Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis

Bu, Lingzheng; Guo, Shaojun; Zhang, Xu; Shen, Xuan; Su, Dong; Lu, Gang; Zhu, Xing; Yao, Jianlin; Guo, Jun; Huang, Xiaoqing

doi:10.1038/ncomms11850

Title: Surface engineering of hierarchical platinum-cobalt nanowires for efficient electrocatalysis

Journal Article · Wed Jun 29 00:00:00 EDT 2016 · Nature Communications

DOI:https://doi.org/10.1038/ncomms11850· OSTI ID:1307420

Bu, Lingzheng ^[1]; Guo, Shaojun ^[2]; Zhang, Xu ^[3]; Shen, Xuan ^[4]; Su, Dong ^[4]; Lu, Gang ^[3]; Zhu, Xing ^[1]; Yao, Jianlin ^[1]; Guo, Jun ^[1]; Huang, Xiaoqing ^[1]

Soochow Univ., Jiangsu (China)
Peking Univ., Beijing (China)
California State Univ. (CalState), Northridge, CA (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)

Despite intense research in past decades, the lack of high-performance catalysts for fuel cell reactions remains a challenge in realizing fuel cell technologies for transportation applications. We report a facile strategy for synthesizing hierarchical platinum-cobalt nanowires with high-index, platinum-rich facets and ordered intermetallic structure. These structural features enable unprecedented performance for the oxygen reduction and alcohol oxidation reactions. The specific/mass activities of the platinum-cobalt nanowires for oxygen reduction reaction are 39.6/33.7 times higher than commercial Pt/C catalyst, respectively. Density functional theory simulations reveal that the active threefold hollow sites on the platinum-rich high-index facets provide an additional factor in enhancing oxygen reduction reaction activities. These nanowires are stable in the electrochemical conditions and also thermally stable. Our work may represent a key step towards scalable production of high-performance platinum-based nanowires for applications in catalysis and energy conversion.

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Research Organization:: Brookhaven Science Associates, LLC, Upton, NY (United States); Brookhaven National Laboratory (BNL), Upton, NY (United States). Center for Functional Nanomaterials (CFN)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; SC00112704

OSTI ID:: 1307420

Alternate ID(s):: OSTI ID: 1336135

Report Number(s):: BNL-112606-2016-JA; ncomms11850

Journal Information:: Nature Communications, Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 523 works

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Solvent-mediated length tuning of ultrathin platinum–cobalt nanowires for efficient electrocatalysis Xu, Hui; Wei, Jingjing; Zhang, Min Journal of Materials Chemistry A, Vol. 6, Issue 47 https://doi.org/10.1039/c8ta08251k	journal	January 2018
Atomic (single, double, and triple atoms) catalysis: frontiers, opportunities, and challenges Chen, Z. W.; Chen, L. X.; Yang, C. C. Journal of Materials Chemistry A, Vol. 7, Issue 8 https://doi.org/10.1039/c8ta11416a	journal	January 2019
Localized surface plasmon enhanced electrocatalytic methanol oxidation of AgPt bimetallic nanoparticles with an ultra-thin shell Bi, Jinglei; Cai, Hairui; Wang, Bin Chemical Communications, Vol. 55, Issue 27 https://doi.org/10.1039/c9cc00331b	journal	January 2019
Synthesis of ammonia via electrochemical nitrogen reduction on high-index faceted Au nanoparticles with a high faradaic efficiency Tan, Lianqiao; Yang, Na; Huang, Xun Chemical Communications, Vol. 55, Issue 96 https://doi.org/10.1039/c9cc06132k	journal	January 2019
Regulating locations of active sites: a novel strategy to greatly improve the stability of PtAu electrocatalysts Xu, Suying; Hou, Wenjie; Jiang, Rui Chemical Communications, Vol. 55, Issue 90 https://doi.org/10.1039/c9cc07275f	journal	January 2019
Concave PtCo nanooctahedra with high-energy {110} facets for the oxygen reduction reaction Li, Zhijuan; Wang, Xiaoru; Zhang, Zhenbo CrystEngComm, Vol. 22, Issue 9 https://doi.org/10.1039/c9ce01488h	journal	January 2020
Ultra-small intermetallic NiZn nanoparticles: a non-precious metal catalyst for efficient electrocatalysis Samanta, Arnab; Das, Sankar; Jana, Subhra Nanoscale Advances, Vol. 2, Issue 1 https://doi.org/10.1039/c9na00611g	journal	January 2020
One-pot synthesis of PtIn/3D-GNs composites with high alloying degree for electro-photo synergistic catalysis Ye, Yixiang; Wang, Yanli; Li, Zhongshui New Journal of Chemistry, Vol. 43, Issue 43 https://doi.org/10.1039/c9nj04367e	journal	January 2019
In situ high-potential-driven surface restructuring of ternary AgPd–Pt _dilute aerogels with record-high performance improvement for formate oxidation electrocatalysis Wang, Jiali; Chen, Fuyi; Jin, Yachao Nanoscale, Vol. 11, Issue 30 https://doi.org/10.1039/c9nr03266e	journal	January 2019
Facile synthesis of ultrathin Pt–Pd nanosheets for enhanced formic acid oxidation and oxygen reduction reaction Yang, Qian; Shi, Lijie; Yu, Beibei Journal of Materials Chemistry A, Vol. 7, Issue 32 https://doi.org/10.1039/c9ta03945g	journal	January 2019
One-step solid-phase boronation to fabricate self-supported porous FeNiB/FeNi foam for efficient electrocatalytic oxygen evolution and overall water splitting Yuan, Hefeng; Wang, Shumin; Gu, Xundi Journal of Materials Chemistry A, Vol. 7, Issue 33 https://doi.org/10.1039/c9ta04076e	journal	January 2019
Advanced engineering of core/shell nanostructures for electrochemical carbon dioxide reduction Shao, Qi; Wang, Pengtang; Liu, Shangheng Journal of Materials Chemistry A, Vol. 7, Issue 36 https://doi.org/10.1039/c9ta07016h	journal	January 2019
Interfacial synergy of ultralong jagged Pt ₈₅ Mo ₁₅ –S nanowires with abundant active sites on enhanced hydrogen evolution in an alkaline solution Wang, Yao; Zhuo, Hongying; Zhang, Xin Journal of Materials Chemistry A, Vol. 7, Issue 42 https://doi.org/10.1039/c9ta09285d	journal	January 2019
SnO ₂ patched ultrathin PtRh nanowires as efficient catalysts for ethanol electrooxidation Fan, Xiaokun; Tang, Min; Wu, Xiaotong Journal of Materials Chemistry A, Vol. 7, Issue 48 https://doi.org/10.1039/c9ta10941b	journal	January 2019
Asymmetric PdPtCu mesoporous hemispheres on nitrogen-functionalized graphene for methanol oxidation electrocatalysis Sun, Lizhi; Lv, Hao; Xu, Dongdong Journal of Materials Chemistry A, Vol. 8, Issue 31 https://doi.org/10.1039/c9ta13478f	journal	January 2020
Cobalt-platinum nanomotors for local gas generation Szkudlarek, Aleksandra; Hnida-Gut, Katarzyna E.; Kollbek, Kamila Nanotechnology, Vol. 31, Issue 7 https://doi.org/10.1088/1361-6528/ab53bd	journal	November 2019
Monatomic Co, ${CoO}_{2}$ , and ${CoO}_{3}$ nanowires on Ir(100) and Pt(100) surfaces: Formation, structure, and energetics Ferstl, P.; Mittendorfer, F.; Redinger, J. Physical Review B, Vol. 96, Issue 8 https://doi.org/10.1103/physrevb.96.085407	journal	August 2017
Surface-modulated palladium-nickel icosahedra as high-performance non-platinum oxygen reduction electrocatalysts Feng, Yonggang; Shao, Qi; Ji, Yujin Science Advances, Vol. 4, Issue 7 https://doi.org/10.1126/sciadv.aap8817	journal	July 2018
Annealing Behaviour of Pt and PtNi Nanowires for Proton Exchange Membrane Fuel Cells Mardle, Peter; Du, Shangfeng Materials, Vol. 11, Issue 8 https://doi.org/10.3390/ma11081473	journal	August 2018
Stability of High-Performance Pt-Based Catalysts for Oxygen Reduction Reactions Lin, Rui; Cai, Xin; Zeng, Hao Advanced Materials, Vol. 30, Issue 17 https://doi.org/10.1002/adma.201705332	journal	March 2018
Ultrathin PtPd-Based Nanorings with Abundant Step Atoms Enhance Oxygen Catalysis Sun, Yingjun; Zhang, Xu; Luo, Mingchuan Advanced Materials, Vol. 30, Issue 38 https://doi.org/10.1002/adma.201802136	journal	August 2018
Alloy Nanocatalysts for the Electrochemical Oxygen Reduction (ORR) and the Direct Electrochemical Carbon Dioxide Reduction Reaction (CO ₂ RR) Kim, Cheonghee; Dionigi, Fabio; Beermann, Vera Advanced Materials, Vol. 31, Issue 31 https://doi.org/10.1002/adma.201805617	journal	December 2018
Pt‐Based Nanocrystal for Electrocatalytic Oxygen Reduction Zhao, Zipeng; Chen, Changli; Liu, Zeyan Advanced Materials, Vol. 31, Issue 31 https://doi.org/10.1002/adma.201808115	journal	December 2018
Intermetallic PtBi Nanoplates Boost Oxygen Reduction Catalysis with Superior Tolerance over Chemical Fuels Feng, Yonggang; Shao, Qi; Lv, Fan Advanced Science, Vol. 7, Issue 1 https://doi.org/10.1002/advs.201800178	journal	September 2019
A Comprehensive Review on Controlling Surface Composition of Pt-Based Bimetallic Electrocatalysts Zhang, Bin-Wei; Yang, Hui-Ling; Wang, Yun-Xiao Advanced Energy Materials, Vol. 8, Issue 20 https://doi.org/10.1002/aenm.201703597	journal	April 2018
Crystallinity-Modulated Electrocatalytic Activity of a Nickel(II) Borate Thin Layer on Ni ₃ B for Efficient Water Oxidation Jiang, Wen-Jie; Niu, Shuai; Tang, Tang Angewandte Chemie International Edition, Vol. 56, Issue 23 https://doi.org/10.1002/anie.201703183	journal	May 2017
Facile Solvothermal Synthesis of Pt ₄ Co Multi-dendrites: An Effective Electrocatalyst for Oxygen Reduction and Glycerol Oxidation Jiang, Liu-Ying; Wang, Ai-Jun; Li, Xin-Sheng ChemElectroChem, Vol. 4, Issue 11 https://doi.org/10.1002/celc.201700640	journal	September 2017
In Situ Incorporation Strategy for Bimetallic FeCo-Doped Carbon as Highly Efficient Bifunctional Oxygen Electrocatalysts Shui, Hengxin; Jin, Tian; Hu, Jun ChemElectroChem, Vol. 5, Issue 10 https://doi.org/10.1002/celc.201800013	journal	April 2018
Gold-Copper Aerogels with Intriguing Surface Electronic Modulation as Highly Active and Stable Electrocatalysts for Oxygen Reduction and Borohydride Oxidation Wang, Jiali; Chen, Fuyi; Jin, Yachao ChemSusChem, Vol. 11, Issue 8 https://doi.org/10.1002/cssc.201800052	journal	March 2018
Nanocatalysts for Electrocatalytic Oxidation of Ethanol Bai, Juan; Liu, Danye; Yang, Jun ChemSusChem, Vol. 12, Issue 10 https://doi.org/10.1002/cssc.201803063	journal	April 2019
Highly Efficient Carbon Dioxide Hydrogenation to Methanol Catalyzed by Zigzag Platinum-Cobalt Nanowires Bai, Shuxing; Shao, Qi; Feng, Yonggang Small, Vol. 13, Issue 22 https://doi.org/10.1002/smll.201604311	journal	April 2017
Highly active zigzag-like Pt-Zn alloy nanowires with high-index facets for alcohol electrooxidation Xu, Yanchao; Cui, Xiaoqiang; Wei, Shuting Nano Research, Vol. 12, Issue 5 https://doi.org/10.1007/s12274-019-2374-z	journal	April 2019
Rational Design and Synthesis of Low-Temperature Fuel Cell Electrocatalysts Tian, Na; Lu, Bang-An; Yang, Xiao-Dong Electrochemical Energy Reviews, Vol. 1, Issue 1 https://doi.org/10.1007/s41918-018-0004-1	journal	March 2018
Electrode Materials for Rechargeable Zinc-Ion and Zinc-Air Batteries: Current Status and Future Perspectives Yang, Dan; Tan, Huiteng; Rui, Xianhong Electrochemical Energy Reviews, Vol. 2, Issue 3 https://doi.org/10.1007/s41918-019-00035-5	journal	May 2019
Fabrication and enhanced hydrogen evolution reaction performance of a Cu ₃ BiS ₃ nanorods/TiO ₂ heterojunction film Li, Jiajia; Han, Xiuxun; Wang, Min New Journal of Chemistry, Vol. 42, Issue 6 https://doi.org/10.1039/c7nj04569g	journal	January 2018
One-step green synthesis of composition-tunable Pt–Cu alloy nanowire networks with high catalytic activity for 4-nitrophenol reduction Zhang, Yingfang; Xia, Yan; Yan, Saisai Dalton Transactions, Vol. 47, Issue 48 https://doi.org/10.1039/c8dt03810d	journal	January 2018
Ternary PtVCo dendrites for the hydrogen evolution reaction, oxygen evolution reaction, overall water splitting and rechargeable Zn–air batteries Ding, Zhaoqing; Tang, Zhenghua; Li, Ligui Inorganic Chemistry Frontiers, Vol. 5, Issue 10 https://doi.org/10.1039/c8qi00623g	journal	January 2018
Size-dependent synthesis and catalytic activities of trimetallic PdAgCu mesoporous nanospheres in ethanol electrooxidation Lv, Hao; Sun, Lizhi; Zou, Lu Chemical Science, Vol. 10, Issue 7 https://doi.org/10.1039/c8sc04696d	journal	January 2019
Ligand-mediated bifunctional catalysis for enhanced oxygen reduction and methanol oxidation tolerance in fuel cells Lu, Linfang; Wang, Zhiqiang; Zou, Shihui Journal of Materials Chemistry A, Vol. 6, Issue 39 https://doi.org/10.1039/c8ta06071a	journal	January 2018
The OH ⁻ -driven synthesis of Pt–Ni nanocatalysts with atomic segregation for alkaline hydrogen evolution reaction Zhang, Cong; Chen, Biaohua; Mei, Donghai Journal of Materials Chemistry A, Vol. 7, Issue 10 https://doi.org/10.1039/c8ta12250d	journal	January 2019
Multidimensional nanostructured membrane electrode assemblies for proton exchange membrane fuel cell applications Wang, Guoliang; Zou, Liangliang; Huang, Qinghong Journal of Materials Chemistry A, Vol. 7, Issue 16 https://doi.org/10.1039/c8ta12382a	journal	January 2019
Atomically dispersed metal catalysts for the oxygen reduction reaction: synthesis, characterization, reaction mechanisms and electrochemical energy applications Liu, Minmin; Wang, Linlin; Zhao, Kangning Energy & Environmental Science, Vol. 12, Issue 10 https://doi.org/10.1039/c9ee01722d	journal	January 2019
Cyanogel auto-reduction induced synthesis of PdCo nanocubes on carbon nanobowls: a highly active electrocatalyst for ethanol electrooxidation Xu, Guang-Rui; Zhai, Ya-Nan; Li, Fu-min Nanoscale, Vol. 11, Issue 28 https://doi.org/10.1039/c9nr04767k	journal	January 2019
Nanoscale engineering of porous Fe-doped Pd nanosheet assemblies for efficient methanol and ethanol electrocatalyses Xu, Hui; Shang, Hongyuan; Wang, Cheng Nanoscale, Vol. 12, Issue 3 https://doi.org/10.1039/c9nr09755d	journal	January 2020
Shaping well-defined noble-metal-based nanostructures for fabricating high-performance electrocatalysts: advances and perspectives Yin, Hai-Jing; Zhou, Jun-Hao; Zhang, Ya-Wen Inorganic Chemistry Frontiers, Vol. 6, Issue 10 https://doi.org/10.1039/c9qi00689c	journal	January 2019
Understanding the roles of amorphous domains and oxygen-containing groups of nitrogen-doped carbon in oxygen reduction catalysis: toward superior activity Biemolt, Jasper; Rothenberg, Gadi; Yan, Ning Inorganic Chemistry Frontiers, Vol. 7, Issue 1 https://doi.org/10.1039/c9qi00983c	journal	January 2020
Transition metal-doped ultrathin RuO ₂ networked nanowires for efficient overall water splitting across a broad pH range Wang, Juan; Ji, Yujin; Yin, Rongguan Journal of Materials Chemistry A, Vol. 7, Issue 11 https://doi.org/10.1039/c9ta00598f	journal	January 2019
Morphology controllable synthesis of PtNi concave nanocubes enclosed by high-index facets supported on porous graphene for enhanced hydrogen evolution reaction Yang, Juntao; Ning, Guoqing; Yu, Lei Journal of Materials Chemistry A, Vol. 7, Issue 30 https://doi.org/10.1039/c9ta03442k	journal	January 2019
Design of ultrathin Pt-Mo-Ni nanowire catalysts for ethanol electrooxidation Mao, Junjie; Chen, Wenxing; He, Dongsheng Science Advances, Vol. 3, Issue 8 https://doi.org/10.1126/sciadv.1603068	journal	August 2017
Highly Durable and Active Pt-Based Nanoscale Design for Fuel-Cell Oxygen-Reduction Electrocatalysts Chung, Dong Young; Yoo, Ji Mun; Sung, Yung-Eun Advanced Materials, Vol. 30, Issue 42 https://doi.org/10.1002/adma.201704123	journal	January 2018
Tungsten‐Doped L1 ₀ ‐PtCo Ultrasmall Nanoparticles as a High‐Performance Fuel Cell Cathode Liang, Jiashun; Li, Na; Zhao, Zhonglong Angewandte Chemie International Edition, Vol. 58, Issue 43 https://doi.org/10.1002/anie.201908824	journal	October 2019
Noble metal-free catalysts for oxygen reduction reaction Huang, Xiaoxiao; Wang, Yazhou; Li, Wei Science China Chemistry, Vol. 60, Issue 12 https://doi.org/10.1007/s11426-017-9153-6	journal	November 2017
1-Naphthol induced Pt3Ag nanocorals as bifunctional cathode and anode catalysts of direct formic acid fuel cells Jiang, Xian; Liu, Yang; Wang, Jiaxin Nano Research, Vol. 12, Issue 2 https://doi.org/10.1007/s12274-018-2218-2	journal	October 2018
Highly crystalline PtCu nanotubes with three dimensional molecular accessible and restructured surface for efficient catalysis Li, Hui-Hui; Fu, Qi-Qi; Xu, Liang Energy & Environmental Science, Vol. 10, Issue 8 https://doi.org/10.1039/c7ee00573c	journal	January 2017
Kinetically controlled synthesis of AuPt bi-metallic aerogels and their enhanced electrocatalytic performances Shi, Qiurong; Zhu, Chengzhou; Du, Dan Journal of Materials Chemistry A, Vol. 5, Issue 37 https://doi.org/10.1039/c7ta06375j	journal	January 2017
Preparation of Ni@Pt core@shell conformal nanofibre oxygen reduction electrocatalysts via microwave-assisted galvanic displacement Ercolano, Giorgio; Farina, Filippo; Stievano, Lorenzo Catalysis Science & Technology, Vol. 9, Issue 24 https://doi.org/10.1039/c9cy01514k	journal	January 2019
Semiconductor nanowire plasmonic lasers Li, Chun; Liu, Zhen; Chen, Jie Nanophotonics, Vol. 8, Issue 12 https://doi.org/10.1515/nanoph-2019-0206	journal	October 2019
Ternary PtPdCu Multicubes as a Highly Active and Durable Catalyst toward the Oxygen Reduction Reaction An, Hong Ming; Zhao, Zhi Liang; Wang, Qi ChemElectroChem, Vol. 5, Issue 10 https://doi.org/10.1002/celc.201800202	journal	March 2018
Uniformly dispersed platinum-cobalt alloy nanoparticles with stable compositions on carbon substrates for methanol oxidation reaction Liu, Hui; Li, Chengyin; Chen, Dong Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-10223-2	journal	September 2017
Wire-like Pt on mesoporous Ti0.7W0.3O2 Nanomaterial with Compelling Electro-Activity for Effective Alcohol Electro-Oxidation Pham, Hau Quoc; Huynh, Tai Thien; Mai, Anh Tram Ngoc Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-51235-4	journal	October 2019
Nanostructure Optimization of Platinum-Based Nanomaterials for Catalytic Applications Duan, Sibin; Du, Zhe; Fan, Hongsheng Nanomaterials, Vol. 8, Issue 11 https://doi.org/10.3390/nano8110949	journal	November 2018

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