Neutron diffraction measurement of residual stresses, dislocation density and texture in Zr-bonded U-10Mo “mini” fuel foils and plates

Brown, Donald William; Okuniewski, Maria A.; Sisneros, Thomas A.; Clausen, Bjorn; Moore, Glenn A.; Balogh, Levente

doi:10.1016/j.jnucmat.2016.09.022

Title: Neutron diffraction measurement of residual stresses, dislocation density and texture in Zr-bonded U-10Mo “mini” fuel foils and plates

Journal Article · Thu Dec 01 00:00:00 EST 2016 · Journal of Nuclear Materials

DOI:https://doi.org/10.1016/j.jnucmat.2016.09.022· OSTI ID:1329601

Brown, Donald William ^[1]; Okuniewski, Maria A. ^[2]; Sisneros, Thomas A. ^[1]; Clausen, Bjorn ^[1]; Moore, Glenn A. ^[3]; Balogh, Levente ^[4]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Purdue Univ., West Lafayette, IN (United States); Idaho National Lab. (INL), Idaho Falls, ID (United States)
Idaho National Lab. (INL), Idaho Falls, ID (United States)
Queens Univ., Kingston, ON (Canada)

Here, Al clad U-10Mo fuel plates are being considered for conversion of several research reactors from high-enriched to low-enriched U fuel. Neutron diffraction measurements of the textures, residual phase stresses, and dislocation densities in the individual phases of the mini-foils throughout several processing steps and following hot-isostatic pressing to the Al cladding, have been completed. Recovery and recrystallization of the bare U-10Mo fuel foil, as indicated by the dislocation density and texture, are observed depending on the state of the material prior to annealing and the duration and temperature of the annealing process. In general, the cladding procedure significantly reduces the dislocation density, but the final state of the clad plate, both texture and dislocation density, depends strongly on the final processing step of the fuel foil. In contrast, the residual stress state of the final plate is dominated by the thermal expansion mismatch of the constituent materials.

View Accepted Manuscript (DOE)

View Accepted Manuscript (Publisher)

Cite

Export

Save

Research Organization:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation

Grant/Contract Number:: AC52-06NA25396; AC07-05ID14517

OSTI ID:: 1329601

Alternate ID(s):: OSTI ID: 1396816

Report Number(s):: LA-UR-16-25037

Journal Information:: Journal of Nuclear Materials, Vol. 482, Issue C; ISSN 0022-3115

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 9 works

Citation information provided by
Web of Science

References (32)

Development of very-high-density low-enriched-uranium fuels Snelgrove, J. L.; Hofman, G. L.; Meyer, M. K. Nuclear Engineering and Design, Vol. 178, Issue 1 https://doi.org/10.1016/S0029-5493(97)00217-3	journal	December 1997
Fabrication of Monolithic RERTR Fuels by Hot Isostatic Pressing Jue, Jan-Fong; Park, Blair H.; Clark, Curtis R. Nuclear Technology, Vol. 172, Issue 2 https://doi.org/10.13182/NT10-A10905	journal	November 2010
Microstructural analysis of as-processed U–10wt.%Mo monolithic fuel plate in AA6061 matrix with Zr diffusion barrier Perez, E.; Yao, B.; Keiser, D. D. Journal of Nuclear Materials, Vol. 402, Issue 1 https://doi.org/10.1016/j.jnucmat.2010.04.016	journal	July 2010
Role of Si on the Diffusional Interactions Between U-Mo and Al-Si Alloys at 823 K (550 °C) Perez, Emmanuel; Sohn, Yong-Ho; Keiser, Dennis D. Metallurgical and Materials Transactions A, Vol. 44, Issue 1 https://doi.org/10.1007/s11661-012-1368-1	journal	August 2012
UMo/Al nuclear fuel plate behavior under thermal treatment (425-550°C) Palancher, H.; Bonnin, A.; Colin, C. V. Powder Diffraction, Vol. 28, Issue S2 https://doi.org/10.1017/S0885715613000894	journal	September 2013
Modeling thermal and stress behavior of the fuel–clad interface in monolithic fuel mini-plates Miller, Gregory K.; Burkes, Douglas E.; Wachs, Daniel M. Materials & Design, Vol. 31, Issue 7 https://doi.org/10.1016/j.matdes.2010.02.016	journal	August 2010
Assessment of residual stresses on U10Mo alloy based monolithic mini-plates during Hot Isostatic Pressing Ozaltun, Hakan; Herman Shen, M. -H.; Medvedev, Pavel Journal of Nuclear Materials, Vol. 419, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2011.08.029	journal	December 2011
High energy X-ray diffraction measurement of residual stresses in a monolithic aluminum clad uranium–10wt% molybdenum fuel plate assembly Brown, D. W.; Okuniewski, M. A.; Almer, J. D. Journal of Nuclear Materials, Vol. 441, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2013.05.064	journal	October 2013
Neutron diffraction measurement of residual stresses in Al-clad U–10Mo fuel plates Brown, D. W.; Okuniewski, M. A.; Clausen, B. Journal of Nuclear Materials, Vol. 474 https://doi.org/10.1016/j.jnucmat.2016.02.012	journal	June 2016
Development of the hot isostatic press manufacturing process for monolithic nuclear fuel Crapps, Justin; Clarke, Kester; Katz, Joel Nuclear Engineering and Design, Vol. 254 https://doi.org/10.1016/j.nucengdes.2012.09.002	journal	January 2013
SMARTS - a spectrometer for strain measurement in engineering materials Bourke, M. A. M.; Dunand, D. C.; Ustundag, E. Applied Physics A: Materials Science & Processing, Vol. 74, Issue 0 https://doi.org/10.1007/s003390201747	journal	December 2002
Neutron Strain measurement Krawitz, A. D. Materials Science and Technology, Vol. 27, Issue 3 https://doi.org/10.1179/1743284710Y.0000000029	journal	March 2011
Critical comparison of two independent measurements of residual stress in an electron-beam welded uranium cylinder: Neutron diffraction and the contour method Brown, D. W.; Holden, T. M.; Clausen, B. Acta Materialia, Vol. 59, Issue 3 https://doi.org/10.1016/j.actamat.2010.09.022	journal	February 2011
Experimental error caused by sample displacement in time-of-flight neutron diffractometry Wang, X. -L.; Wang, Y. D.; Richardson, J. W. Journal of Applied Crystallography, Vol. 35, Issue 5 https://doi.org/10.1107/S0021889802009202	journal	September 2002
Rietveld refinement with spallation neutron powder diffraction data Von Dreele, R. B.; Jorgensen, J. D.; Windsor, C. G. Journal of Applied Crystallography, Vol. 15, Issue 6 https://doi.org/10.1107/S0021889882012722	journal	December 1982
Large Strain Deformation in Uranium 6 Wt Pct Niobium Tupper, Catherine N.; Brown, Don W.; Field, Robert D. Metallurgical and Materials Transactions A, Vol. 43, Issue 2 https://doi.org/10.1007/s11661-011-0931-5	journal	November 2011
Quantitative texture analysis by Rietveld refinement Von Dreele, R. B. Journal of Applied Crystallography, Vol. 30, Issue 4 https://doi.org/10.1107/S0021889897005918	journal	August 1997
Elastic properties of rolled uranium–10wt.% molybdenum nuclear fuel foils Brown, D. W.; Alexander, D. J.; Clarke, K. D. Scripta Materialia, Vol. 69, Issue 9 https://doi.org/10.1016/j.scriptamat.2013.07.025	journal	November 2013
Residual stresses in annealed zircaloy MacEwen, S. R.; Tome, C.; Faber, J. Acta Metallurgica, Vol. 37, Issue 3 https://doi.org/10.1016/0001-6160(89)90025-4	journal	March 1989
Development of intergranular thermal residual stresses in beryllium during cooling from processing temperatures Brown, D. W.; Sisneros, T. A.; Clausen, B. Acta Materialia, Vol. 57, Issue 4 https://doi.org/10.1016/j.actamat.2008.09.044	journal	February 2009
Lattice Parameters, Thermal Expansions, and Grüneisen Coefficients of Zirconium, 4.2 to 1130°K Goldak, J.; Lloyd, L. T.; Barrett, C. S. Physical Review, Vol. 144, Issue 2 https://doi.org/10.1103/PhysRev.144.478	journal	April 1966
Coefficients of Thermal Expansion for Zirconium Russell, R. B. JOM, Vol. 6, Issue 9 https://doi.org/10.1007/BF03398344	journal	September 1954
X-ray line broadening from filed aluminium and wolfram Williamson, G. K.; Hall, W. H. Acta Metallurgica, Vol. 1, Issue 1 https://doi.org/10.1016/0001-6160(53)90006-6	journal	January 1953
The separation of particle size and strain by the method of the variance Aqua, E. N. Acta Crystallographica, Vol. 20, Issue 4 https://doi.org/10.1107/S0365110X66001245	journal	April 1966
The determination of density and distribution of dislocations in deformed single crystals from broadened X-ray diffraction profiles Wilkens, M. Physica Status Solidi (a), Vol. 2, Issue 2 https://doi.org/10.1002/pssa.19700020224	journal	June 1970
Notes on the order-of-reflection dependence of microstrain broadening Leineweber, A.; Mittemeijer, E. J. Journal of Applied Crystallography, Vol. 43, Issue 5 https://doi.org/10.1107/S0021889810030451	journal	September 2010
Separation of particle size and lattice strain in integral breadth measurements Halder, N. C.; Wagner, C. N. J. Acta Crystallographica, Vol. 20, Issue 2 https://doi.org/10.1107/S0365110X66000628	journal	February 1966
The determination of crystallite-size and lattice-strain parameters in conjunction with the profile-refinement method for the determination of crystal structures de Keijser, Th.; Mittemeijer, E. J.; Rozendaal, H. C. F. Journal of Applied Crystallography, Vol. 16, Issue 3 https://doi.org/10.1107/S0021889883010493	journal	June 1983
The diffraction of X rays by distorted crystal aggregates - I Stokes, A. R.; Wilson, A. J. C. Proceedings of the Physical Society, Vol. 56, Issue 3 https://doi.org/10.1088/0959-5309/56/3/303	journal	May 1944
Correlation between strength and microstructure of ball-milled Al–Mg alloys determined by X-ray diffraction Ribárik, G.; Gubicza, J.; Ungár, T. Materials Science and Engineering: A, Vol. 387-389 https://doi.org/10.1016/j.msea.2004.01.089	journal	December 2004
Crystallite size distribution and dislocation structure determined by diffraction profile analysis: principles and practical application to cubic and hexagonal crystals Ungár, T.; Gubicza, J.; Ribárik, G. Journal of Applied Crystallography, Vol. 34, Issue 3 https://doi.org/10.1107/S0021889801003715	journal	May 2001
The influence of multiaxial stress states, stress gradients and elastic anisotropy on the evaluation of (Residual) stresses by X-rays Dölle, H. Journal of Applied Crystallography, Vol. 12, Issue 6 https://doi.org/10.1107/S0021889879013169	journal	December 1979

Cited By (2)

Interface formation and bonding mechanisms of hot-rolled stainless steel clad plate Liu, B. X.; An, Q.; Yin, F. X. Journal of Materials Science, Vol. 54, Issue 17 https://doi.org/10.1007/s10853-019-03581-x	journal	April 2019
Texture Evolution in U-10Mo Nuclear Fuel Foils during Plasma Spray Coating with Zr Takajo, Shigehiro; Hollis, Kendall; Cummins, Dustin Quantum Beam Science, Vol. 2, Issue 2 https://doi.org/10.3390/qubs2020012	journal	May 2018

Similar Records

Neutron Diffraction Measurement of Residual Stresses, Dislocation Density and Texture in Zr-bonded U-10Mo ''Mini'' Fuel Foils and Plates

Technical Report · Thu Aug 07 00:00:00 EDT 2014 · OSTI ID:1329601

Brown, Donald W.; Okuniewski, M. A.; Sisneros, Thomas A.; +3 more

Dissolution Flowsheet for U-10Mo Scrap Generated from the Fabrication of High Performance Research Reactor Fuel

Technical Report · Sun Sep 01 00:00:00 EDT 2019 · OSTI ID:1329601

Daniel, W. E.; Rudisill, T. S.; O'Rourke, P. E.

Annealing of (DU-10Mo)-Zr Co-Rolled Foils

Technical Report · Fri Jan 20 00:00:00 EST 2017 · OSTI ID:1329601

Pacheco, Robin Montoya; Alexander, David John; Mccabe, Rodney James; +5 more

Related Subjects

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS

Title: Neutron diffraction measurement of residual stresses, dislocation density and texture in Zr-bonded U-10Mo “mini” fuel foils and plates

Citation Formats

References (32)

Cited By (2)

Similar Records

Related Subjects