Interfacial charge-mediated non-volatile magnetoelectric coupling in Co0.3Fe0.7/Ba0.6Sr0.4TiO3/Nb:SrTiO3 multiferroic heterostructures

Zhou, Ziyao; Howe, Brandon M.; Liu, Ming; Nan, Tianxiang; Chen, Xing; Mahalingam, Krishnamurthy; Sun, Nian X.; Brown, Gail J.

doi:10.1038/srep07740

Title: Interfacial charge-mediated non-volatile magnetoelectric coupling in Co_0.3Fe_0.7/Ba_0.6Sr_0.4TiO₃/Nb:SrTiO₃ multiferroic heterostructures

Journal Article · Tue Jan 13 00:00:00 EST 2015 · Scientific Reports

DOI:https://doi.org/10.1038/srep07740· OSTI ID:1222944

Zhou, Ziyao ^[1]; Howe, Brandon M. ^[2]; Liu, Ming ^[2]; Nan, Tianxiang ^[3]; Chen, Xing ^[4]; Mahalingam, Krishnamurthy ^[2]; Sun, Nian X. ^[3]; Brown, Gail J. ^[2]

Northeastern Univ., Boston, MA (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Air Force Research Lab. (AFRL), Wright-Patterson AFB, OH (United States)
Northeastern Univ., Boston, MA (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)

The central challenge in realizing non-volatile, E-field manipulation of magnetism lies in finding an energy efficient means to switch between the distinct magnetic states in a stable and reversible manner. In this work, we demonstrate using electrical polarization-induced charge screening to change the ground state of magnetic ordering in order to non-volatilely tune magnetic properties in ultra-thin Co_0.3Fe_0.7/Ba_0.6Sr_0.4TiO₃/Nb:SrTiO₃ (001) multiferroic heterostructures. A robust, voltage-induced, non-volatile manipulation of out-of-plane magnetic anisotropy up to 40 Oe is demonstrated and confirmed by ferromagnetic resonance measurements. This discovery provides a framework for realizing charge-sensitive order parameter tuning in ultra-thin multiferroic heterostructures, demonstrating great potential for delivering compact, lightweight, reconfigurable, and energy-efficient electronic devices.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1222944

Journal Information:: Scientific Reports, Vol. 5; ISSN 2045-2322

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 31 works

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Title: Interfacial charge-mediated non-volatile magnetoelectric coupling in Co0.3Fe0.7/Ba0.6Sr0.4TiO3/Nb:SrTiO3 multiferroic heterostructures

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Title: Interfacial charge-mediated non-volatile magnetoelectric coupling in Co_0.3Fe_0.7/Ba_0.6Sr_0.4TiO₃/Nb:SrTiO₃ multiferroic heterostructures