Acyclic aza-containing ligands for use as catalytic carbon capture systems

Floyd, III, William C.; Valdez, Carlos A.; Aines, Roger; Baker, Sarah; Satcher, Jr., Joe H.

Title: Acyclic aza-containing ligands for use as catalytic carbon capture systems

Patent · Tue Feb 16 00:00:00 EST 2016

OSTI ID:1344783

Floyd, III, William C.; Valdez, Carlos A.; Aines, Roger; Baker, Sarah; Satcher, Jr., Joe H.

According to one embodiment, a catalyst includes a metal ion, and an acyclic ligand having at least one aza-containing moiety, where the ligand is complexed to the metal ion.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: AC52-07NA27344

Assignee:: Lawrence Livermore National Security, LLC (Livermore, CA)

Patent Number(s):: 9,259,725

Application Number:: 14/051,380

OSTI ID:: 1344783

Resource Relation:: Patent File Date: 2013 Oct 10

Country of Publication:: United States

Language:: English

References (14)

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Multidentate aza ligands able to complex metal ions and the use thereof in diagnostics and therapy Giovenzana, Giovanni Battista; Palmisano, Giovanni; Sisti, Massimo https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7186400 US Patent Document 7,186,400	patent	March 2007
Phosphodiester Hydrolysis by a New Zinc(II) Macrocyclic Tetraamine Complex with an Alcohol Pendant: Elucidation of the Roles of Ser-102 and Zinc(II) in Alkaline Phosphatase Kimura, Eiichi; Kodama, Yorimitsu; Koike, Tohru Journal of the American Chemical Society, Vol. 117, Issue 32 https://doi.org/10.1021/ja00137a002	journal	August 1995
A functional model for carbonic anhydrase: thermodynamic and kinetic study of a tetraazacyclododecane complex of zinc(II) Zhang, Xiaoping; van Eldik, Rudi Inorganic Chemistry, Vol. 34, Issue 22 https://doi.org/10.1021/ic00126a034	journal	October 1995
Catalysis By Metal-Activated Hydroxide in Zinc and Manganese Metalloenzymes Christianson, David W.; Cox, J. David Annual Review of Biochemistry, Vol. 68, Issue 1 https://doi.org/10.1146/annurev.biochem.68.1.33	journal	June 1999
Carboxy and Diphosphate Ester Hydrolysis Promoted by Dinuclear Zinc(II) Macrocyclic Complexes. Role of Zn(II)-Bound Hydroxide as the Nucleophilic Function Bencini, Andrea; Berni, Emanuela; Bianchi, Antonio Inorganic Chemistry, Vol. 38, Issue 26 https://doi.org/10.1021/ic990820g	journal	December 1999
Crystal Structures and Solution Behavior of Paramagnetic Divalent Transition Metal Complexes (Fe, Co) of the Sterically Encumbered Tridentate Macrocycles 1,4,7-R ₃ -1,4,7-Triazacyclononane: Coordination Numbers 5 (R = i -Pr) and 6 (R = i -Bu) Diebold, Alain; Elbouadili, Abdelaziz; Hagen, Karl S. Inorganic Chemistry, Vol. 39, Issue 17 https://doi.org/10.1021/ic000456h	journal	August 2000
1,4,7,10-Tetraazacyclododecane Metal Complexes as Potent Promoters of Carboxyester Hydrolysis under Physiological Conditions Subat, Michael; Woinaroschy, Kristina; Anthofer, Stefan Inorganic Chemistry, Vol. 46, Issue 10 https://doi.org/10.1021/ic070101z	journal	May 2007
Carbon Dioxide Postcombustion Capture: A Novel Screening Study of the Carbon Dioxide Absorption Performance of 76 Amines Puxty, Graeme; Rowland, Robert; Allport, Andrew Environmental Science & Technology, Vol. 43, Issue 16, p. 6427-6433 https://doi.org/10.1021/es901376a	journal	August 2009
Modern Views on Desilicification: Biosilica and Abiotic Silica Dissolution in Natural and Artificial Environments Ehrlich, Hermann; Demadis, Konstantinos D.; Pokrovsky, Oleg S. Chemical Reviews, Vol. 110, Issue 8 https://doi.org/10.1021/cr900334y	journal	August 2010
Non-CO2 greenhouse gases and climate change Montzka, S. A.; Dlugokencky, E. J.; Butler, J. H. Nature, Vol. 476, Issue 7358 https://doi.org/10.1038/nature10322	journal	August 2011
Analysis and Status of Post-Combustion Carbon Dioxide Capture Technologies Bhown, Abhoyjit S.; Freeman, Brice C. Environmental Science & Technology, Vol. 45, Issue 20 https://doi.org/10.1021/es104291d	journal	October 2011
Toward a Small Molecule, Biomimetic Carbonic Anhydrase Model: Theoretical and Experimental Investigations of a Panel of Zinc(II) Aza-Macrocyclic Catalysts Koziol, Lucas; Valdez, Carlos A.; Baker, Sarah E. Inorganic Chemistry, Vol. 51, Issue 12 https://doi.org/10.1021/ic300526b	journal	June 2012
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