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Title: Potential {sup 14}CO{sub 2} releases from spent fuel containers at Yucca Mountain

Conference ·
DOI:https://doi.org/10.2172/10132933· OSTI ID:138015

The potential release of gaseous {sup 14}CO{sub 2} from small perforations in spent fuel containers has been evaluated as a function of temperature, hole size, effective porosity of corrosion products within the hole, and time, based on the waste package design parameters and environmental conditions described in the Yucca Mountain Site Characterization Report (SCP). The SCP does not specify initial fill gas (argon) pressure and temperature. It is shown that, if significant {sup 14}C oxidation takes place during the initial, inert-gas phase, an incentive exists to initially underpressurize the containers. This will avoid large, spiked releases of gaseous {sup 14}CO{sub 2} and will result in delayed, smaller, and more uniform release rates over time. Therefore larger size perforations could be tolerated while meeting the applicable regulations. 16 refs., 2 figs., 3 tabs.

Research Organization:
Brookhaven National Lab. (BNL), Upton, NY (United States)
DOE Contract Number:
AC02-76CH00016
OSTI ID:
138015
Report Number(s):
BNL-45658; CONF-910435-49; ON: DE91008091; TRN: 91:005937
Resource Relation:
Conference: 2. annual American Nuclear Society (ANS) international high level radioactive waste management conference, Las Vegas, NV (United States), 28 Apr - 3 May 1991; Other Information: PBD: [1991]
Country of Publication:
United States
Language:
English