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Title: High-Performance Non-Fullerene Organic Solar Cells Based on a Selenium-Containing Polymer Donor and a Twisted Perylene Bisimide Acceptor

Journal Article · · Advanced Science
 [1];  [2];  [3];  [1];  [2];  [1];  [4];  [2];  [5];  [1]
  1. Beihang Univ., Beijing (China). Heeger Beijing Research and Development Center
  2. Chinese Academy of Sciences (CAS), Beijing (China). Inst. of Chemistry
  3. Heeger Beijing Research and Development Center, School of Chemistry and Environment, Beihang University, Beijing 100191 P. R. China
  4. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Science Division
  5. Univ. of Massachusetts, Amherst, MA (United States). Polymer Science and Engineering Dept.

A novel polymer donor (PBDTS-Se) is designed to match with a non-fullerene acceptor (SdiPBI-S). The corresponding solar cells show a high efficiency of 8.22%, which result from synergetic improvements of light harvesting, charge carrier transport and collection, and morphology. The results indicate that rational design of novel donor materials is important for non-fullerene organic solar cells.

Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1379298
Journal Information:
Advanced Science, Vol. 3, Issue 9; ISSN 2198-3844
Publisher:
WileyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 84 works
Citation information provided by
Web of Science

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Cited By (23)

Achieving a High Fill Factor and Stability in Perylene Diimide–Based Polymer Solar Cells Using the Molecular Lock Effect between 4,4′‐Bipyridine and a Tri(8‐hydroxyquinoline)aluminum(III) Core journal May 2019
Design of Diketopyrrolopyrrole (DPP)-Based Small Molecules for Organic-Solar-Cell Applications journal November 2016
Ternary Organic Solar Cells Based on Two Compatible Nonfullerene Acceptors with Power Conversion Efficiency >10% journal September 2016
Nonfullerene Tandem Organic Solar Cells with High Open-Circuit Voltage of 1.97 V journal September 2016
Alkyl Side-Chain Engineering in Wide-Bandgap Copolymers Leading to Power Conversion Efficiencies over 10% journal December 2016
Recent Advances in Wide-Bandgap Photovoltaic Polymers journal March 2017
Isomerization of Perylene Diimide Based Acceptors Enabling High‐Performance Nonfullerene Organic Solar Cells with Excellent Fill Factor journal January 2019
Donor Derivative Incorporation: An Effective Strategy toward High Performance All‐Small‐Molecule Ternary Organic Solar Cells journal August 2019
Effect of Benzene Rings’ Incorporation on Photovoltaic Performance of Indacenodithiophene-cored Molecular Acceptors journal February 2018
A Novel Thiophene-Fused Ending Group Enabling an Excellent Small Molecule Acceptor for High-Performance Fullerene-Free Polymer Solar Cells with 11.8% Efficiency journal May 2017
Chlorination Strategy‐Induced Abnormal Nanomorphology Tuning in High‐Efficiency Organic Solar Cells: A Study of Phenyl‐Substituted Benzodithiophene‐Based Nonfullerene Acceptors journal July 2019
Chalcogen‐Fused Perylene Diimides‐Based Nonfullerene Acceptors for High‐Performance Organic Solar Cells: Insight into the Effect of O, S, and Se journal December 2019
Deciphering the Role of Fluorination: Morphological Manipulation Prompts Charge Separation and Reduces Carrier Recombination in All‐Small‐Molecule Photovoltaics journal April 2020
Benzodithiophenedione-based polymers: recent advances in organic photovoltaics journal January 2020
9-Fluorenone and 9,10-anthraquinone potential fused aromatic building blocks to synthesize electron acceptors for organic solar cells journal January 2017
Influence of alkyl chains on photovoltaic properties of 3D rylene propeller electron acceptors journal January 2017
A three-dimensional thiophene-annulated perylene bisimide as a fullerene-free acceptor for a high performance polymer solar cell with the highest PCE of 8.28% and a V OC over 1.0 V journal January 2018
Pyran-annulated perylene diimide derivatives as non-fullerene acceptors for high performance organic solar cells journal January 2018
Non-fullerene acceptor engineering with three-dimensional thiophene/selenophene-annulated perylene diimides for high performance polymer solar cells journal January 2018
A fully fused non-fullerene acceptor containing angular-shaped S , N -heteroacene and perylene diimide for additive-free organic solar cells journal January 2019
Functionalizing tetraphenylpyrazine with perylene diimides (PDIs) as high-performance nonfullerene acceptors journal January 2019
Comparing non-fullerene acceptors with fullerene in polymer solar cells: a case study with FTAZ and PyCNTAZ text January 2017
A Novel Thiophene-fused Ending Group Enabling an Excellent Small Molecule Acceptor for High-performance Fullerene-free Polymer Solar Cells with 11.8% Efficiency preprint January 2017

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