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  1. A Comparative Study of Single-pulse and Double-pulse Laser-Induced Breakdown Spectroscopy with Uranium-containing Samples

    Laser-induced breakdown spectroscopy (LIBS) holds potential advantages in special nuclear material (SNM) sensing and nuclear forensics which require rapid analysis, minimal sample preparation and stand-off distance capability. SNM, such as U, however, result in crowded emission spectra with LIBS, and characteristic emission lines are challenging to discern. It is well-known that double-pulse LIBS (DPLIBS) improves the signal intensity for analytes over conventional single-pulse LIBS (SPLIBS). This study investigates U signal in a glass matrix using DPLIBS and compares to signal features obtained using SPLIBS. DPLIBS involves sequential firing of 1.06 µm Nd:YAG pre-pulse and 10.6 µm TEA CO2 heating pulsemore » in near collinear geometry. Optimization of experimental parameters including inter-pulse delay and energy follows identification of characteristic lines and signals for bulk analyte Ca and minor constituent analyte U for both DPLIBS and SPLIBS. Spatial and temporal coupling of the two pulses in the proposed DPLIBS technique yields improvements in analytical merits with negligible further damage to the sample compared to SPLIBS. Subsequently, the study discusses optimum plasma emission conditions of U lines and relative figures of merit in both SPLIBS and DPLIBS. Investigation into plasma characteristics also addresses plausible mechanisms related to observed U analyte signal variation between SPLIBS and DPLIBS.« less
  2. Low energy helium ion irradiation induced nanostructure formation on tungsten surface

  3. Collimation of laser-produced plasmas using axial magnetic field

    We investigated the expansion dynamics of laser-produced plasmas expanding into an axial magnetic field. Plasmas were generated by focusing 1.064 µm Nd:YAG laser pulses onto a planar tin target in vacuum and allowed to expand into a 0.5 T magnetic-filed where field lines were aligned along the plume expansion direction. Gated images employing intensified CCD showed focusing of the plasma plume, which were also compared with results obtained using particle-in-cell modelling methods. The estimated density and temperature of the plasma plumes employing emission spectroscopy revealed significant changes in the presence and absence of the 0.5T magnetic field. In the presencemore » of the field, the electron temperature is increased with distance from the target, while the density showed opposite effects.« less
  4. Heavy ion irradiation on ultrafine-and nanocrystalline-grained tungsten: effect of 3 MeV Si Cu and W ions.

    Abstract not provided.
  5. Role of carbon impurities on the surface morphology evolution of tungsten under high dose helium ion irradiation

  6. Heat loads to divertor nearby components from secondary radiation evolved during plasma instabilities

    A fundamental issue in tokamak operation related to power exhaust during plasma instabilities is the understanding of heat and particle transport from the core plasma into the scrape-off layer and to plasma-facing materials. During abnormal and disruptive operation in tokamaks, radiation transport processes play a critical role in divertor/edge-generated plasma dynamics and are very important in determining overall lifetimes of the divertor and nearby components. This is equivalent to or greater than the effect of the direct impact of escaped core plasma on the divertor plate. We have developed and implemented comprehensive enhanced physical and numerical models in the upgradedmore » HEIGHTS package for simulating detailed photon and particle transport in the evolved edge plasma during various instabilities. The paper describes details of a newly developed 3D Monte Carlo radiation transport model, including optimization methods of generated plasma opacities in the full range of expected photon spectra. Response of the ITER divertor's nearby surfaces due to radiation from the divertor-developed plasma was simulated by using actual full 3D reactor design and magnetic configurations. We analyzed in detail the radiation emission spectra and compared the emission of both carbon and tungsten as divertor plate materials. The integrated 3D simulation predicted unexpectedly high damage risk to the open stainless steel legs of the dome structure in the current ITER design from the intense radiation during a disruption on the tungsten divertor plate.« less
  7. Characterization of ultrafast laser-ablation plasma plumes at various Ar ambient pressures

    Expansion dynamics and internal plume structures of fs laser ablated brass plasma in Ar at various pressure levels ranging from vacuum to atmospheric were studied using multitude of diagnostic tools including time resolved and time integrated 2-dimensional imaging, optical time of flight measurements and visible emission spectroscopy. Temporal evolution of excited Cu and Zn species in the plume were imaged using band pass interference filters and compared its hydrodynamic expansion features with spectrally integrated images of the plume. 2D imaging coupled with monochromatic line selection showed several interesting features at various pressure levels which include velocity differences among the plumemore » species, emission intensity distribution, plasma temperature, electron density etc. Plume confinement, enhanced signal intensity, and dual peak structures in time-of-flight profiles were observed at intermediate pressure range of ~10 Torr. Optimum signal to background ratio was also observed in this pressure range. As a result, possible mechanisms for observed changes in plume shape, optical emission intensity and dual peak structures in time-of-flight profiles were discussed.« less
  8. Fusion Energy Sciences Exascale Requirements Review. An Office of Science review sponsored jointly by Advanced Scientific Computing Research and Fusion Energy Sciences, January 27-29, 2016, Gaithersburg, Maryland

    The additional computing power offered by the planned exascale facilities could be transformational across the spectrum of plasma and fusion research — provided that the new architectures can be efficiently applied to our problem space. The collaboration that will be required to succeed should be viewed as an opportunity to identify and exploit cross-disciplinary synergies. To assess the opportunities and requirements as part of the development of an overall strategy for computing in the exascale era, the Exascale Requirements Review meeting of the Fusion Energy Sciences (FES) community was convened January 27–29, 2016, with participation from a broad range ofmore » fusion and plasma scientists, specialists in applied mathematics and computer science, and representatives from the U.S. Department of Energy (DOE) and its major computing facilities. This report is a summary of that meeting and the preparatory activities for it and includes a wealth of detail to support the findings. Technical opportunities, requirements, and challenges are detailed in this report (and in the recent report on the Workshop on Integrated Simulation). Science applications are described, along with mathematical and computational enabling technologies. Also see http://exascaleage.org/fes/ for more information.« less
  9. Gas dynamic effects on formation of carbon dimers in laser-produced plasmas

    We investigated the effect of helium and nitrogen pressures on the dynamics of molecular species formation during laser ablation of carbon. For producing plasmas, planar carbon targets were irradiated with 1064 nm, 6 ns pulses from an Nd:yttrium aluminum garnet laser. The emission from excited C{sub 2} and CN molecules was studied using space resolved optical time-of-flight emission spectroscopy and spectrally resolved fast imaging. The intensity oscillations in C{sub 2} and CN monochromatic fast imaging and their emission space-time contours suggest that recombination is the major mechanism of C{sub 2} formation within the laser ablation carbon plumes in the presencemore » of ambient gas.« less
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