High-pressure floating-zone growth of perovskite nickelate LaNiO3 single crystals
Abstract
We report the first single crystal growth of the correlated metal LaNiO3 using a high-pressure optical-image floating zone furnace. The crystals were studied using single crystal/powder X-ray diffraction, resistivity, specific heat, and magnetic susceptibility. The availability of bulk LaNiO3 crystals will (i) promote deep understanding in this correlated material, including the mechanism of enhanced paramagnetic susceptibility, and (ii) provide rich opportunities as a substrate for thin film growth such as important ferroelectric and/or multiferroic materials. As a result, this study demonstrates the power of high pO2 single crystal growth of nickelate perovskites and correlated electron oxides more generally.
- Authors:
-
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1371941
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Crystal Growth and Design
- Additional Journal Information:
- Journal Volume: 17; Journal Issue: 5; Journal ID: ISSN 1528-7483
- Publisher:
- American Chemical Society
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
Citation Formats
Zhang, Junjie, Zheng, Hong, Ren, Yang, and Mitchell, J. F. High-pressure floating-zone growth of perovskite nickelate LaNiO3 single crystals. United States: N. p., 2017.
Web. doi:10.1021/acs.cgd.7b00205.
Zhang, Junjie, Zheng, Hong, Ren, Yang, & Mitchell, J. F. High-pressure floating-zone growth of perovskite nickelate LaNiO3 single crystals. United States. https://doi.org/10.1021/acs.cgd.7b00205
Zhang, Junjie, Zheng, Hong, Ren, Yang, and Mitchell, J. F. 2017.
"High-pressure floating-zone growth of perovskite nickelate LaNiO3 single crystals". United States. https://doi.org/10.1021/acs.cgd.7b00205. https://www.osti.gov/servlets/purl/1371941.
@article{osti_1371941,
title = {High-pressure floating-zone growth of perovskite nickelate LaNiO3 single crystals},
author = {Zhang, Junjie and Zheng, Hong and Ren, Yang and Mitchell, J. F.},
abstractNote = {We report the first single crystal growth of the correlated metal LaNiO3 using a high-pressure optical-image floating zone furnace. The crystals were studied using single crystal/powder X-ray diffraction, resistivity, specific heat, and magnetic susceptibility. The availability of bulk LaNiO3 crystals will (i) promote deep understanding in this correlated material, including the mechanism of enhanced paramagnetic susceptibility, and (ii) provide rich opportunities as a substrate for thin film growth such as important ferroelectric and/or multiferroic materials. As a result, this study demonstrates the power of high pO2 single crystal growth of nickelate perovskites and correlated electron oxides more generally.},
doi = {10.1021/acs.cgd.7b00205},
url = {https://www.osti.gov/biblio/1371941},
journal = {Crystal Growth and Design},
issn = {1528-7483},
number = 5,
volume = 17,
place = {United States},
year = {Fri Apr 07 00:00:00 EDT 2017},
month = {Fri Apr 07 00:00:00 EDT 2017}
}
Web of Science
Figures / Tables:
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