Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies

Bekenstein, Yehonadav; Koscher, Brent A.; Eaton, Samuel W.; Yang, Peidong; Alivisatos, A. Paul

doi:10.1021/jacs.5b11199

Title: Highly luminescent colloidal nanoplates of perovskite cesium lead halide and their oriented assemblies

Journal Article · Tue Dec 15 00:00:00 EST 2015 · Journal of the American Chemical Society

DOI:https://doi.org/10.1021/jacs.5b11199· OSTI ID:1351533

Bekenstein, Yehonadav ^[1]; Koscher, Brent A. ^[1]; Eaton, Samuel W. ^[2]; Yang, Peidong ^[3]; Alivisatos, A. Paul ^[3]

Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Univ. of California, Berkeley, CA (United States)
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Kavli Energy NanoScience Institute, Berkeley, CA (United States)

Anisotropic colloidal quasi-two-dimensional nanoplates (NPLs) hold great promise as functional materials due to their combination of low dimensional optoelectronic properties and versatility through colloidal synthesis. Recently, lead-halide perovskites have emerged as important optoelectronic materials with excellent efficiencies in photovoltaic and light-emitting applications. Here we report the synthesis of quantum confined all inorganic cesium lead halide nanoplates in the perovskite crystal structure that are also highly luminescent (PLQY 84%). The controllable self-assembly of nanoplates either into stacked columnar phases or crystallographic-oriented thin-sheet structures is demonstrated. Furthermore, the broad accessible emission range, high native quantum yields, and ease of self-assembly make perovskite NPLs an ideal platform for fundamental optoelectronic studies and the investigation of future devices.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI ID:: 1351533

Report Number(s):: LBNL-1004421; ir:1004421

Journal Information:: Journal of the American Chemical Society, Vol. 137, Issue 51; ISSN 0002-7863

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 904 works

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Study of the Partial Substitution of Pb by Sn in Cs–Pb–Sn–Br Nanocrystals Owing to Obtaining Stable Nanoparticles with Excellent Optical Properties Vitoreti, Ana Beatriz Ferreira; Agouram, Said; Solis de la Fuente, Mauricio The Journal of Physical Chemistry C, Vol. 122, Issue 25 https://doi.org/10.1021/acs.jpcc.8b02499	journal	December 2017
Ultrathin One- and Two-Dimensional Colloidal Semiconductor Nanocrystals: Pushing Quantum Confinement to the Limit Berends, Anne C.; de Mello Donega, Celso The Journal of Physical Chemistry Letters, Vol. 8, Issue 17 https://doi.org/10.1021/acs.jpclett.7b01640	journal	August 2017
Role of Nonradiative Defects and Environmental Oxygen on Exciton Recombination Processes in CsPbBr ₃ Perovskite Nanocrystals Lorenzon, Monica; Sortino, Luca; Akkerman, Quinten Nano Letters, Vol. 17, Issue 6 https://doi.org/10.1021/acs.nanolett.7b01253	journal	May 2017
Shape-Pure, Nearly Monodispersed CsPbBr ₃ Nanocubes Prepared Using Secondary Aliphatic Amines Imran, Muhammad; Ijaz, Palvasha; Baranov, Dmitry Nano Letters, Vol. 18, Issue 12 https://doi.org/10.1021/acs.nanolett.8b03598	journal	November 2018
All-Inorganic Metal Halide Perovskite Nanocrystals: Opportunities and Challenges Zhang, Qiao; Yin, Yadong ACS Central Science, Vol. 4, Issue 6 https://doi.org/10.1021/acscentsci.8b00201	journal	May 2018
Doped Halide Perovskite Nanocrystals for Reabsorption-Free Luminescent Solar Concentrators Meinardi, Francesco; Akkerman, Quinten A.; Bruni, Francesco ACS Energy Letters, Vol. 2, Issue 10 https://doi.org/10.1021/acsenergylett.7b00701	journal	September 2017
Controlling the Phase Segregation in Mixed Halide Perovskites through Nanocrystal Size Gualdrón-Reyes, Andrés. F.; Yoon, Seog Joon; Barea, Eva M. ACS Energy Letters, Vol. 4, Issue 1 https://doi.org/10.1021/acsenergylett.8b02207	journal	November 2018
Role of Acid–Base Equilibria in the Size, Shape, and Phase Control of Cesium Lead Bromide Nanocrystals Almeida, Guilherme; Goldoni, Luca; Akkerman, Quinten ACS Nano, Vol. 12, Issue 2 https://doi.org/10.1021/acsnano.7b08357	journal	January 2018
Exploration of Near-Infrared-Emissive Colloidal Multinary Lead Halide Perovskite Nanocrystals Using an Automated Microfluidic Platform Lignos, Ioannis; Morad, Viktoriia; Shynkarenko, Yevhen ACS Nano, Vol. 12, Issue 6 https://doi.org/10.1021/acsnano.8b01122	journal	May 2018
Crystal Structure, Morphology, and Surface Termination of Cyan-Emissive, Six-Monolayers-Thick CsPbBr ₃ Nanoplatelets from X-ray Total Scattering Bertolotti, Federica; Nedelcu, Georgian; Vivani, Anna ACS Nano, Vol. 13, Issue 12 https://doi.org/10.1021/acsnano.9b07626	journal	November 2019
Concurrent Ultrafast Electron- and Hole-Transfer Dynamics in CsPbBr ₃ Perovskite and Quantum Dots Dana, Jayanta; Maity, Partha; Jana, Biswajit ACS Omega, Vol. 3, Issue 3 https://doi.org/10.1021/acsomega.8b00276	journal	March 2018
Solution Synthesis Approach to Colloidal Cesium Lead Halide Perovskite Nanoplatelets with Monolayer-Level Thickness Control Akkerman, Quinten A.; Motti, Silvia Genaro; Srimath Kandada, Ajay Ram Journal of the American Chemical Society, Vol. 138, Issue 3 https://doi.org/10.1021/jacs.5b12124	journal	January 2016
An intrinsic growth instability in isotropic materials leads to quasi-two-dimensional nanoplatelets Riedinger, Andreas; Ott, Florian D.; Mule, Aniket Nature Materials, Vol. 16, Issue 7 https://doi.org/10.1038/nmat4889	journal	April 2017
Chemistry and properties at a sub-nanometer scale Ni, Bing; Wang, Xun Chemical Science, Vol. 7, Issue 7 https://doi.org/10.1039/c6sc00432f	journal	January 2016
Efficient perovskite light-emitting diodes based on a solution-processed tin dioxide electron transport layer Wang, Heyong; Yu, Hongling; Xu, Weidong Journal of Materials Chemistry C, Vol. 6, Issue 26 https://doi.org/10.1039/c8tc01871e	journal	January 2018
Coherent Nanotwins and Dynamic Disorder in Cesium Lead Halide Perovskite Nanocrystals Federica, Bertolotti,; Loredana, Protesescu,; V., Kovalenko, Maksym ETH Zurich https://doi.org/10.3929/ethz-b-000191764	text	January 2017
Microcarrier-Assisted Inorganic Shelling of Lead Halide Perovskite Nanocrystals N., Dirin, Dmitry; M., Benin, Bogdan; Sergii, Yakunin, ETH Zurich https://doi.org/10.3929/ethz-b-000376105	text	January 2019
Scalable photonic sources using two-dimensional lead halide perovskite superlattices Jagielski, Jakub; Solari, Simon F.; Jordan, Lucie ETH Zurich https://doi.org/10.3929/ethz-b-000396545	text	January 2020
Polymer Nanoreactors Shield Perovskite Nanocrystals from Degradation Hintermayr, Verena A.; Lampe, Carola; Löw, Maximilian arXiv https://doi.org/10.48550/arxiv.1909.08889	text	January 2019
Metal Halide Perovskite Nanocrystals: Synthesis, Post-Synthesis Modifications and Their Optical Properties Shamsi, Javad; Urban, Alexander S.; Imran, Muhammad arXiv https://doi.org/10.48550/arxiv.2010.14939	text	January 2020

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