal	January 2020
Functional group engineering in naphthalimides: a conceptual insight to fine-tune the supramolecular self-assembly and condensed state luminescence Meher, Niranjan; Iyer, Parameswar Krishnan Nanoscale, Vol. 11, Issue 28 https://doi.org/10.1039/c9nr04593g	journal	January 2019
Ultrathin 2D metal–organic framework nanosheets prepared via sonication exfoliation of membranes from interfacial growth and exhibition of enhanced catalytic activity by their gold nanocomposites Wu, Songting; Qin, Lu; Zhang, Ke RSC Advances, Vol. 9, Issue 17 https://doi.org/10.1039/c9ra00662a	journal	January 2019
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Strategies to Improve Electrical and Ionic Conductivities of Metal–Organic Frameworks Gordillo, Monica A.; Saha, Sourav Comments on Inorganic Chemistry, Vol. 40, Issue 2 https://doi.org/10.1080/02603594.2019.1704738	journal	December 2019
Graphene-like metal-organic frameworks: Morphology control, optimization of thin film electrical conductivity and fast sensing applications Hoppe, Bastian; Hindricks, Karen D. J.; Warwas, Dawid P. Cambridge : Royal Society of Chemistry https://doi.org/10.15488/4168	other	January 2018
Direct grafting-from of PEDOT from a photoreactive Zr-based MOF – a novel route to electrically conductive composite materials Mohmeyer, Alexander; Schaate, Andreas; Hoppe, Bastian Cambridge : Royal Society of Chemistry https://doi.org/10.15488/4712	text	January 2019
Affinity Ionic Liquids for Chemoselective Gas Sensing Chang, Albert; Li, Hsin-Yi; Chang, I-Nan Molecules, Vol. 23, Issue 9 https://doi.org/10.3390/molecules23092380	journal	September 2018
Adsorption and Detection of Hazardous Trace Gases by Metal-Organic Frameworks Woellner, Michelle; Hausdorf, Steffen; Klein, Nicole Advanced Materials, Vol. 30, Issue 37 https://doi.org/10.1002/adma.201704679	journal	June 2018
Unpaired 3d Electrons on Atomically Dispersed Cobalt Centres in Coordination Polymers Regulate both Oxygen Reduction Reaction (ORR) Activity and Selectivity for Use in Zinc–Air Batteries Lian, Yuebin; Yang, Wenjuan; Zhang, Chufeng Angewandte Chemie International Edition, Vol. 59, Issue 1 https://doi.org/10.1002/anie.201910879	journal	November 2019
Synthesis of Bimetallic Conductive 2D Metal–Organic Framework (Co _x Ni _y ‐CAT) and Its Mass Production: Enhanced Electrochemical Oxygen Reduction Activity Yoon, Hajin; Lee, Sujeong; Oh, Sojin Small, Vol. 15, Issue 17 https://doi.org/10.1002/smll.201805232	journal	April 2019
Room temperature resistive gas sensor based on ZIF-8/MWCNT/AgNPs nanocomposite for VOCs detection Jafari, Nasim; Zeinali, Sedigheh; Shadmehr, Jafar Journal of Materials Science: Materials in Electronics, Vol. 30, Issue 13 https://doi.org/10.1007/s10854-019-01592-7	journal	June 2019
Vapochromic and chemiresistive characteristics of a nanostructured molecular material composed of a zinc( ii )-salophen complex Oliveri, Ivan Pietro; Malandrino, Graziella; Mirabella, Salvo Dalton Transactions, Vol. 47, Issue 44 https://doi.org/10.1039/c8dt03904f	journal	January 2018
Porphyrin-based porous polyimide polymer/Pd nanoparticle composites as efficient catalysts for Suzuki–Miyaura coupling reactions Zhu, Wei; Wang, Xuan; Li, Tao Polymer Chemistry, Vol. 9, Issue 12 https://doi.org/10.1039/c8py00092a	journal	January 2018
Coordination polymer-based conductive materials: ionic conductivity vs. electronic conductivity Wang, Hai-Ning; Meng, Xing; Dong, Long-Zhang Journal of Materials Chemistry A, Vol. 7, Issue 42 https://doi.org/10.1039/c9ta08253k	journal	January 2019
Competitive formation between 2D and 3D metal-organic frameworks: insights into the selective formation and lamination of a 2D MOF Oh, Sojin; Park, Jeehyun; Oh, Moonhyun International Union of Crystallography (IUCr) https://doi.org/10.1107/s2052252519007760/yc5019sup1.pdf	text	January 2019
Two-dimensional magnetic metal-organic frameworks with the Shastry-Sutherland lattice Zhang, Li-Chuan; Zhang, Lizhi; Qin, Guangzhao RWTH Aachen University https://doi.org/10.18154/rwth-2019-11577	text	January 2019
Efficient fluorescence detection of aromatic toxicants and toxicant metabolites in human breast milk DiScenza, Dana J.; Lynch, Julie; Verderame, Molly Taylor & Francis https://doi.org/10.6084/m9.figshare.5165869	text	January 2017
Computer-aided discovery of a metal-organic framework with superior oxygen uptake. Moghadam, Peyman Z.; Islamoglu, Timur; Goswami, Subhadip Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.30869	text	January 2018
Efficient fluorescence detection of aromatic toxicants and toxicant metabolites in human breast milk DiScenza, Dana J.; Lynch, Julie; Verderame, Molly Taylor & Francis https://doi.org/10.6084/m9.figshare.5165869.v1	text	January 2017
Superconductivity in a Copper(II)-Based Coordination Polymer with Perfect Kagome Structure Huang, Xing; Zhang, Shuai; Liu, Liyao Angewandte Chemie International Edition, Vol. 57, Issue 1 https://doi.org/10.1002/anie.201707568	journal	December 2017
Grand Challenges and Future Opportunities for Metal–Organic Frameworks Hendon, Christopher H.; Rieth, Adam J.; Korzyński, Maciej D. ACS Central Science, Vol. 3, Issue 6 https://doi.org/10.1021/acscentsci.7b00197	journal	June 2017
Single Crystals of Electrically Conductive Two-Dimensional Metal–Organic Frameworks: Structural and Electrical Transport Properties Day, Robert W.; Bediako, D. Kwabena; Rezaee, Mehdi ACS Central Science, Vol. 5, Issue 12 https://doi.org/10.1021/acscentsci.9b01006	journal	December 2019
Metal–Organic Frameworks as Active Materials in Electronic Sensor Devices Campbell, Michael; Dincă, Mircea Sensors, Vol. 17, Issue 5 https://doi.org/10.3390/s17051108	journal	May 2017

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