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Title: Communication: X-ray coherent diffractive imaging by immersion in nanodroplets

Journal Article · · Structural Dynamics
DOI:https://doi.org/10.1063/1.4933297· OSTI ID:1230062
 [1];  [1];  [1];  [2];  [3];  [4];  [5];  [3];  [6];  [7];  [4];  [5];  [8];  [1];  [9];  [2];  [10];  [4];  [11];  [6] more »;  [4];  [6];  [12];  [6];  [1] « less
  1. Univ. of Southern California, Los Angeles, CA (United States)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Univ. of California Berkeley, Berkeley, CA (United States)
  3. SLAC National Accelerator Lab., Menlo Park, CA (United States)
  4. Max-Planck-Institut fur Kernphysik, Heidelberg (Germany); Max Planck Advanced Study Group at the Center for Free-Electron Laser Science (CFEL), Hamburg (Germany)
  5. Max-Planck-Institut fur Kernphysik, Heidelberg (Germany); Max Planck Advanced Study Group at the Center for Free-Electron Laser Science (CFEL), Hamburg (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)
  6. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  7. Max-Planck-Institut fur extraterrestrische Physik, Garching (Germany)
  8. Max Planck Advanced Study Group at the Center for Free-Electron Laser Science (CFEL), Hamburg (Germany); Max-Planck-Institut fur Medizinische Forschung, Heidelberg (Germany)
  9. PNSensor GmbH, Munich (Germany)
  10. Max Planck Advanced Study Group at the Center for Free-Electron Laser Science (CFEL), Hamburg (Germany); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany); Max-Planck-Institut fur Medizinische Forschung, Heidelberg (Germany); Kansas State Univ., Manhattan, KS (United States)
  11. Max-Planck-Institut fur Kernphysik, Heidelberg (Germany); Max Planck Advanced Study Group at the Center for Free-Electron Laser Science (CFEL), Hamburg (Germany); Kansas State Univ., Manhattan, KS (United States)
  12. SLAC National Accelerator Lab., Menlo Park, CA (United States); Argonne National Lab. (ANL), Argonne, IL (United States); Northwestern Univ., Evanston, IL (United States)

Lensless x-ray microscopy requires the recovery of the phase of the radiation scattered from a specimen. Here, we demonstrate a de novo phase retrieval technique by encapsulating an object in a superfluid helium nanodroplet, which provides both a physical support and an approximate scattering phase for the iterative image reconstruction. The technique is robust, fast-converging, and yields the complex density of the immersed object. As a result, images of xenon clusters embedded in superfluid helium droplets reveal transient configurations of quantum vortices in this fragile system.

Research Organization:
SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC03-76SF00515; AC02-05CH11231
OSTI ID:
1230062
Alternate ID(s):
OSTI ID: 1407303
Journal Information:
Structural Dynamics, Vol. 2, Issue 5; ISSN 2329-7778
Publisher:
American Crystallographic Association/AIPCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 30 works
Citation information provided by
Web of Science

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Cited By (12)

Kinematics of the Doped Quantum Vortices in Superfluid Helium Droplets journal February 2018
Long-lasting field-free alignment of large molecules inside helium nanodroplets journal January 2019
Infrared spectroscopy in superfluid helium droplets journal December 2018
Shapes of rotating superfluid helium nanodroplets journal February 2017
Three-Dimensional Shapes of Spinning Helium Nanodroplets journal December 2018
Refinement for single-nanoparticle structure determination from low-quality single-shot coherent diffraction data journal January 2020
CAMP@FLASH: an end-station for imaging, electron- and ion-spectroscopy, and pump–probe experiments at the FLASH free-electron laser text January 2018
The LAMP instrument at the Linac Coherent Light Source free-electron laser text January 2018
The LAMP instrument at the Linac Coherent Light Source free-electron laser journal March 2018
Three-dimensional shapes of spinning helium nanodroplets text January 2018
CAMP@FLASH: an end-station for imaging, electron- and ion-spectroscopy, and pump–probe experiments at the FLASH free-electron laser text January 2018
CAMP@FLASH: an end-station for imaging, electron- and ion-spectroscopy, and pump–probe experiments at the FLASH free-electron laser journal August 2018