skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Dual-Gate Modulation of Carrier Density and Disorder in an Oxide Two-Dimensional Electron System

Journal Article · · Nano Letters
 [1];  [2];  [2];  [1];  [1];  [3];  [3];  [2]
  1. Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials
  2. Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Inst. for Materials and Energy Sciences
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Inst. for Materials and Energy Sciences

Carrier density and disorder are two crucial parameters that control the properties of correlated two-dimensional electron systems. Furthermore, in order to disentangle their individual contributions to quantum phenomena, independent tuning of these two parameters is required. By utilizing a hybrid liquid/solid electric dual-gate geometry acting on the conducting LaAlO3/SrTiO3 heterointerface, we obtain an additional degree of freedom to strongly modify the electron confinement profile and thus the strength of interfacial scattering, independent from the carrier density. A dual-gate controlled nonlinear Hall effect is a direct manifestation of this profile, which can be quantitatively understood by a Poisson–Schrödinger sub-band model. In particular, the large nonlinear dielectric response of SrTiO3 enables a very wide range of tunable density and disorder, far beyond that for conventional semiconductors. This study provides a broad framework for understanding various reported phenomena at the LaAlO3/SrTiO3 interface.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-76SF00515; N00014-12-1-0976
OSTI ID:
1348871
Journal Information:
Nano Letters, Vol. 16, Issue 10; ISSN 1530-6984
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 37 works
Citation information provided by
Web of Science

References (50)

Superconductor–insulator transition in La2 − xSr x CuO4 at the pair quantum resistance journal April 2011
Electrostatic Control of the Evolution from a Superconducting Phase to an Insulating Phase in Ultrathin YBa 2 Cu 3 O 7 x Films journal July 2011
Onset of superconductivity in the two-dimensional limit journal May 1989
Superconductor-Insulator Transitions journal August 2010
Electrostatic modification of novel materials journal November 2006
Dominant Mobility Modulation by the Electric Field Effect at the LaAlO 3 / SrTiO 3 Interface journal November 2009
Electric field control of the LaAlO3/SrTiO3 interface ground state journal December 2008
Emergent phenomena at oxide interfaces journal January 2012
Mobility Modulation of the Two-Dimensional Electron Gas Via Controlled Deformation of the Electron Wave Function in Selectively Doped AlGaAs-GaAs Heterojunctions journal March 1985
A high-mobility electron gas at the LaAlO3/SrTiO3 heterointerface journal January 2004
First-Principles Modeling of Electrostatically Doped Perovskite Systems journal March 2011
Superconducting Interfaces Between Insulating Oxides journal August 2007
Magnetic effects at the interface between non-magnetic oxides journal June 2007
Coexistence of magnetic order and two-dimensional superconductivity at LaAlO3/SrTiO3 interfaces journal September 2011
Direct imaging of the coexistence of ferromagnetism and superconductivity at the LaAlO3/SrTiO3 interface journal September 2011
Two-Dimensional Quantum Oscillations of the Conductance at LaAlO3/SrTiO3Interfaces journal December 2010
Quantum longitudinal and Hall transport at the LaAlO3/SrTiO3 interface at low electron densities journal November 2014
Dielectric Properties of Strontium Titanate at Low Temperature journal August 1970
SrTi O 3 : An intrinsic quantum paraelectric below 4 K journal April 1979
Energy Bands for KNi F 3 , SrTi O 3 , KMo O 3 , and KTa O 3 journal December 1972
Towards Two-Dimensional Metallic Behavior at LaAlO 3 / SrTiO 3 Interfaces journal May 2009
A universal critical density underlying the physics of electrons at the LaAlO3/SrTiO3 interface journal January 2012
Two-Dimensional Superconducting Phase in LaTiO 3 / SrTiO 3 Heterostructures Induced by High-Mobility Carrier Doping journal June 2012
Field-effect devices utilizing LaAlO 3 -SrTiO 3 interfaces journal January 2012
Tunable Quasi-Two-Dimensional Electron Gases in Oxide Heterostructures journal September 2006
Transistor operation and mobility enhancement in top-gated LaAlO 3 /SrTiO 3 heterostructures journal September 2013
Electric-field-induced superconductivity in an insulator journal October 2008
Liquid-gated interface superconductivity on an atomically flat film journal November 2009
Superconducting Dome in a Gate-Tuned Band Insulator journal November 2012
Tunable Spin–Orbit Interaction in Trilayer Graphene Exemplified in Electric-Double-Layer Transistors journal April 2012
Zeeman-type spin splitting controlled by an electric field journal July 2013
Generation and electric control of spin–valley-coupled circular photogalvanic current in WSe2 journal September 2014
Collective bulk carrier delocalization driven by electrostatic surface charge accumulation journal July 2012
Suppression of Metal-Insulator Transition in VO2 by Electric Field-Induced Oxygen Vacancy Formation journal March 2013
A high-mobility electronic system at an electrolyte-gated oxide surface journal March 2015
Electrostatic charge accumulation versus electrochemical doping in SrTiO3 electric double layer transistors journal June 2010
Suppression of Ionic Liquid Gate-Induced Metallization of SrTiO 3 (001) by Oxygen journal September 2013
Nonlinear Hall effect and multichannel conduction in LaTiO 3 / SrTiO 3 superlattices journal November 2010
Growth-induced electron mobility enhancement at the LaAlO 3 /SrTiO 3 interface journal February 2015
Enhancing Electron Mobility at the LaAlO 3 /SrTiO 3 Interface by Surface Control journal July 2013
Magneto-transport study of top- and back-gated LaAlO 3 /SrTiO 3 heterostructures journal June 2015
Tunable Rashba Spin-Orbit Interaction at Oxide Interfaces journal March 2010
A self‐consistent solution of Schrödinger–Poisson equations using a nonuniform mesh journal October 1990
Permittivity of Strontium Titanate journal May 1972
Very Large Capacitance Enhancement in a Two-Dimensional Electron System journal May 2011
Anomalous conductivity, Hall factor, magnetoresistance, and thermopower of accumulation layer in SrTiO 3 journal July 2016
Stoichiometry control of the electronic properties of the LaAlO3/SrTiO3 heterointerface journal June 2013
Control of electronic conduction at an oxide heterointerface using surface polar adsorbates journal September 2011
Shubnikov–De Haas Oscillations in SrTiO3/LaAlO3 Interface journal November 2010
Why some interfaces cannot be sharp journal January 2006

Cited By (14)

Correlation between superconductivity, band filling, and electron confinement at the LaAlO 3 / SrTiO 3 interface journal June 2018
Carrier density and disorder tuned superconductor-metal transition in a two-dimensional electron system journal October 2018
Superconducting Tunneling Spectroscopy of Spin-Orbit Coupling and Orbital Depairing in Nb : SrTiO 3 journal October 2018
Polaronic behavior in a weak-coupling superconductor journal January 2018
High efficiency superconducting field effect devices for oxide electronic applications journal January 2020
Half-metallicity in a honeycomb–kagome-lattice Mg 3 C 2 monolayer with carrier doping journal January 2018
Half-metallicity in a honeycomb-kagome-lattice Mg 3 Si 2 monolayer with carrier doping journal April 2019
Room-temperature half-metallicity in monolayer honeycomb structures of group-V binary compounds with carrier doping journal August 2017
Modulating the Electrical Transport in the Two-Dimensional Electron Gas at LaAlO 3 / SrTiO 3 Heterostructures by Interfacial Flexoelectricity journal June 2019
Gate-tunable Rashba spin-orbit coupling and spin polarization at diluted oxide interfaces journal September 2019
Physics of SrTiO 3 -based heterostructures and nanostructures: a review journal February 2018
Physics of SrTiO$_3$-based heterostructures and nanostructures: a review text January 2017
Half-metallicity in honeycomb-kagome-lattice Mg3C2 monolayer with carrier doping text January 2017
Publisher Correction: Carrier density and disorder tuned superconductor-metal transition in a two-dimensional electron system journal October 2018