Anisotropic in-plane thermal conductivity of black phosphorus nanoribbons at temperatures higher than 100 K

Lee, Sangwook; Yang, Fan; Suh, Joonki; Yang, Sijie; Lee, Yeonbae; Li, Guo; Sung Choe, Hwan; Suslu, Aslihan; Chen, Yabin; Ko, Changhyun; Park, Joonsuk; Liu, Kai; Li, Jingbo; Hippalgaonkar, Kedar; Urban, Jeffrey J.; Tongay, Sefaattin; Wu, Junqiao

doi:10.1038/ncomms9573

Title: Anisotropic in-plane thermal conductivity of black phosphorus nanoribbons at temperatures higher than 100 K

Journal Article · Fri Oct 16 00:00:00 EDT 2015 · Nature Communications

DOI:https://doi.org/10.1038/ncomms9573· OSTI ID:1256041

Lee, Sangwook ^[1]; Yang, Fan ^[2]; Suh, Joonki ^[1]; Yang, Sijie ^[3]; Lee, Yeonbae ^[1]; Li, Guo ^[2]; Sung Choe, Hwan ^[1]; Suslu, Aslihan ^[3]; Chen, Yabin ^[1]; Ko, Changhyun ^[1]; Park, Joonsuk ^[4]; Liu, Kai ^[5]; Li, Jingbo; Hippalgaonkar, Kedar ^[6]; Urban, Jeffrey J. ^[2]; Tongay, Sefaattin ^[3]; Wu, Junqiao ^[7]

Univ. of California, Berkeley, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Arizona State Univ., Mesa, AZ (United States)
Stanford Univ., CA (United States)
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Institute of Materials Research and Engineering (Singapore). A*STAR
Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)

Black phosphorus attracts enormous attention as a promising layered material for electronic, optoelectronic and thermoelectric applications. Here we report large anisotropy in in-plane thermal conductivity of single-crystal black phosphorus nanoribbons along the zigzag and armchair lattice directions at variable temperatures. Thermal conductivity measurements were carried out under the condition of steady-state longitudinal heat flow using suspendedpad micro-devices. We discovered increasing thermal conductivity anisotropy, up to a factor of two, with temperatures above 100 K. A size effect in thermal conductivity was also observed in which thinner nanoribbons show lower thermal conductivity. Analysed with the relaxation time approximation model using phonon dispersions obtained based on density function perturbation theory, the high anisotropy is attributed mainly to direction-dependent phonon dispersion and partially to phonon-phonon scattering. Our results revealing the intrinsic, orientation-dependent thermal conductivity of black phosphorus are useful for designing devices, as well as understanding fundamental physical properties of layered materials.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: FG02-11ER46796; AC02-05CH11231

OSTI ID:: 1256041

Alternate ID(s):: OSTI ID: 1407299

Journal Information:: Nature Communications, Vol. 6; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 246 works

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Hybrid nanocomposites of 2D black phosphorus nanosheets encapsulated in PMMA polymer material: new platforms for advanced device fabrication Telesio, Francesca; Passaglia, Elisa; Cicogna, Francesca Nanotechnology, Vol. 29, Issue 29 https://doi.org/10.1088/1361-6528/aabd8d	journal	May 2018
Quasi-bonding driven abnormal isotropic thermal transport in intrinsically anisotropic nanostructure: a case of study of a phosphorus nanotube array Liu, Qingyi; Ouyang, Tao; Qin, Guangzhao Nanotechnology, Vol. 31, Issue 9 https://doi.org/10.1088/1361-6528/ab57b0	journal	December 2019
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The rising star of 2D black phosphorus beyond graphene: synthesis, properties and electronic applications Chen, Pengfei; Li, Neng; Chen, Xingzhu 2D Materials, Vol. 5, Issue 1 https://doi.org/10.1088/2053-1583/aa8d37	journal	October 2017
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Graphene related materials for thermal management Fu, Yifeng; Hansson, Josef; Liu, Ya 2D Materials, Vol. 7, Issue 1 https://doi.org/10.1088/2053-1583/ab48d9	journal	October 2019
Isotropic charge screening of anisotropic black phosphorus revealed by potassium adatoms Tian, Zhen; Gan, Yu; Zhang, Taiming Physical Review B, Vol. 100, Issue 8 https://doi.org/10.1103/physrevb.100.085440	journal	August 2019
Supersonic thermal excitation-induced shock wave in black phosphorene Chen, Jige; Chen, Shunda; Gao, Yi Physical Review B, Vol. 95, Issue 13 https://doi.org/10.1103/physrevb.95.134301	journal	April 2017
Anomalously low electronic thermal conductivity in metallic vanadium dioxide Lee, Sangwook; Hippalgaonkar, Kedar; Yang, Fan Science, Vol. 355, Issue 6323 https://doi.org/10.1126/science.aag0410	journal	January 2017
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Biaxial hyperbolic metamaterials using anisotropic few-layer black phosphorus Song, Xianglian; Liu, Zizhuo; Xiang, Yuanjiang Optics Express, Vol. 26, Issue 5 https://doi.org/10.1364/oe.26.005469	journal	January 2018
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Black Arsenic: A Layered Semiconductor with Extreme in-plane Anisotropy Chen, Yabin; Chen, Chaoyu; Kealhofer, Robert arXiv https://doi.org/10.48550/arxiv.1805.00418	preprint	January 2018
Anisotropic thermal conductivity measurement using a new Asymmetric-Beam Time-Domain Thermoreflectance (AB-TDTR) method Li, Man; Kang, Joon Sang; Hu, Yongjie arXiv https://doi.org/10.48550/arxiv.1809.10543	text	January 2018
Isotropic charge screening of the anisotropic black phosphorus revealed by potassium adatoms Tian, Zhen; Gan, Yu; Zhang, Taiming arXiv https://doi.org/10.48550/arxiv.1908.06554	text	January 2019
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