Optical spectroscopy of the Weyl semimetal TaAs

Xu, B.; Dai, Y. M.; Zhao, L. X.; Wang, K.; Yang, R.; Zhang, W.; Liu, J. Y.; Xiao, H.; Chen, G. F.; Taylor, A. J.; Yarotski, D. A.; Prasankumar, R. P.; Qiu, X. G.

doi:10.1103/PhysRevB.93.121110

Title: Optical spectroscopy of the Weyl semimetal TaAs

Journal Article · Thu Mar 24 00:00:00 EDT 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.93.121110· OSTI ID:1258444

Xu, B. ^[1]; Dai, Y. M. ^[2]; Zhao, L. X. ^[1]; Wang, K. ^[1]; Yang, R. ^[1]; Zhang, W. ^[1]; Liu, J. Y. ^[1]; Xiao, H. ^[1]; Chen, G. F. ^[3]; Taylor, A. J. ^[2]; Yarotski, D. A. ^[2]; Prasankumar, R. P. ^[2]; Qiu, X. G. ^[3]

Chinese Academy of Sciences (CAS), Beijing (China)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Chinese Academy of Sciences (CAS), Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)

Here, we present a systematic study of both the temperature and frequency dependence of the optical response in TaAs, a material that has recently been realized to host the Weyl semimetal state. Our study reveals that the optical conductivity of TaAs features a narrow Drude response alongside a conspicuous linear dependence on frequency. The weight of the Drude peak decreases upon cooling, following a T² temperature dependence, in good agreement with theoretical predictions. Two linear components with distinct slopes dominate the low-temperature optical conductivity. A comparison between our experimental results and theoretical calculations suggests that the linear conductivity below ~230 cm^–1 arises purely from interband transitions near the Weyl points, providing rich information about the Weyl semimetal state in TaAs.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: 2015CB921303; 2015CB921102; 2012CB921302; 2012CB821403; 91121004; 91421304; 11374345; AC52-06NA25396

OSTI ID:: 1258444

Alternate ID(s):: OSTI ID: 1243157

Report Number(s):: LA-UR-15-27435; PRBMDO

Journal Information:: Physical Review B, Vol. 93, Issue 12; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 136 works

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Signatures of merging Dirac points in optics and transport Carbotte, J. P.; Nicol, E. J. arXiv https://doi.org/10.48550/arxiv.1908.02796	text	January 2019
Effect of mechanical strain on the optical properties of nodal-line semimetal ZrSiS Zhou, Weiqing; Rudenko, A. N.; Yuan, Shengjun arXiv https://doi.org/10.48550/arxiv.1908.08789	text	January 2019
Advanced Materials and Device Architectures for Magnetooptical Spatial Light Modulators Kharratian, Soheila; Urey, Hakan; Onbaşlı, Mehmet C. arXiv https://doi.org/10.48550/arxiv.1909.07494	text	January 2019

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36 MATERIALS SCIENCE
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Title: Optical spectroscopy of the Weyl semimetal TaAs

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