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Title: Observation of a topologically non-trivial surface state in half-Heusler PtLuSb (001) thin films

Journal Article · · Nature Communications
DOI:https://doi.org/10.1038/ncomms11993· OSTI ID:1307467

The discovery of topological insulators, materials with bulk band gaps and protected cross-gap surface states in compounds such as Bi2Se3, has generated much interest in identifying topological surface states (TSSs) in other classes of materials. In particular, recent theoretical calculations suggest that TSSs may be found in half-Heusler ternary compounds. If experimentally realizable, this would provide a materials platform for entirely new heterostructure spintronic devices that make use of the structurally identical but electronically varied nature of Heusler compounds. Here we show the presence of a TSS in epitaxially grown thin films of the half-Heusler compound PtLuSb. Spin- and angle-resolved photoemission spectroscopy, complemented by theoretical calculations, reveals a surface state with linear dispersion and a helical tangential spin texture consistent with previous predictions. As a result, this experimental verification of topological behavior is a significant step forward in establishing half-Heusler compounds as a viable material system for future spintronic devices.

Research Organization:
Univ. of California, Santa Barbara, CA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0014388
OSTI ID:
1307467
Journal Information:
Nature Communications, Vol. 7; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 42 works
Citation information provided by
Web of Science

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Valence-band offsets of CoTiSb/In 0.53 Ga 0.47 As and CoTiSb/In 0.52 Al 0.48 As heterojunctions journal August 2017
Electronic structure of epitaxial half-Heusler Co 1-x Ni x TiSb across the semiconductor to metal transition journal August 2018
Nanometer scale structural and compositional inhomogeneities of half-Heusler CoTi 1-x Fe x Sb thin films journal May 2019
Heusler interfaces—Opportunities beyond spintronics? journal August 2019
Crystalline electric field study in a putative topologically trivial rare-earth doped YPdBi compound journal August 2019
Double band inversion in α -Sn: Appearance of topological surface states and the role of orbital composition journal April 2017
Model Hamiltonian and time reversal breaking topological phases of antiferromagnetic half-Heusler materials journal June 2017
Magnetotransport properties and giant anomalous Hall angle in the half-Heusler compound TbPtBi journal January 2019
Prediction of Triple Point Fermions in Simple Half-Heusler Topological Insulators journal September 2017
Linear-in-Frequency Optical Conductivity in GdPtBi due to Transitions near the Triple Points journal October 2018
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Dirac nodal lines protected against spin-orbit interaction in IrO 2 journal June 2019
Peculiar half-metallic state in zigzag nanoribbons of MoS 2 : Spin filtering journal September 2016
Double Band Inversion in $ α$-Sn: Appearance of Topological Surface States and the Role of Orbital Composition text January 2017
Model Hamiltonian and Time Reversal Breaking Topological Phases of Anti-ferromagnetic Half-Heusler Materials text January 2017
Prediction of triple point fermions in simple half-Heusler topological insulators text January 2017
Magnetotransport properties and giant anomalous Hall angle in half-Heusler compound TbPtBi text January 2019