skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Geometric prepatterning-based tuning of the period doubling onset strain during thin-film wrinkling

Journal Article · · Journal of Applied Mechanics
DOI:https://doi.org/10.1115/1.4036325· OSTI ID:1351142
 [1]
  1. Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Wrinkling of thin films is an easy-to-implement and low-cost technique to fabricate stretch-tunable periodic micro and nanoscale structures. However, the tunability of such structures is often limited by the emergence of an undesirable period-doubled mode at high strains. Predictively tuning the onset strain for period doubling via existing techniques requires one to have extensive knowledge about the nonlinear pattern formation behavior. Herein, a geometric prepatterning-based technique is introduced that can be implemented even with limited system knowledge to predictively delay period doubling. The technique comprises prepatterning the film/base bilayer with a sinusoidal pattern that has the same period as the natural period of the system. This technique has been verified via physical and computational experiments on the polydimethylsiloxane (PDMS)/glass bilayer system. It is observed that the onset strain can be increased from the typical value of 20% for flat films to greater than 30% with a modest prepattern aspect ratio (2·amplitude/period) of 0.15. In addition, finite element simulations reveal that (i) the onset strain increases with increasing prepattern amplitude and (ii) the delaying effect can be captured entirely by the prepattern geometry. Therefore, one can implement this technique even with limited system knowledge, such as material properties or film thickness, by simply replicating pre-existing wrinkled patterns to generate prepatterned bilayers. Furthermore, geometric prepatterning is a practical scheme to increase the operating range of stretch-tunable wrinkle-based devices by at least 50%.

Research Organization:
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC52-07NA27344
OSTI ID:
1351142
Report Number(s):
LLNL-JRNL-683274
Journal Information:
Journal of Applied Mechanics, Vol. 84, Issue 5; ISSN 0021-8936
Publisher:
ASMECopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 3 works
Citation information provided by
Web of Science

References (29)

Phase Diagrams of Instabilities in Compressed Film-Substrate Systems journal December 2013
The controlled formation of ordered, sinusoidal structures by plasma oxidation of an elastomeric polymer journal October 1999
Finite deformation mechanics in buckled thin films on compliant supports journal September 2007
Soft matter with hard skin: From skin wrinkles to templating and material characterization journal January 2006
Well-Ordered Wrinkling Patterns on Chemically Oxidized Poly(dimethylsiloxane) Surfaces journal August 2012
Wrinkling of plates coupled with soft elastic media journal September 2001
Tilted Janus polymer pillars journal January 2010
Spontaneous formation of ordered structures in thin films of metals supported on an elastomeric polymer journal May 1998
Non-Lithographic Wrinkle Nanochannels for Protein Preconcentration journal August 2008
Stability Improved Stretchable Metallic Gratings With Tunable Grating Period in Submicron Scale journal August 2015
Sensitivity of the mode locking phenomenon to geometric imperfections during wrinkling of supported thin films journal March 2017
Wrinkles and deep folds as photonic structures in photovoltaics journal April 2012
Complex micropatterning of periodic structures on elastomeric surfaces journal January 2008
Stress focusing in elastic sheets journal April 2007
Principles and applications of micro and nanoscale wrinkles journal November 2010
Microwrinkles: Shape-tunability and applications journal February 2012
Period-doubling and period-tripling in growing bilayered systems journal February 2015
Tunable optical gratings based on buckled nanoscale thin films on transparent elastomeric substrates journal January 2010
The role of substrate pre-stretch in post-wrinkling bifurcations journal January 2014
Spontaneous formation of one-dimensional ripples in transit to highly ordered two-dimensional herringbone structures through sequential and unequal biaxial mechanical stretching journal June 2007
Design of a Compact Biaxial Tensile Stage for Fabrication and Tuning of Complex Micro- and Nano-scale Wrinkle Patterns journal September 2015
The role of nonlinear substrate elasticity in the wrinkling of thin films journal June 2013
Sinusoidal phase grating created by a tunably buckled surface journal November 2004
High Aspect Ratio Wrinkles via Substrate Prestretch journal May 2014
Towards a quantitative understanding of period-doubling wrinkling patterns occurring in film/substrate bilayer systems journal January 2015
Wrinkling Phenomena in Neo-Hookean Film/Substrate Bilayers journal April 2012
The role of mechanical stress on the formation of a curly pattern of human hair journal February 2011
Tuneable elastomeric nanochannels for nanofluidic manipulation journal May 2007
Deterministic Switching of Hierarchy during Wrinkling in Quasi‐Planar Bilayers  journal April 2016

Cited By (2)

Surface wrinkling of an elastic graded layer journal January 2018
Wrinkling of flexoelectric nano-film/substrate systems journal January 2018