Short- and long-range magnetic order in LaMnAsO

McGuire, Michael A.; Garlea, Vasile Ovidiu

doi:10.1103/PhysRevB.93.054404

Title: Short- and long-range magnetic order in LaMnAsO

Journal Article · Tue Feb 02 00:00:00 EST 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.93.054404· OSTI ID:1237161

McGuire, Michael A. ^[1]; Garlea, Vasile Ovidiu ^[1]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

The magnetic properties of the layered oxypnictide LaMnAsO have been revisited using neutron scattering and magnetization measurements. The present measurements identify the Néel temperature T_N = 360(1) K. Below T_N the critical exponent describing the magnetic order parameter is β=0.33–0.35 , consistent with a three-dimensional Heisenberg model. Above this temperature, diffuse magnetic scattering indicative of short-range magnetic order is observed, and this scattering persists up to T_SRO = 650(10) K. Morevoer, the magnetic susceptibility shows a weak anomaly at T_SRO and no anomaly at T_N. Analysis of the diffuse scattering data using a reverse Monte Carlo algorithm indicates that above T_N nearly two-dimensional, short-range magnetic order is present with a correlation length of 9.3(3) Å within the Mn layers at 400 K. The inelastic scattering data reveal a spin gap of 3.5 meV in the long-range ordered state, and strong, low-energy (quasielastic) magnetic excitations emerging in the short-range ordered state. When we compared it with other related compounds correlates the distortion of the Mn coordination tetrahedra to the sign of the magnetic exchange along the layer-stacking direction, and suggests that short-range order above T_N is a common feature in the magnetic behavior of layered Mn-based pnictides and oxypnictides.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1237161

Alternate ID(s):: OSTI ID: 1236727

Journal Information:: Physical Review B, Vol. 93, Issue 5; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 25 works

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