A coupled effect of nuclear and electronic energy loss on ion irradiation damage in lithium niobate

Liu, Peng; Zhang, Yanwen; Xue, Haizhou; Jin, Ke; Crespillo, Miguel L.; Wang, Xuelin; Weber, William J.

doi:10.1016/j.actamat.2015.12.048

Title: A coupled effect of nuclear and electronic energy loss on ion irradiation damage in lithium niobate

Journal Article · Sat Jan 09 00:00:00 EST 2016 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2015.12.048· OSTI ID:1265946

Liu, Peng ^[1]; Zhang, Yanwen ^[2]; Xue, Haizhou ^[3]; Jin, Ke ^[4]; Crespillo, Miguel L. ^[3]; Wang, Xuelin ^[5]; Weber, William J. ^[2]

Shandong Univ., Jinan (China); Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Shandong Univ., Jinan (China)

Understanding irradiation effects induced by elastic energy loss to atomic nuclei and inelastic energy loss to electrons in a crystal, as well as the coupled effect between them, is a scientific challenge. Damage evolution in LiNbO₃ irradiated by 0.9 and 21 MeV Si ions at 300 K has been studied utilizing Rutherford backscattering spectrometry in channeling mode. During the low-energy ion irradiation process, damage accumulation produced due to elastic collisions is described utilizing a disorder accumulation model. Moreover, low electronic energy loss is shown to induce observable damage that increases with ion fluence. For the same electronic energy loss, the velocity of the incident ion could affect the energy and spatial distribution of excited electrons, and therefore effectively modify the diameter of the ion track. Furthermore, nonlinear additive phenomenon of irradiation damage induced by high electronic energy loss in pre-damaged LiNbO₃ has been observed. The result indicates that pre-existing damage induced from nuclear energy loss interacts synergistically with inelastic electronic energy loss to promote the formation of amorphous tracks and lead to rapid phase transformation, much more efficient than what is observed in pristine crystal solely induced by electronic energy loss. As a result, this synergistic effect is attributed to the fundamental mechanism that the defects produced by the elastic collisions result in a decrease in thermal conductivity, increase in the electron-phonon coupling, and further lead to higher intensity in thermal spike from intense electronic energy deposition along high-energy ion trajectory.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725; 11405097

OSTI ID:: 1265946

Alternate ID(s):: OSTI ID: 1352942

Journal Information:: Acta Materialia, Vol. 105; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 35 works

Citation information provided by
Web of Science

References (48)

The formation of waveguides and modulators in LiNbO ₃ by ion implantation Destefanis, G. L.; Gailliard, J. P.; Ligeon, E. L. Journal of Applied Physics, Vol. 50, Issue 12 https://doi.org/10.1063/1.325982	journal	December 1979
Kinetics of ion-beam damage in lithium niobate García-Navarro, A.; Agulló-López, F.; Bianconi, M. Journal of Applied Physics, Vol. 101, Issue 8 https://doi.org/10.1063/1.2714772	journal	April 2007
Damage effects produced in the near-surface region of x-cut LiNbO3 by low dose, high energy implantation of nitrogen, oxygen, and fluorine ions Bentini, G. G.; Bianconi, M.; Correra, L. Journal of Applied Physics, Vol. 96, Issue 1 https://doi.org/10.1063/1.1756219	journal	July 2004
Ionization-induced annealing of pre-existing defects in silicon carbide Zhang, Yanwen; Sachan, Ritesh; Pakarinen, Olli H. Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9049	journal	August 2015
Radiation effects in nuclear materials: Role of nuclear and electronic energy losses and their synergy Thomé, Lionel; Debelle, A.; Garrido, F. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 307 https://doi.org/10.1016/j.nimb.2012.11.077	journal	July 2013
Competing effects of electronic and nuclear energy loss on microstructural evolution in ionic-covalent materials Zhang, Y.; Varga, T.; Ishimaru, M. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 327 https://doi.org/10.1016/j.nimb.2013.10.095	journal	May 2014
Structure and band gap determination of irradiation-induced amorphous nano-channels in LiNbO ₃ Sachan, R.; Pakarinen, O. H.; Liu, P. Journal of Applied Physics, Vol. 117, Issue 13 https://doi.org/10.1063/1.4915932	journal	April 2015
Generation of high-confinement step-like optical waveguides in LiNbO3 by swift heavy ion-beam irradiation Olivares, J.; García, G.; García-Navarro, A. Applied Physics Letters, Vol. 86, Issue 18 https://doi.org/10.1063/1.1922082	journal	May 2005
Lattice preamorphization by ion irradiation: Fluence dependence of the electronic stopping power threshold for amorphization Agulló-López, F.; García, G.; Olivares, J. Journal of Applied Physics, Vol. 97, Issue 9 https://doi.org/10.1063/1.1896444	journal	May 2005
Optical determination of three-dimensional nanotrack profiles generated by single swift-heavy ion impacts in lithium niobate Olivares, J.; García-Navarro, A.; García, G. Applied Physics Letters, Vol. 89, Issue 7 https://doi.org/10.1063/1.2236221	journal	August 2006
Defect-induced melting and solid-state amorphization Fecht, H. J. Nature, Vol. 356, Issue 6365 https://doi.org/10.1038/356133a0	journal	March 1992
Assessment of swift-ion damage by RBS/C: Determination of the amorphization threshold Rivera, A.; Olivares, J.; Crespillo, M. L. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 267, Issue 8-9 https://doi.org/10.1016/j.nimb.2009.01.134	journal	May 2009
Effect of defect accumulation on ion-beam damage morphology by electronic excitation in lithium niobate: A MonteCarlo approach Rivera, A.; Crespillo, M. L.; Olivares, J. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 13 https://doi.org/10.1016/j.nimb.2010.03.031	journal	July 2010
Giant enhancement of material damage associated to electronic excitation during ion irradiation: The case of LiNbO ₃: Material degradation associated to electronic excitation during ion irradiation Rivera, A.; Olivares, J.; García, G. physica status solidi (a), Vol. 206, Issue 6 https://doi.org/10.1002/pssa.200824409	journal	March 2009
Amorphization kinetics under swift heavy ion irradiation: A cumulative overlapping-track approach García, G.; Rivera, A.; Crespillo, M. L. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 269, Issue 4 https://doi.org/10.1016/j.nimb.2010.12.073	journal	February 2011
Periodic poling of optical waveguides produced by swift-heavy-ion irradiation in LiNbO3 Caballero-Calero, O.; García-Cabañes, A.; Carrascosa, M. Applied Physics B, Vol. 95, Issue 3 https://doi.org/10.1007/s00340-009-3458-3	journal	March 2009
Photorefractive response and optical damage of LiNbO3 optical waveguides produced by swift heavy ion irradiation Villarroel, J.; Carrascosa, M.; García-Cabañes, A. Applied Physics B, Vol. 95, Issue 3 https://doi.org/10.1007/s00340-009-3386-2	journal	February 2009
Dimensional changes of metallic glasses during bombardment with fast heavy ions Hou, Ming-dong; Klaumünzer, S.; Schumacher, G. Physical Review B, Vol. 41, Issue 2 https://doi.org/10.1103/PhysRevB.41.1144	journal	January 1990
Effects induced by high electronic excitations in pure metals: A detailed study in iron Dunlop, A.; Lesueur, D.; Legrand, P. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 90, Issue 1-4 https://doi.org/10.1016/0168-583X(94)95566-2	journal	May 1994
Influence of chemical disorder on energy dissipation and defect evolution in concentrated solid solution alloys Zhang, Yanwen; Stocks, G. Malcolm; Jin, Ke Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms9736	journal	October 2015
Molecular dynamics simulations of swift heavy ion induced defect recovery in SiC Backman, M.; Toulemonde, M.; Pakarinen, O. H. Computational Materials Science, Vol. 67 https://doi.org/10.1016/j.commatsci.2012.09.010	journal	February 2013
Athermal crystallization induced by electronic excitations in ion-irradiated silicon carbide Benyagoub, A.; Audren, A.; Thomé, L. Applied Physics Letters, Vol. 89, Issue 24 https://doi.org/10.1063/1.2405410	journal	December 2006
MeV gold irradiation induced damage in α-quartz: Competition between nuclear and electronic stopping Toulemonde, M.; Ramos, S. M. M.; Bernas, H. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 178, Issue 1-4 https://doi.org/10.1016/S0168-583X(00)00496-1	journal	May 2001
Synergy of elastic and inelastic energy loss on ion track formation in SrTiO3 Weber, William J.; Zarkadoula, Eva; Pakarinen, Olli H. Scientific Reports, Vol. 5, Issue 1 https://doi.org/10.1038/srep07726	journal	January 2015
Radiation damage by light- and heavy-ion bombardment of single-crystal LiNbO_3 Huang, Hsu-Cheng; Zhang, Lihua; Malladi, Girish Optical Materials Express, Vol. 5, Issue 5 https://doi.org/10.1364/OME.5.001071	journal	January 2015
The role of electronic energy loss in ion beam modification of materials Weber, William J.; Duffy, Dorothy M.; Thomé, Lionel Current Opinion in Solid State and Materials Science, Vol. 19, Issue 1 https://doi.org/10.1016/j.cossms.2014.09.003	journal	February 2015
SRIM – The stopping and range of ions in matter (2010) Ziegler, James F.; Ziegler, M. D.; Biersack, J. P. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 268, Issue 11-12 https://doi.org/10.1016/j.nimb.2010.02.091	journal	June 2010
High Aspect Ratio Microstructures in LiNbO ₃ Produced by Ion Beam Enhanced Etching Schrempel, Frank; Gischkat, Thomas; Hartung, Holger MRS Proceedings, Vol. 908 https://doi.org/10.1557/PROC-0908-OO16-01	journal	January 2005
New ion beam materials laboratory for materials modification and irradiation effects research Zhang, Y.; Crespillo, M. L.; Xue, H. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 338 https://doi.org/10.1016/j.nimb.2014.07.028	journal	November 2014
Experimental determination of track cross-section in Gd3Ga5O12 and comparison to the inelastic thermal spike model applied to several materials Meftah, A.; Costantini, J. M.; Khalfaoui, N. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 237, Issue 3-4 https://doi.org/10.1016/j.nimb.2005.02.025	journal	August 2005
Response of strontium titanate to ion and electron irradiation Zhang, Y.; Lian, J.; Zhu, Z. Journal of Nuclear Materials, Vol. 389, Issue 2 https://doi.org/10.1016/j.jnucmat.2009.02.014	journal	May 2009
Damage accumulation and defect relaxation in $4 H − SiC$ Zhang, Y.; Gao, F.; Jiang, W. Physical Review B, Vol. 70, Issue 12 https://doi.org/10.1103/PhysRevB.70.125203	journal	September 2004
Effects of implantation temperature on damage accumulation in Al-implanted 4H–SiC Zhang, Y.; Weber, W. J.; Jiang, W. Journal of Applied Physics, Vol. 95, Issue 8 https://doi.org/10.1063/1.1666974	journal	April 2004
Atomic collision and ionization effects in oxides Zhang, Y.; Bae, In-Tae; Weber, W. J. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 266, Issue 12-13 https://doi.org/10.1016/j.nimb.2008.03.197	journal	June 2008
Models and mechanisms of irradiation-induced amorphization in ceramics Weber, W. J. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 166-167 https://doi.org/10.1016/S0168-583X(99)00643-6	journal	May 2000
Latent track formation in LiNbO ₃ single crystals irradiated by GeV uranium ions Canut, B.; Brenier, R.; Meftah, A. Radiation Effects and Defects in Solids, Vol. 136, Issue 1-4 https://doi.org/10.1080/10420159508218840	journal	December 1995
The concept of effective electronic stopping power for modelling the damage cross-section in refractory oxides irradiated by GeV ions or MeV clusters Canut, B.; Ramos, S. M. M. Radiation Effects and Defects in Solids, Vol. 145, Issue 1-2 https://doi.org/10.1080/10420159808220019	journal	July 1998
Damage induced by high electronic stopping power in SiO2 quartz Toulemonde, M.; Balanzat, E.; Bouffard, S. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 46, Issue 1-4 https://doi.org/10.1016/0168-583X(90)90670-P	journal	February 1990
Channeling irradiation of LiNbO3 Schrempel, F.; Steinbach, T.; Gischkat, Th. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 266, Issue 12-13 https://doi.org/10.1016/j.nimb.2008.03.147	journal	June 2008
Motion of swift charged particles, as influenced by strings of atoms in crystals Lindhard, J. Physics Letters, Vol. 12, Issue 2 https://doi.org/10.1016/0031-9163(64)91133-3	journal	September 1964
Swift heavy ions in magnetic insulators: A damage-cross-section velocity effect Meftah, A.; Brisard, F.; Costantini, J. M. Physical Review B, Vol. 48, Issue 2 https://doi.org/10.1103/PhysRevB.48.920	journal	July 1993
Mechanism of the swift heavy ion induced epitaxial recrystallization in predamaged silicon carbide Benyagoub, A.; Audren, A. Journal of Applied Physics, Vol. 106, Issue 8 https://doi.org/10.1063/1.3236627	journal	October 2009
Ion implantation in semiconductors—Part II: Damage production and annealing Gibbons, J. F. Proceedings of the IEEE, Vol. 60, Issue 9 https://doi.org/10.1109/PROC.1972.8854	journal	January 1972
The radial distribution of dose around the path of a heavy ion in liquid water Waligórski, M. P. R.; Hamm, R. N.; Katz, R. International Journal of Radiation Applications and Instrumentation. Part D. Nuclear Tracks and Radiation Measurements, Vol. 11, Issue 6 https://doi.org/10.1016/1359-0189(86)90057-9	journal	January 1986
Thermal conductivity degradation of ceramic materials due to low temperature, low dose neutron irradiation Snead, L. L.; Zinkle, S. J.; White, D. P. Journal of Nuclear Materials, Vol. 340, Issue 2-3 https://doi.org/10.1016/j.jnucmat.2004.11.009	journal	April 2005
Effect of ion irradiation on the thermal conductivity of UO2 and U3O8 epitaxial layers Weisensee, Patricia B.; Feser, Joseph P.; Cahill, David G. Journal of Nuclear Materials, Vol. 443, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2013.07.021	journal	November 2013
Ion beam modification of dielectric materials in the electronic excitation regime: Cumulative and exciton models Agulló-López, Fernando; Climent-Font, Aurelio; Muñoz-Martín, Ángel Progress in Materials Science, Vol. 76 https://doi.org/10.1016/j.pmatsci.2015.06.002	journal	March 2016
Thick optical waveguides in lithium niobate induced by swift heavy ions (~10 MeV/amu) at ultralow fluences Olivares, José; Crespillo, Miguel L.; Caballero-Calero, Olga Optics Express, Vol. 17, Issue 26 https://doi.org/10.1364/OE.17.024175	journal	January 2009

Cited By (4)

Effects of intermediate energy heavy‐ion irradiation on the microstructure of rutile TiO ₂ single crystal Smith, Kassiopeia A.; Savva, Andreas I.; Wu, Yaqiao Journal of the American Ceramic Society, Vol. 101, Issue 9 https://doi.org/10.1111/jace.15576	journal	April 2018
Two-stage synergy of electronic energy loss with defects in LiTaO 3 under ion irradiation Sellami, Neila; Crespillo, Miguel L.; Zhang, Yanwen Materials Research Letters, Vol. 6, Issue 6 https://doi.org/10.1080/21663831.2018.1455753	journal	March 2018
Effect of proton irradiation on anatase TiO2 nanotube anodes for lithium-ion batteries Smith, Kassiopeia A.; Savva, Andreas I.; Mao, Keyou S. Journal of Materials Science, Vol. 54, Issue 20 https://doi.org/10.1007/s10853-019-03825-w	journal	July 2019
Latent tracks and novel infrared waveguide formation in lithium tantalate irradiated with swift heavy ions Liu, Yong; Crespillo, Miguel L.; Huang, Qing Journal of Physics D: Applied Physics, Vol. 52, Issue 17 https://doi.org/10.1088/1361-6463/ab0534	journal	February 2019

Similar Records

Role of atomic-level defects and electronic energy loss on amorphization in LiNbO₃ single crystals

Journal Article · Tue Jun 20 00:00:00 EDT 2017 · Journal of Physics. D, Applied Physics · OSTI ID:1265946

Sellami, N.; Crespillo, M. L.; Xue, H.; +2 more

Structural damage response of lanthanum and yttrium aluminate crystals to nuclear collisions and electronic excitation: Threshold assessment of irradiation damage

Journal Article · Sat Apr 24 00:00:00 EDT 2021 · Journal of Materials Science and Technology · OSTI ID:1265946

Liu, Yong; Han, Xinqing; Huang, Qing; +4 more

Femtosecond laser and swift-ion damage in lithium niobate: A comparative analysis

Journal Article · Thu May 01 00:00:00 EDT 2008 · Journal of Applied Physics · OSTI ID:1265946

Garcia-Navarro, A; Agullo-Lopez, F; Olivares, J; +2 more

Related Subjects

73 NUCLEAR PHYSICS AND RADIATION PHYSICS
lithium niobate
radiation damage
coupled model
irradiation effect
order to disorder phase transformation
microstructure formation mechanism

Title: A coupled effect of nuclear and electronic energy loss on ion irradiation damage in lithium niobate

Citation Formats

References (48)

Cited By (4)

Similar Records

Related Subjects