skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Energy dependence of the prompt γ -ray emission from the ( d , p ) -induced fission of U * 234 and Pu * 240

Journal Article · · Physical Review C
 [1];  [1];  [2];  [3];  [4];  [1];  [1];  [5];  [6];  [7];  [1];  [8];  [1];  [1];  [1];  [1];  [1];  [1];  [9];  [1] more »;  [1];  [1];  [10];  [1];  [11] « less
  1. Univ. of Oslo, Oslo (Norway)
  2. CNRS/Univ. Paris-Sud, Univ. Paris Saclay, Orsay Cedex (France)
  3. Extreme Light Infrastructure - Nuclear Physics (ELI-NP), Bucharest-Magurele (Romania)
  4. European Commission, Geel (Belgium)
  5. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California, Berkeley, CA (United States)
  6. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  7. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  8. Univ. of Oslo, Oslo (Norway); Helmholtz Institute Mainz, Mainz (Germany); GSI Helmholtzzentrum fur Schwerionenforschung, Darmstadt (Germany)
  9. Univ. of California, Berkeley, CA (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
  10. Grand Accelerateur National d'lons Lourd (France)
  11. iThemba LABS, Somerset West (South Africa)

Prompt-fission γ rays are responsible for approximately 5% of the total energy released in fission, and therefore important to understand when modeling nuclear reactors. In this work we present prompt γ-ray emission characteristics in fission as a function of the nuclear excitation energy of the fissioning system. Emitted γ-ray spectra were measured, and γ-ray multiplicities and average and total γ energies per fission were determined for the U(d,pf)233 reaction for excitation energies between 4.8 and 10 MeV, and for the Pu(d,pf)239 reaction between 4.5 and 9 MeV. The spectral characteristics show no significant change as a function of excitation energy above the fission barrier, despite the fact that an extra -5 MeV of energy is potentially available in the excited fragments for γ decay. The measured results are compared with model calculations made for prompt γ-ray emission with the fission model code gef. Further comparison with previously obtained results from thermal neutron induced fission is made to characterize possible differences arising from using the surrogate (d,p) reaction.

Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
Grant/Contract Number:
AC52-07NA27344; AC02-05CH11231
OSTI ID:
1378551
Alternate ID(s):
OSTI ID: 1368426; OSTI ID: 1429356
Report Number(s):
LLNL-JRNL-737322; PRVCAN
Journal Information:
Physical Review C, Vol. 96, Issue 1; ISSN 2469-9985
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 6 works
Citation information provided by
Web of Science

References (45)

Late-time emission of prompt fission γ rays journal December 2016
Systematics of prompt γ -ray emission in fission journal March 2013
Prompt γ -ray production in neutron-induced fission of 239 Pu journal April 2013
Decay Curves and Half-lives of Gamma-Emitting States from a Study of Prompt Fission Gamma Radiation journal March 1971
Properties of prompt-fission γ rays journal August 2014
The Mechanism of Nuclear Fission journal September 1939
RIPL – Reference Input Parameter Library for Calculation of Nuclear Reactions and Nuclear Data Evaluations journal December 2009
�ber den Nachweis und das Verhalten der bei der Bestrahlung des Urans mittels Neutronen entstehenden Erdalkalimetalle journal January 1939
The prompt response of bismuth germanate and NaI(Tl) scintillation detectors to fast neutrons journal August 1983
Spectrum of Photons Emitted in Coincidence with Fission of U 235 by Thermal Neutrons journal January 1971
Improved values for the characteristics of prompt-fission γ -ray spectra from the reaction 235 U( n th , f ) journal May 2013
Electrodeposition of U and Pu on thin C and Ti substrates
  • Henderson, R. A.; Gostic, J. M.; Burke, J. T.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 655, Issue 1 https://doi.org/10.1016/j.nima.2011.06.023
journal November 2011
Intermediate structure in the 239Pu(d, pf) reaction journal January 1976
Study of the surrogate-reaction method applied to neutron-induced capture cross sections journal June 2012
Prompt γ-rays emitted in the thermal-neutron induced fission of 233U and 239Pu journal October 1973
Investigation of the U 238 ( d , p ) surrogate reaction via the simultaneous measurement of γ -decay and fission probabilities journal August 2016
ENDF/B-VII.1 Nuclear Data for Science and Technology: Cross Sections, Covariances, Fission Product Yields and Decay Data journal December 2011
Nuclear Data Sheets for A = 234 journal March 2007
Statistical γ -decay properties of Ni 64 and deduced ( n , γ ) cross section of the s -process branch-point nucleus Ni 63 journal October 2016
Disintegration of Uranium by Neutrons: a New Type of Nuclear Reaction journal February 1939
Evidence for the stochastic aspect of prompt γ emission in spontaneous fission journal February 2012
The SiRi particle-telescope system
  • Guttormsen, M.; Bürger, A.; Hansen, T. E.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 648, Issue 1 https://doi.org/10.1016/j.nima.2011.05.055
journal August 2011
Excited superdeformed Kπ=0+ rotational bands in β-vibrational fission resonances of 240Pu journal April 2001
Compound-nuclear reaction cross sections from surrogate measurements journal March 2012
Prompt-fission γ -ray spectral characteristics from Pu 239 ( n th , f ) journal June 2017
Scissors resonance in the quasicontinuum of Th, Pa, and U isotopes journal January 2014
Angular momentum transfer in 12C-, 20Ne- and 40Ar-induced fission journal October 1984
Prompt Gamma Rays from U 235 ( n , f ) , Pu 239 ( n , f ) , and Spontaneous Fission of Cf 252 journal March 1973
A new fission-fragment detector to complement the CACTUS-SiRi setup at the Oslo Cyclotron Laboratory
  • Tornyi, T. G.; Görgen, A.; Guttormsen, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 738 https://doi.org/10.1016/j.nima.2013.12.005
journal February 2014
The statistical model and nuclear level densities journal October 1960
Statistical Gamma-Decay at Low Angular Momentum journal January 1990
Prompt Gamma Rays Emitted in the Thermal-Neutron-Induced Fission of U 235 journal September 1972
Comparative measurement of prompt fission γ -ray emission from fast-neutron-induced fission of U 235 and U 238 journal September 2015
Constant-temperature level densities in the quasicontinuum of Th and U isotopes journal August 2013
General Description of Fission Observables: GEF Model Code journal January 2016
The Inelastic Scattering of Neutrons journal July 1952
Systematics of nuclear level density parameters journal September 2005
The unfolding of continuum γ-ray spectra
  • Guttormsen, M.; Tveter, T. S.; Bergholt, L.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 374, Issue 3 https://doi.org/10.1016/0168-9002(96)00197-0
journal June 1996
Total prompt energy release in the neutron-induced fission of 235U, 238U, and 239Pu journal June 2006
New prompt spectral γ -ray data from the reaction 252 Cf(sf) and its implication on present evaluated nuclear data files journal February 2013
Neutron Fission Cross Sections for 231 Th, 233 Th, 235 U, 237 U, 239 U, 241 Pu, and 243 Pu from 0.5 to 2.25 MeV Using ( t, pf ) Reactions journal August 1970
Systematics of Nuclear Level Density Parameters conference November 2011
Constant-temperature level densities in the quasi-continuum of Th and U isotopes text January 2013
Scissors resonance in the quasi-continuum of Th, Pa and U isotopes text January 2013
A new fission-fragment detector to complement the CACTUS-SiRi setup at the Oslo Cyclotron Laboratory preprint January 2013

Cited By (1)

Review on the progress in nuclear fission—experimental methods and theoretical descriptions journal September 2018

Similar Records

Prompt fission product yields in the U238(n,f) reaction
Journal Article · Tue Feb 05 00:00:00 EST 2019 · Physical Review C · OSTI ID:1378551

Determining the average prompt-fission-neutron multiplicity for Pu239(n,f) via a Pu240(α,α'f) surrogate reaction
Journal Article · Mon Dec 23 00:00:00 EST 2019 · Physical Review C · OSTI ID:1378551

Experiments on the synthesis of superheavy nuclei Fl284 and Fl285 in the Pu239,240+Ca48 reactions
Journal Article · Tue Sep 15 00:00:00 EDT 2015 · Physical Review C, Nuclear Physics · OSTI ID:1378551