Electrocatalysts for carbon dioxide conversion

Masel, Richard I; Salehi-Khojin, Amin

Title: Electrocatalysts for carbon dioxide conversion

Patent · Tue Apr 21 00:00:00 EDT 2015

OSTI ID:1178252

Masel, Richard I; Salehi-Khojin, Amin

Electrocatalysts for carbon dioxide conversion include at least one catalytically active element with a particle size above 0.6 nm. The electrocatalysts can also include a Helper Catalyst. The catalysts can be used to increase the rate, modify the selectivity or lower the overpotential of electrochemical conversion of CO.sub.2. Chemical processes and devices using the catalysts also include processes to produce CO, HCO.sup.-, H.sub.2CO, (HCO.sub.2).sup.-, H.sub.2CO.sub.2, CH.sub.3OH, CH.sub.4, C.sub.2H.sub.4, CH.sub.3CH.sub.2OH, CH.sub.3COO.sup.-, CH.sub.3COOH, C.sub.2H.sub.6, (COOH).sub.2, or (COO.sup.-).sub.2, and a specific device, namely, a CO.sub.2 sensor.

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Research Organization:: Dioxide Materials, Inc., Champaign, IL (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: SC0004453

Assignee:: Dioxide Materials, Inc. (Champaign, IL)

Patent Number(s):: 9,012,345

Application Number:: 13/445,887

OSTI ID:: 1178252

Resource Relation:: Patent File Date: 2012 Apr 12

Country of Publication:: United States

Language:: English

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Method for preparing formic acid Saari, Kari; Tirronen, Esko; Vuori, Antti https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6429333 US Patent Document 6,429,333	patent	August 2002
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Method for production of formic acid Hladiy, Serhiy; Starchevskyy, Mykhaylo; Pazderskyy, Yuriy https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6713649 US Patent Document 6,713,649	patent	March 2004
Method for producing anhydrous formic acid Auer, Heinz; Bessling, Bernd; Hammer, Hans https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6841700 US Patent Document 6,841,700	patent	January 2005
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Felxible method for the common production of formic acid, a carboxylic acid having at least two carbon atoms, and/or the derivatives of the same Zehner, Peter; Pastre, Jörg; Stuer, Wolfram https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6992212 US Patent Document 6,992,212	patent	January 2006
Process for producing formic ester or methanol and synthesis catalyst therefor Fujimoto, Kaoru; Tsubaki, Noritatsu; Fujimoto, Kenichiro https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7081547 US Patent Document 7,081,547	patent	July 2006
Catalyst for preparing hydrocarbon Jun, Ki Won; Hwang, Jin-Soo; Lee, Kyu Wan https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7157404 US Patent Document 7,157,404	patent	January 2007
Material for a facility for the production of anhydrous formic acid Auer, Heinz; Bessling, Bernd; Hammer, Hans https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7241365 US Patent Document 7,241,365	patent	July 2007
Flexible method for the joint production of (i) formic acid, (ii) a carboxylic acid comprising at least two carbon atoms and/or the derivatives thereof, and (iii) a carboxylic acid anhydride Pastre, Jörg; Exner, Kai Michael; Stuer, Wolfram https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7253316 US Patent Document 7,253,316	patent	August 2007
Method and device for producing formates and the use thereof Adami, Christoph; Karl, Jorn; Hauk, Alexander https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7323593 US Patent Document 7,323,593	patent	January 2008
Method and device for producing formic acid formates and use of said formates Adami, Christoph; Karl, Jorn; Hauk, Alexander https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7351860 US Patent Document 7,351,860	patent	April 2008
Method for the production of formic acid Karl, Jorn; Hauk, Alexander https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7420088 US Patent Document 7,420,088	patent	September 2008
Method for producing methanol, dimethyl ether, derived synthetic hydrocarbons and their products from carbon dioxide and water (moisture) of the air as sole source material Olah, George A.; Aniszfeld, Robert https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7459590 US Patent Document 7,459,590	patent	December 2008
Process for reduction of carbon dioxide with organometallic complex Ogo, Seiji; Fukuzumi, Shuichi https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7479570 US Patent Document 7,479,570	patent	January 2009
Efficient and selective conversion of carbon dioxide to methanol, dimethyl ether and derived products Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7605293 US Patent Document 7,605,293	patent	October 2009
Efficient and selective chemical recycling of carbon dioxide to methanol, dimethyl ether and derived products Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7608743 US Patent Document 7,608,743	patent	October 2009
Production of sodium diformate Hauk, Alexander; Gropp, Stefan; Lenz, Robert W. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7612233 US Patent Document 7,612,233	patent	November 2009
Low contaminant formic acid fuel for direct liquid fuel cell Masel, Richard I.; Zhu, Yimin; Kahn, Zakia https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7618725 US Patent Document 7,618,725	patent	November 2009
Electrolysis of carbon dioxide in aqueous media to carbon monoxide and hydrogen for production of methanol Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7704369 US Patent Document 7,704,369	patent	April 2010
Conversion of carbon dioxide to organic products Bocarsly, Andrew B.; Cole, Emily Barton https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/8313634 US Patent Document 8,313,634	patent	November 2012
Reduction of carbon dioxide to carboxylic acids, glycols, and carboxylates Cole, Emily Barton; Teamey, Kyle; Bocarsly, Andrew B. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/8592633 US Patent Document 8,592,633	patent	November 2013
Electrophoresis process using ionic liquids Anderson, Norman G.; Braatz, James A. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20040031685 US Patent Document 10/218111; 20040031685	patent-application	February 2004
Electrocatalyst powders, methods for producing powder and devices fabricated from same Kodas, Toivo T.; Hampden-Smith, Mark J.; Atanassov, Plamen https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20040072683 US Patent Document 10/297528; 20040072683	patent-application	April 2004
Electrochemical carbon dioxide sensor Manoukian, Mourad; LaConti, Anthony B.; Tempelman, Linda A. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20060096871 US Patent Document 11/252090; 20060096871	patent-application	May 2006
Use of recirculated exhaust gas in a burner-based exhaust generation system for reduced fuel consumption and for cooling Burrahm, Robert Wayne; Ross, Michael Glenn; Webb, Cynthia Chaffin https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20060234174 US Patent Document 11/376961; 20060234174	patent-application	October 2006
Efficient and selective conversion of carbon dioxide to methanol, dimethyl ether and derived products Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20060235091 US Patent Document 11/402050; 20060235091	patent-application	October 2006
Process for reduction of carbon dioxide with organometallic complex Ogo, Seiji; Fukuzumi, Shuichi https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070036706 US Patent Document 10/572376; 20070036706	patent-application	February 2007
Electrochemical Cell for Production of Synthesis Gas Using Atmospheric Air and Water Hartvigsen, Joseph J.; Joshi, Ashok V.; Elangovan, S. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070045125 US Patent Document 11/467524; 20070045125	patent-application	March 2007
Electrochemical methods and processes for carbon dioxide recovery from alkaline solvents for carbon dioxide capture from air Lackner, Klaus; Wright, Allen https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070187247 US Patent Application 11/227660; 20070187247	patent-application	August 2007
Method for Producing Methanol, Dimethyl Ether, Derived Synthetic Hydrocarbons and Their Products from Carbon Dioxide and Water (Moisture) of the Air as Sole Source Material Olah, George A.; Aniszfeld, Robert https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20080039538 US Patent Document 11/780171; 20080039538	patent-application	February 2008
Catalytic Composition for the Insertion of Carbon Dioxide Into Organic Compounds Rodriguez, Mercedes Alvaro; Carbonell Llopis, Esther; Corma Canos, Avelino https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20080103040 US Patent Document 11/660995; 20080103040	patent-application	May 2008
Continuous Co-Current Electrochemical Reduction of Carbon Dioxide Oloman, Colin; Li, Hui https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20080223727 US Patent Document 12/090052; 20080223727	patent-application	September 2008
Electrolysis of Carbon Dioxide in Aqueous Media to Carbon Monoxide and Hydrogen for Production of Methanol Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20090014336 US Patent Document 12/171904; 20090014336	patent-application	January 2009
Carbon and fuel production from atmospheric CO₂ and H₂O by artificial photosynthesis and method of operation thereof Young, Edgar D. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20090016948 US Patent Document 12/214728; 20090016948	patent-application	January 2009
Methods of Sequestering CO₂ Constantz, Brent R.; Youngs, Andrew; Tuet, Philip Brian https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20090169452 US Patent Document 12/344019; 20090169452	patent-application	July 2009
Methods of Sequestering CO₂ Constantz, Brent R.; Youngs, Andrew; Tuet, Philip Brian https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100132556 US Patent Document 12/698802; 20100132556	patent-application	June 2010
Electrochemical Sensor Varney, Mark; Garrett, Micheal; Williams, Deryk https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100133120 US Patent Document 12/531093; 20100133120	patent-application	June 2010
Electrochemical Methods of Sequestering CO₂ Constantz, Brent R.; Youngs, Andrew; Tuet, Philip Brian https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100135865 US Patent Document 12/698483; 20100135865	patent-application	June 2010
Method for Conversion of Atmospheric Carbon Dioxide into Useful Materials Kaplan, Thomas Proger https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100137457 US Patent Document 12/494379; 20100137457	patent-application	June 2010
Conversion of Carbon Dioxide to Organic Products Bocarsly, Andrew B.; Cole, Emily Barton https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100187123 US Patent Document 12/696840; 20100187123	patent-application	July 2010
Electrolysis of Carbon Dioxide in Aqueous Media to Carbon Monoxide and Hydrogen for Production of Methanol Olah, George A.; Prakash, G. K. Surya https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100193370 US Patent Document 12/754952; 20100193370	patent-application	August 2010
Multi-gas microsensor assembly Manoukian, Mourad; LaConti, Anthony B.; Krebs, W. Michael https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20100276287 US Patent Document 12/660197; 20100276287	patent-application	November 2010
Purification of Carbon Dioxide from a Mixture of Gases Teamey, Kyle; Cole, Emily Barton; Sivasankar, Narayanappa https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110114501 US Patent Document 12/845995; 20110114501	patent-application	May 2011
Reducing Carbon Dioxide To Products Cole, Emily; Sivasankar, Narayanappa; Bocarsly, Andrew https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110114502 US Patent Application 12/846221; 20110114502	patent-application	May 2011
Electrochemical Production of Urea from NOx and Carbon Dioxide Sivasankar, Narayanappa; Cole, Emily; Teamey, Kyle https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110114503 US Patent Document 12/875227; 20110114503	patent-application	May 2011
Electrochemical Production of Synthesis Gas from Carbon Dioxide Sivasankar, Narayanappa; Cole, Emily Barton; Teamey, Kyle https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110114504 US Patent Document 12/846002; 20110114504	patent-application	May 2011
Heterocycle Catalyzed Electrochemical Process Cole, Emily Barton; Bocarsly, Andrew https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110226632 US Patent Document 12/846011; 20110226632	patent-application	September 2011
Novel catalyst mixtures Masel, Richard https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20110237830 US Patent Application 12/830338; 20110237830	patent-application	September 2011
Novel Catalyst Mixtures Masel, Richard https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20120308903 US Patent Application 13/174365; 20120308903	patent-application	December 2012

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