Thermal flux limited electron Kapitza conductance in copper-niobium multilayers

Cheaito, Ramez; Hattar, Khalid Mikhiel; Gaskins, John T.; Yadav, Ajay K.; Duda, John C.; Beechem, III, Thomas Edwin; Ihlefeld, Jon; Piekos, Edward S.; Baldwin, Jon K.; Misra, Amit; Hopkins, Patrick E.

doi:10.1063/1.4913420

Title: Thermal flux limited electron Kapitza conductance in copper-niobium multilayers

Journal Article · Thu Mar 05 00:00:00 EST 2015 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4913420· OSTI ID:1183079

Cheaito, Ramez ^[1]; Hattar, Khalid Mikhiel ^[2]; Gaskins, John T. ^[1]; Yadav, Ajay K. ^[3]; Duda, John C. ^[1]; Beechem, III, Thomas Edwin ^[2]; Ihlefeld, Jon ^[2]; Piekos, Edward S. ^[2]; Baldwin, Jon K. ^[4]; Misra, Amit ^[5]; Hopkins, Patrick E. ^[1]

Univ. of Virginia, Charlottesville, VA (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Univ. of California, Berkeley, CA (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Univ. of Michigan, Ann Arbor, MI (United States)

We study the interplay between the contributions of electron thermal flux and interface scattering to the Kapitza conductance across metal-metal interfaces through measurements of thermal conductivity of copper-niobium multilayers. Thermal conductivities of copper-niobium multilayer films of period thicknesses ranging from 5.4 to 96.2 nm and sample thicknesses ranging from 962 to 2677 nm are measured by time-domain thermoreflectance over a range of temperatures from 78 to 500 K. The Kapitza conductances between the Cu and Nb interfaces in multilayer films are determined from the thermal conductivities using a series resistor model and are in good agreement with the electron diffuse mismatch model. Our results for the thermal boundary conductance between Cu and Nb are compared to literature values for the thermal boundary conductance across Al-Cu and Pd-Ir interfaces, and demonstrate that the interface conductance in metallic systems is dictated by the temperature derivative of the electron energy flux in the metallic layers, rather than electron mean free path or scattering processes at the interface.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1183079

Alternate ID(s):: OSTI ID: 1420541

Report Number(s):: SAND-2014-16696J; 534589

Journal Information:: Applied Physics Letters, Vol. 106, Issue 09; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 20 works

Citation information provided by
Web of Science

References (30)

Nanoscale thermal transport Cahill, David G.; Ford, Wayne K.; Goodson, Kenneth E. Journal of Applied Physics, Vol. 93, Issue 2, p. 793-818 https://doi.org/10.1063/1.1524305	journal	January 2003
Thermal boundary resistance Swartz, E. T.; Pohl, R. O. Reviews of Modern Physics, Vol. 61, Issue 3, p. 605-668 https://doi.org/10.1103/RevModPhys.61.605	journal	July 1989
Thermal Transport across Solid Interfaces with Nanoscale Imperfections: Effects of Roughness, Disorder, Dislocations, and Bonding on Thermal Boundary Conductance Hopkins, Patrick E. ISRN Mechanical Engineering, Vol. 2013 https://doi.org/10.1155/2013/682586	journal	January 2013
Energy dissipation and transport in nanoscale devices Pop, Eric Nano Research, Vol. 3, Issue 3 https://doi.org/10.1007/s12274-010-1019-z	journal	March 2010
Tuning Phonon Transport: From Interfaces to Nanostructures Norris, Pamela M.; Le, Nam Q.; Baker, Christopher H. Journal of Heat Transfer, Vol. 135, Issue 6 https://doi.org/10.1115/1.4023584	journal	May 2013
Design of radiation resistant metallic multilayers for advanced nuclear systems Zhernenkov, Mikhail; Gill, Simerjeet; Stanic, Vesna Applied Physics Letters, Vol. 104, Issue 24 https://doi.org/10.1063/1.4883481	journal	June 2014
Design of Radiation Tolerant Nanostructured Metallic Multilayers Zhang, X.; Fu, E. G.; Li, Nan Journal of Engineering Materials and Technology, Vol. 134, Issue 4 https://doi.org/10.1115/1.4006979	journal	August 2012
Field-dependent thermoelectric power and thermal conductivity in multilayered and granular giant magnetoresistive systems Shi, Jing; Pettit, Kevin; Kita, E. Physical Review B, Vol. 54, Issue 21 https://doi.org/10.1103/PhysRevB.54.15273	journal	December 1996
Field-dependent thermal and electrical transports in Cu∕CoFe multilayer Yang, Y.; Zhu, J. -G.; White, R. M. Journal of Applied Physics, Vol. 99, Issue 6 https://doi.org/10.1063/1.2174124	journal	March 2006
Perpendicular-current studies of electron transport across metal/metal interfaces Pratt, W. P.; Bass, J. Applied Surface Science, Vol. 256, Issue 2 https://doi.org/10.1016/j.apsusc.2009.06.008	journal	October 2009
Measurements of transport properties of Ag/Al and Ag/Cu multilayered films Soe, W. -H.; Kaizuka, T.; Yamamoto, R. Journal of Magnetism and Magnetic Materials, Vol. 126, Issue 1-3 https://doi.org/10.1016/0304-8853(93)90655-L	journal	September 1993
Experimental Validation of the Interfacial Form of the Wiedemann-Franz Law Wilson, R. B.; Cahill, David G. Physical Review Letters, Vol. 108, Issue 25 https://doi.org/10.1103/PhysRevLett.108.255901	journal	June 2012
Role of electron–phonon coupling in thermal conductance of metal–nonmetal interfaces Majumdar, Arun; Reddy, Pramod Applied Physics Letters, Vol. 84, Issue 23 https://doi.org/10.1063/1.1758301	journal	June 2004
Electronic Kapitza conductance due to inelastic electron-boundary scattering Sergeev, A. V. Physical Review B, Vol. 58, Issue 16 https://doi.org/10.1103/PhysRevB.58.R10199	journal	October 1998
Spectral analysis of thermal boundary conductance across solid/classical liquid interfaces: A molecular dynamics study Giri, Ashutosh; Hopkins, Patrick E. Applied Physics Letters, Vol. 105, Issue 3 https://doi.org/10.1063/1.4891332	journal	July 2014
Effects of electron scattering at metal-nonmetal interfaces on electron-phonon equilibration in gold films Hopkins, Patrick E.; Kassebaum, Jared L.; Norris, Pamela M. Journal of Applied Physics, Vol. 105, Issue 2 https://doi.org/10.1063/1.3068476	journal	January 2009
Thermal conductance of metal-metal interfaces Gundrum, Bryan C.; Cahill, David G.; Averback, Robert S. Physical Review B, Vol. 72, Issue 24 https://doi.org/10.1103/PhysRevB.72.245426	journal	December 2005
Effects of subconduction band excitations on thermal conductance at metal-metal interfaces Hopkins, Patrick E.; Beechem, Thomas E.; Duda, John C. Applied Physics Letters, Vol. 96, Issue 1 https://doi.org/10.1063/1.3276908	journal	January 2010
Time-resolved thermal transport in compositionally modulated metal films Clemens, Bruce M.; Eesley, Gary L.; Paddock, Carolyn A. Physical Review B, Vol. 37, Issue 3 https://doi.org/10.1103/PhysRevB.37.1085	journal	January 1988
Electrons and Phonons Ziman, J. M. https://doi.org/10.1093/acprof:oso/9780198507796.001.0001	book	January 2001
Thermal-conductivity measurements of GaAs/AlAs superlattices using a picosecond optical pump-and-probe technique Capinski, W. S.; Maris, H. J.; Ruf, T. Physical Review B, Vol. 59, Issue 12 https://doi.org/10.1103/PhysRevB.59.8105	journal	March 1999
Thermal conductivity of Si/SiGe and SiGe/SiGe superlattices Huxtable, Scott T.; Abramson, Alexis R.; Tien, Chang-Lin Applied Physics Letters, Vol. 80, Issue 10 https://doi.org/10.1063/1.1455693	journal	March 2002
Ultra-Low Thermal Conductivity in W/Al2O3 Nanolaminates Costescu, R. M. Science, Vol. 303, Issue 5660 https://doi.org/10.1126/science.1093711	journal	February 2004
Heat-Transport Mechanisms in Superlattices Koh, Yee Kan; Cao, Yu; Cahill, David G. Advanced Functional Materials, Vol. 19, Issue 4 https://doi.org/10.1002/adfm.200800984	journal	February 2009
A thermodynamic analysis of the binary alloy systems Cu-Cr, Cu-Nb and Cu-V Hämäläinen, M.; Jääskeläinen, K.; Luoma, R. Calphad, Vol. 14, Issue 2 https://doi.org/10.1016/0364-5916(90)90014-Q	journal	April 1990
Unusual alloying behavior at the equilibrium immiscible Cu–Nb interfaces Gong, H. R.; Liu, B. X. Journal of Applied Physics, Vol. 96, Issue 5 https://doi.org/10.1063/1.1775042	journal	September 2004
Thermal stability of self-supported nanolayered Cu/Nb films Misra, A.; Hoagland, R. G.; Kung ‡, H. Philosophical Magazine, Vol. 84, Issue 10 https://doi.org/10.1080/14786430310001659480	journal	April 2004
Analysis of heat flow in layered structures for time-domain thermoreflectance Cahill, David G. Review of Scientific Instruments, Vol. 75, Issue 12 https://doi.org/10.1063/1.1819431	journal	December 2004
Pulse accumulation, radial heat conduction, and anisotropic thermal conductivity in pump-probe transient thermoreflectance Schmidt, Aaron J.; Chen, Xiaoyuan; Chen, Gang Review of Scientific Instruments, Vol. 79, Issue 11 https://doi.org/10.1063/1.3006335	journal	November 2008
Criteria for Cross-Plane Dominated Thermal Transport in Multilayer Thin Film Systems During Modulated Laser Heating Hopkins, Patrick E.; Serrano, Justin R.; Phinney, Leslie M. Journal of Heat Transfer, Vol. 132, Issue 8 https://doi.org/10.1115/1.4000993	journal	May 2010

Cited By (7)

A Review of Experimental and Computational Advances in Thermal Boundary Conductance and Nanoscale Thermal Transport across Solid Interfaces Giri, Ashutosh; Hopkins, Patrick E. Advanced Functional Materials https://doi.org/10.1002/adfm.201903857	journal	August 2019
Femtosecond laser generation of microbumps and nanojets on single and bilayer Cu/Ag thin films Naghilou, Aida; He, Miao; Schubert, Jasmin S. Physical Chemistry Chemical Physics, Vol. 21, Issue 22 https://doi.org/10.1039/c9cp02174d	journal	January 2019
Thin Ti adhesion layer breaks bottleneck to hot hole relaxation in Au films Zhou, Xin; Tokina, Marina V.; Tomko, John A. The Journal of Chemical Physics, Vol. 150, Issue 18 https://doi.org/10.1063/1.5096901	journal	May 2019
Spatially resolved thermoreflectance techniques for thermal conductivity measurements from the nanoscale to the mesoscale Olson, David H.; Braun, Jeffrey L.; Hopkins, Patrick E. Journal of Applied Physics, Vol. 126, Issue 15 https://doi.org/10.1063/1.5120310	journal	October 2019
Titanium contacts to graphene: process-induced variability in electronic and thermal transport Freedy, Keren M.; Giri, Ashutosh; Foley, Brian M. Nanotechnology, Vol. 29, Issue 14 https://doi.org/10.1088/1361-6528/aaaacd	journal	February 2018
Determining heat-transfer coefficients of solid objects by laser photothermal IR radiometry Aleksandrov, S. E.; Gavrilov, G. A.; Kapralov, A. A. Technical Physics Letters, Vol. 43, Issue 7 https://doi.org/10.1134/s106378501707015x	journal	July 2017
Titanium Contacts to Graphene: Process-Induced Variability in Electronic and Thermal Transport Freedy, Keren M.; Giri, Ashutosh; Foley, Brian M. arXiv https://doi.org/10.48550/arxiv.1712.00331	text	January 2017

Similar Records

Thermal flux limited electron Kapitza conductance in copper-niobium multilayers

Journal Article · Mon Mar 02 00:00:00 EST 2015 · Applied Physics Letters · OSTI ID:1183079

Cheaito, Ramez; Gaskins, John T.; Duda, John C.; +7 more

Interfacial thermal transport in spin caloritronic material systems

Journal Article · Thu Nov 11 00:00:00 EST 2021 · Physical Review Materials · OSTI ID:1183079

Angeles, Frank; Sun, Qiyang; Ortiz, Victor H.; +3 more

Development of SRF monolayer/multilayer thin film materials to increase the performance of SRF accelerating structures beyond bulk Nb

Thesis/Dissertation · Mon Sep 01 00:00:00 EDT 2014 · OSTI ID:1183079

VALENTE-FELICIANO, Anne-Marie

Related Subjects

75 CONDENSED MATTER PHYSICS
SUPERCONDUCTIVITY AND SUPERFLUIDITY

Title: Thermal flux limited electron Kapitza conductance in copper-niobium multilayers

Citation Formats

References (30)

Cited By (7)

Similar Records

Related Subjects