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Title: Resonant tunnelling in a quantum oxide superlattice

Journal Article · · Nature Communications
DOI:https://doi.org/10.1038/ncomms8424· OSTI ID:1190747
 [1];  [2];  [3];  [4];  [5]
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division; Sungkyunkwan Univ., Suwon (Republic of Korea). Dept. of Physics
  2. Sungkyunkwan Univ., Suwon (Republic of Korea). Dept. of Physics; Sungkyunkwan Univ., Suwon (Republic of Korea). Institute of Basic Science
  3. Southern Methodist Univ., Dallas, TX (United States). Department of Mechanical Engineering
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division; Korea Inst. of Science and Technology, Seoul (Korea)
  5. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division

Resonant tunneling is a quantum mechanical process that has long been attracting both scientific and technological attention owing to its intriguing underlying physics and unique applications for high-speed electronics. The materials system exhibiting resonant tunneling, however, has been largely limited to the conventional semiconductors, partially due to their excellent crystalline quality. Here we show that a deliberately designed transition metal oxide superlattice exhibits a resonant tunneling behaviour with a clear negative differential resistance. The tunneling occurred through an atomically thin, lanthanum δ- doped SrTiO3 layer, and the negative differential resistance was realized on top of the bi-polar resistance switching typically observed for perovskite oxide junctions. This combined process resulted in an extremely large resistance ratio (~105) between the high and low resistance states. Lastly, the unprecedentedly large control found in atomically thin δ-doped oxide superlattices can open a door to novel oxide-based high-frequency logic devices.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1190747
Journal Information:
Nature Communications, Vol. 6; ISSN 2041-1723
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 42 works
Citation information provided by
Web of Science

References (39)

Resonant tunneling in semiconductor double barriers journal June 1974
Quantum States of Confined Carriers in Very Thin Al x Ga 1 x As -GaAs- Al x Ga 1 x As Heterostructures journal September 1974
Resonant tunneling diodes: models and properties journal April 1998
Resonant tunneling characteristics in SiO2/Si double-barrier structures in a wide range of applied voltage journal August 2003
Transport processes via localized states in thin a -Si tunnel barriers journal July 1985
Strong polarization enhancement in asymmetric three-component ferroelectric superlattices journal January 2005
Exploiting dimensionality and defect mitigation to create tunable microwave dielectrics journal October 2013
Fractionally δ-Doped Oxide Superlattices for Higher Carrier Mobilities journal January 2012
Theory of Tunneling Spectroscopy of d -Wave Superconductors journal April 1995
Spin-Polarized Intergrain Tunneling in La 2 / 3 Sr 1 / 3 MnO 3 journal September 1996
Role of Metal-Oxide Interface in Determining the Spin Polarization of Magnetic Tunnel Junctions journal October 1999
APPLIED PHYSICS: Tunneling Across a Ferroelectric journal July 2006
Tunneling Electroresistance Induced by Interfacial Phase Transitions in Ultrathin Oxide Heterostructures journal November 2013
Tunnel junctions with multiferroic barriers journal March 2007
Origin of Negative Differential Resistance Observed on Bipolar Resistance Switching Device with Ti/Pr 0.7 Ca 0.3 MnO 3 /Pt Structure journal April 2008
Negative differential resistance induced by Mn substitution at SrRuO 3 / Nb : SrTiO 3 Schottky interfaces journal May 2008
Negative differential resistance in La0.67Ca0.33MnO3−δ∕Nb–SrTiO3 p-n junction journal January 2007
Symmetrical Negative Differential Resistance Behavior of a Resistive Switching Device journal February 2012
Nanoionics-based resistive switching memories journal November 2007
Resistive switching in transition metal oxides journal June 2008
Memristive devices for computing journal January 2013
Atomic Layer Engineering of Perovskite Oxides for Chemically Sharp Heterointerfaces journal October 2012
Artificial charge-modulationin atomic-scale perovskite titanate superlattices journal September 2002
Optical Study of the Free-Carrier Response of LaTiO 3 / SrTiO 3 Superlattices journal December 2007
Nonlinear Hall effect and multichannel conduction in LaTiO 3 / SrTiO 3 superlattices journal November 2010
Transparent conducting oxides: A δ-doped superlattice approach journal August 2014
Transport properties of LaTiO3/SrTiO3 heterostructures journal May 2010
Two-dimensional superconductivity at a Mott insulator/band insulator interface LaTiO3/SrTiO3 journal October 2010
Built-in and induced polarization across LaAlO3/SrTiO3 heterojunctions journal October 2010
Nonvolatile Memory with Multilevel Switching: A Basic Model journal April 2004
Hysteretic current–voltage characteristics and resistance switching at an epitaxial oxide Schottky junction SrRuO3∕SrTi0.99Nb0.01O3 journal January 2005
Comprehensive study of the resistance switching in SrTiO3 and Nb-doped SrTiO3 journal March 2011
Electrode-dependent electrical properties of metal/Nb-doped SrTiO3 junctions journal March 2008
Electrical properties and colossal electroresistance of heteroepitaxial Sr Ru O 3 Sr Ti 1 x Nb x O 3 ( 0.0002 x 0.02 ) Schottky junctions journal April 2007
Resistive switching and resonant tunneling in epitaxial perovskite tunnel barriers journal July 2009
Theory of resonant tunneling in heterostructures journal July 1988
Physics of Semiconductor Devices book January 2007
A Comparative Study on Methods for Convergence Acceleration of Iterative Vector Sequences journal March 1996
Enhanced effective mass in doped SrTiO3 and related perovskites journal August 2009

Cited By (11)

Ferroelectric Tunnel Junctions: Modulations on the Potential Barrier journal October 2019
Nonequilibrium Synthesis of Highly Porous Single-Crystalline Oxide Nanostructures journal January 2017
ZnO composite nanolayer with mobility edge quantization for multi-value logic transistors journal April 2019
Tuning the charge flow between Marcus regimes in an organic thin-film device journal May 2019
Growth control of oxygen stoichiometry in homoepitaxial SrTiO3 films by pulsed laser epitaxy in high vacuum journal January 2016
A multiple negative differential resistance heterojunction device and its circuit application to ternary static random access memory journal January 2020
In-plane rotation and transition from rectification to bipolar resistive switching in ZnO/SrTiO 3 :Nb heterojunctions by substrate pretreatment journal January 2019
Force and light tuning vertical tunneling current in the atomic layered MoS 2 journal May 2018
Tuning the charge flow between Marcus regimes in an organic thin-film device text January 2019
Growth control of oxygen stoichiometry in homoepitaxial SrTiO3 films by pulsed laser epitaxy in high vacuum text January 2016
Phase Instability amid Dimensional Crossover in Artificial Oxide Crystal text January 2019

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