skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Spectroscopic study of Gd nanostructures quantum confined in Fe corrals

Journal Article · · Scientific Reports
DOI:https://doi.org/10.1038/srep12092· OSTI ID:1224979
 [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [1];  [2];  [1];  [1]
  1. Nanjing Univ., Nanjing (People's Republic of China)
  2. Argonne National Lab. (ANL), Argonne, IL (United States)

Low dimensional nanostructures have attracted attention due to their rich physical properties and potential applications. The essential factor for their functionality is their electronic properties, which can be modified by quantum confinement. Here the electronic states of Gd atom trapped in open Fe corrals on Ag(111) were studied via scanning tunneling spectroscopy. A single spectroscopic peak above the Fermi level is observed after Gd adatoms are trapped inside Fe corrals, while two peaks appear in empty corrals. The single peak position is close to the higher energy peak of the empty corrals. These findings, attributed to quantum confinement of the corrals and Gd structures trapped inside, are supported by tight-binding calculations. As a result, this demonstrates and provides insights into atom trapping in open corrals of various diameters, giving an alternative approach to modify the properties of nano-objects.

Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC02-06CH11357
OSTI ID:
1224979
Journal Information:
Scientific Reports, Vol. 5; ISSN 2045-2322
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 3 works
Citation information provided by
Web of Science

References (39)

Imaging standing waves in a two-dimensional electron gas journal June 1993
Confinement of Electrons to Quantum Corrals on a Metal Surface journal October 1993
Quantum mirages formed by coherent projection of electronic structure journal February 2000
Development of One-Dimensional Band Structure in Artificial Gold Chains journal August 2002
Designer Dirac fermions and topological phases in molecular graphene journal March 2012
Oscillatory Magnetic Anisotropy Originating from Quantum Well States in Fe Films journal May 2009
Spin-Dependent Quantum Interference Within a Single Magnetic Nanostructure journal February 2010
Realizing All-Spin-Based Logic Operations Atom by Atom journal May 2011
Bistability in Atomic-Scale Antiferromagnets journal January 2012
Creating an Artificial Two-Dimensional Skyrmion Crystal by Nanopatterning journal April 2013
Reversible electromechanical characteristics of carbon nanotubes underlocal-probe manipulation journal June 2000
Strength and Breaking Mechanism of Multiwalled Carbon Nanotubes Under Tensile Load journal January 2000
Measurement of the Elastic Properties and Intrinsic Strength of Monolayer Graphene journal July 2008
Edge Nonlinear Optics on a MoS2 Atomic Monolayer journal May 2014
Superconductivity Modulated by Quantum Size Effects journal December 2004
Reduction of the Superconducting Gap of Ultrathin Pb Islands Grown on Si(111) journal May 2009
Superconductivity at the Two-Dimensional Limit journal April 2009
Ferromagnetism in one-dimensional monatomic metal chains journal March 2002
Information Transfer by Vector Spin Chirality in Finite Magnetic Chains journal May 2012
Tunneling through a controllable vacuum gap journal January 1982
Spectroscopy of electronic states of metals with a scanning tunneling microscope journal July 1986
Electron Fringes on a Quantum Wedge journal April 1997
Phase Contribution of Image Potential on Empty Quantum Well States in Pb Islands on the Cu(111) Surface journal May 2009
Supramolecular gratings for tuneable confinement of electrons on metal surfaces journal February 2007
Two-dimensional quantum diffusion of Gd adatoms in nano-size Fe corrals journal February 2013
Self-regulated Gd atom trapping in open Fe nanocorrals journal July 2014
Local density of states from spectroscopic scanning-tunneling-microscope images: Ag(111) journal September 1997
Size-dependent quantum diffusion of Gd atoms within Fe nano-corrals journal December 2013
Electron-beam tip/sample heating device for a scanning tunneling microscopy journal December 2005
Spectroscopy of self-assembled one-dimensional atomic string: The role of step edge journal August 2013
Adsorbates in a Box: Titration of Substrate Electronic States journal August 2010
Surface Electronic Structure of Si (111)-(7×7) Resolved in Real Space journal May 1986
Short-period oscillations in the interlayer magnetic coupling of wedged Fe(100)/Mo(100)/Fe(100) grown on Mo(100) by molecular-beam epitaxy journal March 1992
Electron Confinement to Nanoscale Ag Islands on Ag(111): A Quantitative Study journal April 1998
Controlled Modification of Individual Adsorbate Electronic Structure journal December 2000
Scanning-Tunneling Spectroscopy of Surface-State Electrons Scattered by a Slightly Disordered Two-Dimensional Dilute “Solid”: Ce on Ag(111) journal September 2004
Adatom Self-Organization Induced by Quantum Confinement of Surface Electrons journal November 2006
Optical nonlinearities of small metal particles: surface-mediated resonance and quantum size effects journal January 1986
Information transfer by vector spin chirality in finite magnetic chains text January 2012

Cited By (2)

Quantum corral effects on competing orders and electronic states in chiral d + id or f -wave superconductors journal January 2018
Green's function approach to the Kondo effect in nanosized quantum corrals journal April 2018

Similar Records

Size-dependent quantum diffusion of Gd atoms within Fe nano-corrals
Journal Article · Sun Dec 01 00:00:00 EST 2013 · Surface Science · OSTI ID:1224979

Self-regulated Gd atom trapping in open Fe nanocorrals
Journal Article · Tue Jul 01 00:00:00 EDT 2014 · Physical Review. B, Condensed Matter and Materials Physics · OSTI ID:1224979

Single-atom gating and magnetic interactions in quantum corrals
Journal Article · Sat Apr 01 00:00:00 EDT 2017 · Physical Review B · OSTI ID:1224979