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U.S. Department of Energy
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  1. Options, Initial Design Requirements, Estimated Costs, Reactor Commitments, and Potential Uses of a Graphite Leadout Type Experiment Supporting Various Commercial HTR Vendors

    Multiple commercial High Temperature Reactor (HTR) vendors and nuclear graphite suppliers would benefit by collaborating on a new irradiation capsule(s) that would include graphite grades not included within the AGC Experiment. This new irradiation capsule(s) would provide data to answer vendor graphite licensing issues. Rather than spending money (and especially) time in designing separate irradiation capsules for each designer, the capsule(s) would be used for multiple graphite and composite designs to maximize efficiency and promote multiple HTR designs. However, the primary motivation for assisting vendors with this new irradiation capsule(s) is lack of availability in the existing Material Test Reactors (MTRs). Cost reduction is a secondary goal. A common, collaborative, capsule design can be achieved for graphite and composites due to the similarity of different grades. Irradiation, disassembly, shipping, and PIE costs would be cost-shared by all users. It is anticipated that interest would extend across all DOE campaigns (micro-Rx, SMR, GCR, MSR, etc.) due to the similar requirements for all graphite grades.

  2. Qualifying nuclear graphite components using ASME guidelines

    Qualifying nuclear graphite components using ASME guidelines, including Semi-probabilistic, probabilistic, and deterministic approaches to design, theory of methods, pre-assessment analysis inputs, post assessment analysis outputs, simplified assessment, full assessment, and application.

  3. ASME Irradiation Model

    ASME Irradiation Model: How to deal with irradiation data in ASME code rules. Includes discussion on challenges to nuclear graphite, such as lack of sufficient irradiation data to qualify graphite for nuclear application for all grades and temperatures, variety of grades, and time/room in available MTRs to get all the required data. Discussion of Irradiation behavior, Leveraging data generated by GIF countries the past 20 years, Dimensional Change Theory, behavior, analysis, turnaround, and data. Future discussions include Arrhenius approach to predict turnaround behavior for the ASME MDS requirements for all nuclear graphite.

  4. SEMI-EMPIRICAL MODELING OF IRRADIATION-INDUCED DIMENSIONAL CHANGE IN H-451 NUCLEAR GRAPHITE

    Nuclear graphite has been used as a moderator material in nuclear reactor designs dating back to the first reactor to reach criticality, Chicago Pile 1, in 1942. In addition, it is anticipated to be used in the conceptual Generation four (GenIV) Molten-salt reactors (MSRs) and the High-temperature gas-cooled reactors (HTRs). The macroscopic dimensional change observed in irradiated nuclear graphite is a property change of significant importance. Largely, volumetric change provides valuable insight into the in-service lifetime of graphite components used in nuclear reactors. The dimensional change behavior varies amongst each grade of nuclear graphite due to processing techniques and the resulting microstructure. In this work, historic data for nuclear graphite H-451 is revisited. A semi-empirical methodology is proposed to describe the dimensional change behavior as a function of temperature for nuclear graphite H-451. The turnaround dose, or when there is a reversal of the dimensional change from contraction to expansion, is proposed to be a thermally activated process and thus can be described by an Arrhenius model. On the atomic scale, H-451 is sp2-bonded carbon atoms with some degree of disorder regardless of orientation. Towards that end, the activation energy is assumed to be a constant irrespective of orientation.

  5. Accurate Dosimetry for Future Advanced Reactor Deployment and Operation

    Accurate Dosimetry for Future Advanced Reactor Deployment and Operation from a customer's perspective. The main discussion points will be why we should be interested in this topic of nuclear renaissance, practical examples, and Dosimetry's role in advance reactor operations.

  6. An In Situ Transmission Electron Microscopy Study on the Synergistic Effects of Au-ion Irradiation and High Temperature on Nuclear Graphite Microstructure

    The combined effect of high-temperature and heavy-ion irradiation on Mrozowski cracks (MC) and nuclear graphite crystallographic dimensions have been studied using in situ heating and in situ ion-irradiation in the transmission electron microscope (TEM). Electron transparent lamella of nuclear graphite, IG-110, was irradiated, using a 2.8 MeV Au beam at an ion flux of 3.991 x 1010 ion cm-2 s-1 for 70 minutes at 800 oC. Upon high-temperature irradiation, Mrozowski crack closure was studied quantitatively. The analysis showed linear, positive expansion of nuclear graphite which is significantly different from the dimensional changes previously reported for low-dose neutron irradiation of nuclear graphite in which the material undergoes negative to positive expansion via a turnaround radiation dose. The trend of the thermal expansion coefficient (CTE) of pristine IG-110 in this study is consistent with previous reports in the 100-800 oC temperature region in which the dimensional change ranges from negative to positive values.

  7. GRAPHITE–MOLTEN SALT CONSIDERATIONS FOR COMPONENTS IN NUCLEAR APPLICATIONS

    The new High Temperature Reactor (HTR) designs being considered for future Gen IV nuclear reactor deployment include designs utilizing molten salt as the primary coolant. These molten-salt cooled, graphite core designs pose new material compatibility challenges that are not considered within the gas-cooled HTR designs that have been previously built and operated. While the Molten Salt Reactor Experiment (MSRE) demonstrated that the molten salt can be considered chemically inert to graphite the novel physical and thermal interactions that the molten salt poses may be just as impactful as the chemical reactivity. Specifically, molten salt intrusion into the open pore structure of nuclear graphite grades can provide additional internal stresses within the microstructure exacerbating the stress buildup from irradiation induced dimensional change. Additionally, designs using a molten salt containing liquid fuel could provide “hot spots” within graphite structural components causing local thermal stresses. Abrasion and erosion concerns are magnified with molten salt due to the extremely high density of the salts (some have higher densities than the structural graphite components). Finally, the graphite-graphite and fuel pebble-graphite tribological behavior are distinctly difference within the molten salt from the inert gas environments and must be investigated. These topics and others are currently under investigation within the DOE Advanced Reactor Technologies (ART) graphite program and will be discussed in depth.

  8. Real-Time Observation of Nanoscale Kink Band Mediated Plasticity in Ion-Irradiated Graphite: An In Situ TEM Study

    Graphite IG-110 is a synthetic polycrystalline material used as a neutron moderator in reactors. Graphite is inherently brittle and is known to exhibit a further increase in brittleness due to radiation damage at room temperature. To understand the irradiation effects on pre-existing defects and their overall influence on external load, micropillar compression tests were performed using in situ nanoindentation in the Transmission Electron Microscopy (TEM) for both pristine and ion-irradiated samples. While pristine specimens showed brittle and subsequent catastrophic failure, the 2.8 MeV Au2+ ion (fluence of 4.378 × 1014 cm-2) irradiated specimens sustained extensive plasticity at room temperature without failure. In situ TEM characterization showed nucleation of nanoscale kink band structures at numerous sites, where the localized plasticity appeared to close the defects and cracks while allowing large average strain. We propose that compressive mechanical stress due to dimensional change during ion irradiation transforms buckled basal layers in graphite into kink bands. The externally applied load during the micropillar tests proliferates the nucleation and motion of kink bands to accommodate the large plastic strain. The inherent non-uniformity of graphite microstructure promotes such strain localization, making kink bands the predominant mechanism behind unprecedented toughness in an otherwise brittle material.

  9. Status on Development of Graphite Analytical Tool (GAT)

    The DOE-ART Graphite R&D program has been generating significant amounts of irradiated and unirradiated graphite data since 2006 when the program was part of the DOE NGNP (Next Generation Nuclear Plant) Project. This data includes critical irradiation creep and irradiated material property changes from the Advanced Graphite Creep (AGR) experiment as well as significant amounts of data on unirradiated material property values on several current nuclear graphite grades (Baseline program). Previously, Idaho National Laboratory has developed an internal analysis tool to assist with analysis of the unirradiated and irradiated data. The Graphite Analytical Tool (GAT) is intended to provide easy access to the graphite data in the form of comparing unirradiated and irradiated material property changes, comparison of material property differences between various nuclear graphite grades, and illustrate trends within the irradiated and unirradiated data generated within the DOE-ART Graphite R&D program. This report summarizes the progress to-date on the development of this analytical tool.

  10. Advanced Reactors Development in USA

    Small and micro-reactor advanced reactor development in the USA. Advanced Reactor programs, nuclear renaissance, and INL as a test bed facility. These slides are for presentations in general on the past, INL and nuclear engineering worldwide, GEN IV reactor designs, SMRs and micro Rx designs, multiple commercial designs, and what INL as a test bed means and who uses this to their advantage.


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